Many-body interactions in photo-excited lead iodide perovskite
Lead halide perovskite is emerging as a promising semiconductor material for thin film solar cells. Despite a large number of recent photophysical studies, the nature of photo-excitation in lead halide perovskite remains a subject of debate. Here we use transient absorption spectroscopy to re-examin...
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| Published in | Journal of materials chemistry. A, Materials for energy and sustainability Vol. 3; no. 17; pp. 9285 - 9290 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
01.01.2015
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Lead halide perovskite is emerging as a promising semiconductor material for thin film solar cells. Despite a large number of recent photophysical studies, the nature of photo-excitation in lead halide perovskite remains a subject of debate. Here we use transient absorption spectroscopy to re-examine lead halide perovskite thin films that have been reported to give very high solar cell efficiencies. We focus on many-body interactions that are manifested in (1) the transient Stark effect exerted by hot carriers on subsequent e–h pair generation; and (2) the Auger recombination due to three-body carrier–carrier interactions. These observations establish the dominance of free carriers from above band-gap excitation in lead halide perovskite. We also suggest the effective dynamic screening of charge carriers, likely due to orientational freedom of methylammonium cations in the perovskite lattice, and the presence of negligible charge carrier trapping in lead halide perovskite thin films grown in the presence of chloride precursors. |
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| AbstractList | Lead halide perovskite is emerging as a promising semiconductor material for thin film solar cells. Despite a large number of recent photophysical studies, the nature of photo-excitation in lead halide perovskite remains a subject of debate. Here we use transient absorption spectroscopy to re-examine lead halide perovskite thin films that have been reported to give very high solar cell efficiencies. We focus on many-body interactions that are manifested in (1) the transient Stark effect exerted by hot carriers on subsequent e-h pair generation; and (2) the Auger recombination due to three-body carrier-carrier interactions. These observations establish the dominance of free carriers from above band-gap excitation in lead halide perovskite. We also suggest the effective dynamic screening of charge carriers, likely due to orientational freedom of methylammonium cations in the perovskite lattice, and the presence of negligible charge carrier trapping in lead halide perovskite thin films grown in the presence of chloride precursors. |
| Author | Niesner, Daniel Zhu, X.-Y. Trinh, M. Tuan Wu, Xiaoxi |
| Author_xml | – sequence: 1 givenname: M. Tuan surname: Trinh fullname: Trinh, M. Tuan organization: Department of Chemistry, Columbia University, New York, USA – sequence: 2 givenname: Xiaoxi surname: Wu fullname: Wu, Xiaoxi organization: Department of Chemistry, Columbia University, New York, USA – sequence: 3 givenname: Daniel surname: Niesner fullname: Niesner, Daniel organization: Department of Chemistry, Columbia University, New York, USA – sequence: 4 givenname: X.-Y. surname: Zhu fullname: Zhu, X.-Y. organization: Department of Chemistry, Columbia University, New York, USA |
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| Snippet | Lead halide perovskite is emerging as a promising semiconductor material for thin film solar cells. Despite a large number of recent photophysical studies, the... |
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| SubjectTerms | Carriers cations Charge carriers Chlorides films (materials) Halides lead Perovskites photochemical reactions Photovoltaic cells screening semiconductors Solar cells spectroscopy Thin films |
| Title | Many-body interactions in photo-excited lead iodide perovskite |
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