A critical review on graphitic carbon nitride (g-C3N4)-based materials: Preparation, modification and environmental application

•Recent advances in g-C3N4 composites were systematically analyzed and summarized.•Their preparation, characterization, and modification were discussed.•Various applications of g-C3N4 in environmental applications were summarized.•Some concluding remarks and suggestion for future works were proposed...

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Published in	Coordination chemistry reviews Vol. 453; p. 214338
Main Authors	Wang, Jianlong, Wang, Shizong
Format	Journal Article
Language	English
Published	Elsevier B.V 15.02.2022
Subjects	Carbon nitride Disinfectant Environmental application Modification Disinfectant Modification Environmental application Carbon nitride
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Abstract	•Recent advances in g-C3N4 composites were systematically analyzed and summarized.•Their preparation, characterization, and modification were discussed.•Various applications of g-C3N4 in environmental applications were summarized.•Some concluding remarks and suggestion for future works were proposed. Graphitic carbon nitride (g-C3N4)-based materials have received extensive attention due to their unique characteristics, such as optical properties, high chemical stability, facile synthesis. In this review, the recent advances in g-C3N4 composites were systematically analyzed and summarized, including preparation, characterization, modification, and environmental application, particularly focusing on the modification mechanisms and environmental applications. Firstly, the preparation methods of g-C3N4 on the basis of pyrolysis were introduced. Then, the characterization techniques for determining the structure of g-C3N4 and the corresponding specific parameters, such as X diffraction angle and C-N binding energy were briefly introduced. Thirdly, various modification methods of g-C3N4 were discussed. Fourthly, the diverse applications of g-C3N4 in the field of environmental remediation were summarized in detail, such as photo-catalyst, Fenton-like catalyst, adsorbent, and disinfectant. Finally, the concluding remarks and perspectives were made for further study. This review will deepen the understanding of the state of the art of g-C3N4, including the preparation, characterization, modification and environmental application.
AbstractList	•Recent advances in g-C3N4 composites were systematically analyzed and summarized.•Their preparation, characterization, and modification were discussed.•Various applications of g-C3N4 in environmental applications were summarized.•Some concluding remarks and suggestion for future works were proposed. Graphitic carbon nitride (g-C3N4)-based materials have received extensive attention due to their unique characteristics, such as optical properties, high chemical stability, facile synthesis. In this review, the recent advances in g-C3N4 composites were systematically analyzed and summarized, including preparation, characterization, modification, and environmental application, particularly focusing on the modification mechanisms and environmental applications. Firstly, the preparation methods of g-C3N4 on the basis of pyrolysis were introduced. Then, the characterization techniques for determining the structure of g-C3N4 and the corresponding specific parameters, such as X diffraction angle and C-N binding energy were briefly introduced. Thirdly, various modification methods of g-C3N4 were discussed. Fourthly, the diverse applications of g-C3N4 in the field of environmental remediation were summarized in detail, such as photo-catalyst, Fenton-like catalyst, adsorbent, and disinfectant. Finally, the concluding remarks and perspectives were made for further study. This review will deepen the understanding of the state of the art of g-C3N4, including the preparation, characterization, modification and environmental application.
ArticleNumber	214338
Author	Wang, Jianlong Wang, Shizong
Author_xml	– sequence: 1 givenname: Jianlong surname: Wang fullname: Wang, Jianlong email: wangjl@tsinghua.edu.cn organization: Laboratory of Environmental Technology, INET, Tsinghua University, Beijing 100084, PR China – sequence: 2 givenname: Shizong surname: Wang fullname: Wang, Shizong organization: Laboratory of Environmental Technology, INET, Tsinghua University, Beijing 100084, PR China
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Snippet	•Recent advances in g-C3N4 composites were systematically analyzed and summarized.•Their preparation, characterization, and modification were...
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SubjectTerms	Carbon nitride Disinfectant Environmental application Modification
Title	A critical review on graphitic carbon nitride (g-C3N4)-based materials: Preparation, modification and environmental application
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