Graphene-assisted construction of electrocatalysts for carbon dioxide reduction
•Review of graphene-assisted construction strategies of both metal and non-metal based electrocatalysts.•Discussion of CO2RR electrocatalytic performances of various graphene − metal composites.•Overview of enhancement approaches of the graphene-based non-metal CO2RR catalytic activities.•Challenges...
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| Published in | Chemical engineering journal (Lausanne, Switzerland : 1996) Vol. 425; p. 130587 |
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| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.12.2021
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| Subjects | |
| Online Access | Get full text |
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| Abstract | •Review of graphene-assisted construction strategies of both metal and non-metal based electrocatalysts.•Discussion of CO2RR electrocatalytic performances of various graphene − metal composites.•Overview of enhancement approaches of the graphene-based non-metal CO2RR catalytic activities.•Challenges and perspectives for the future development of graphene-based CO2RR electrocatalysts.
The electrochemical conversion of the greenhouse gas, carbon dioxide (CO2), to energy fuels and value-added chemicals presents one of the most valuable approaches to harvest pollutants and produce renewable energy. However, the stable molecular structure of CO2 and the sluggish reaction kinetics make CO2 reduction reaction (CO2RR) formidably challenging to achieve reaction rate and selectivity practical in industry. Graphene and its derivatives have been considered a group of intriguing materials to develop advanced CO2RR electrocatalysts due to their large specific surface area, remarkable electron transfer ability, superior stability, and easy tunability of the structure and surface properties. Herein, we comprehensively discuss the state-of-the-art electrocatalysts constructed with graphene and derivatives for active and selective CO2RR within the recent five years, mainly including the electrocatalysts with both metal-based (e.g., noble, non-noble, or combined thereof) and non-metal (e.g., doped, modified, defected, or composited) catalytic sites. To present the versatile, high-performance metal-based CO2RR electrocatalysts constructed with graphene, we further subdivide them according to the sizes, oxidation states, metal species synergies, dimensionalities, and versatility. Finally, we provide the challenges and perspectives in this emerging area of utilising CO2 to produce various carbon-based fuels and chemicals via graphene chemistry. |
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| AbstractList | •Review of graphene-assisted construction strategies of both metal and non-metal based electrocatalysts.•Discussion of CO2RR electrocatalytic performances of various graphene − metal composites.•Overview of enhancement approaches of the graphene-based non-metal CO2RR catalytic activities.•Challenges and perspectives for the future development of graphene-based CO2RR electrocatalysts.
The electrochemical conversion of the greenhouse gas, carbon dioxide (CO2), to energy fuels and value-added chemicals presents one of the most valuable approaches to harvest pollutants and produce renewable energy. However, the stable molecular structure of CO2 and the sluggish reaction kinetics make CO2 reduction reaction (CO2RR) formidably challenging to achieve reaction rate and selectivity practical in industry. Graphene and its derivatives have been considered a group of intriguing materials to develop advanced CO2RR electrocatalysts due to their large specific surface area, remarkable electron transfer ability, superior stability, and easy tunability of the structure and surface properties. Herein, we comprehensively discuss the state-of-the-art electrocatalysts constructed with graphene and derivatives for active and selective CO2RR within the recent five years, mainly including the electrocatalysts with both metal-based (e.g., noble, non-noble, or combined thereof) and non-metal (e.g., doped, modified, defected, or composited) catalytic sites. To present the versatile, high-performance metal-based CO2RR electrocatalysts constructed with graphene, we further subdivide them according to the sizes, oxidation states, metal species synergies, dimensionalities, and versatility. Finally, we provide the challenges and perspectives in this emerging area of utilising CO2 to produce various carbon-based fuels and chemicals via graphene chemistry. |
| ArticleNumber | 130587 |
| Author | Huang, Yugang Lin, Yinlei Xu, Xuejun Hu, Huawen He, Minghui Zhang, Yuyuan Deng, Lifang Chen, Dongchu Ou, Jian Zhen Zhao, Hong |
| Author_xml | – sequence: 1 givenname: Huawen surname: Hu fullname: Hu, Huawen email: huawenhu@126.com organization: School of Materials Science and Hydrogen Energy, Foshan University, Foshan, Guangdong 528000, China – sequence: 2 givenname: Jian Zhen surname: Ou fullname: Ou, Jian Zhen email: Jianzhen.ou@rmit.edu.au organization: School of Materials Science and Hydrogen Energy, Foshan University, Foshan, Guangdong 528000, China – sequence: 3 givenname: Xuejun surname: Xu fullname: Xu, Xuejun organization: School of Materials Science and Hydrogen Energy, Foshan University, Foshan, Guangdong 528000, China – sequence: 4 givenname: Yinlei surname: Lin fullname: Lin, Yinlei organization: School of Materials Science and Hydrogen Energy, Foshan University, Foshan, Guangdong 528000, China – sequence: 5 givenname: Yuyuan surname: Zhang fullname: Zhang, Yuyuan organization: School of Materials Science and Hydrogen Energy, Foshan University, Foshan, Guangdong 528000, China – sequence: 6 givenname: Hong surname: Zhao fullname: Zhao, Hong organization: School of Materials Science and Hydrogen Energy, Foshan University, Foshan, Guangdong 528000, China – sequence: 7 givenname: Dongchu surname: Chen fullname: Chen, Dongchu organization: School of Materials Science and Hydrogen Energy, Foshan University, Foshan, Guangdong 528000, China – sequence: 8 givenname: Minghui surname: He fullname: He, Minghui organization: State Key Laboratory of Pulp and Paper Engineering, School of Light Industry and Engineering, South China University of Technology, Guangzhou 510640, China – sequence: 9 givenname: Yugang surname: Huang fullname: Huang, Yugang organization: Key Laboratory of Molecular Target and Clinical Pharmacology & School of Pharmaceutical Sciences, Guangzhou Medical University, Guangzhou 511436, China – sequence: 10 givenname: Lifang surname: Deng fullname: Deng, Lifang organization: CAS Key Laboratory of Renewable Energy, Guangzhou Institute of Energy Conversion, Guangzhou, Guangdong 510640, China |
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