Super-elastic Scintillating Fibers and Fabrics for Efficient and Visual Radiation Detection
The fabrication of advanced radiation detectors is an important subject due to the wide use of radiation sources in scientific instruments, medical services, security check, non-destructive inspection, and nuclear industries. However, the manufacture of flexible and stretchable radiation detectors r...
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Published in | Advanced fiber materials (Online) Vol. 5; no. 4; pp. 1493 - 1504 |
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Main Authors | , , , , , , , , , |
Format | Journal Article |
Language | English |
Published |
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Springer Nature Singapore
01.08.2023
Springer Nature B.V |
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Abstract | The fabrication of advanced radiation detectors is an important subject due to the wide use of radiation sources in scientific instruments, medical services, security check, non-destructive inspection, and nuclear industries. However, the manufacture of flexible and stretchable radiation detectors remains a challenge. Here, we report the scalable fabrication of super-elastic scintillating fibers and fabrics for visual radiation detection by thermal drawing and melt-spinning methods using styrene-
b
-(ethylene-
co
-butylene)-
b
-styrene, and scintillating Gd
2
O
2
S: Tb (GOS). Microstructure evolution, rheological properties, and radiation–composite interaction are studied to reveal the excellent processability, elasticity, and radiation detection ability of the fabricated fibers. Benefiting from the physical crosslinking structural features of the polymer matrix and the excellent radiation absorption capacities of GOS, the resulting fiber can sustain high strains of 765% with a high content of GOS dopants (2 wt.%) and has excellent X-ray detection performance with the limit down to 53 nGy
air
s
−1
. Furthermore, stretchable fabrics are constructed, and their applications in various fields, such as radiation warning, and X-ray imaging, are demonstrated. Our work not only provides a new type of super-elastic scintillating fibers and fabrics for smart textiles but also demonstrates their potential applications in the nuclear field.
Graphical Abstract |
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AbstractList | The fabrication of advanced radiation detectors is an important subject due to the wide use of radiation sources in scientific instruments, medical services, security check, non-destructive inspection, and nuclear industries. However, the manufacture of flexible and stretchable radiation detectors remains a challenge. Here, we report the scalable fabrication of super-elastic scintillating fibers and fabrics for visual radiation detection by thermal drawing and melt-spinning methods using styrene-
b
-(ethylene-
co
-butylene)-
b
-styrene, and scintillating Gd
2
O
2
S: Tb (GOS). Microstructure evolution, rheological properties, and radiation–composite interaction are studied to reveal the excellent processability, elasticity, and radiation detection ability of the fabricated fibers. Benefiting from the physical crosslinking structural features of the polymer matrix and the excellent radiation absorption capacities of GOS, the resulting fiber can sustain high strains of 765% with a high content of GOS dopants (2 wt.%) and has excellent X-ray detection performance with the limit down to 53 nGy
air
s
−1
. Furthermore, stretchable fabrics are constructed, and their applications in various fields, such as radiation warning, and X-ray imaging, are demonstrated. Our work not only provides a new type of super-elastic scintillating fibers and fabrics for smart textiles but also demonstrates their potential applications in the nuclear field.
Graphical Abstract The fabrication of advanced radiation detectors is an important subject due to the wide use of radiation sources in scientific instruments, medical services, security check, non-destructive inspection, and nuclear industries. However, the manufacture of flexible and stretchable radiation detectors remains a challenge. Here, we report the scalable fabrication of super-elastic scintillating fibers and fabrics for visual radiation detection by thermal drawing and melt-spinning methods using styrene-b-(ethylene-co-butylene)-b-styrene, and scintillating Gd2O2S: Tb (GOS). Microstructure evolution, rheological properties, and radiation–composite interaction are studied to reveal the excellent processability, elasticity, and radiation detection ability of the fabricated fibers. Benefiting from the physical crosslinking structural features of the polymer matrix and the excellent radiation absorption capacities of GOS, the resulting fiber can sustain high strains of 765% with a high content of GOS dopants (2 wt.%) and has excellent X-ray detection performance with the limit down to 53 nGyair s−1. Furthermore, stretchable fabrics are constructed, and their applications in various fields, such as radiation warning, and X-ray imaging, are demonstrated. Our work not only provides a new type of super-elastic scintillating fibers and fabrics for smart textiles but also demonstrates their potential applications in the nuclear field. |
Author | Qiu, Jianrong Lv, Shichao Yan, Yurong Xu, Sijia Du, Minghui Zhou, Shifeng Wang, Jin Qi, Yankun Li, Hongwei Zhang, Zhihao |
Author_xml | – sequence: 1 givenname: Minghui surname: Du fullname: Du, Minghui organization: State Key Laboratory of Luminescent Materials and Devices, School of Materials Science and Engineering, South China University of Technology, Institute of Photonics Technology, Jinan University – sequence: 2 givenname: Jin surname: Wang fullname: Wang, Jin organization: National Engineering Research Center of Novel Equipment for Polymer Processing, School of Mechanical and Automotive Engineering, South China University of Technology – sequence: 3 givenname: Sijia surname: Xu fullname: Xu, Sijia organization: Key Lab Guangdong High Property & Functional Polymer Materials, School of Materials Science and Engineering, South China University of Technology – sequence: 4 givenname: Hongwei surname: Li fullname: Li, Hongwei organization: State Key Laboratory of Luminescent Materials and Devices, School of Materials Science and Engineering, South China University of Technology, Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques, Guangdong Engineering Technology Research and Development Center of Special Optical Fiber Materials and Devices – sequence: 5 givenname: Zhihao surname: Zhang fullname: Zhang, Zhihao organization: State Key Laboratory of Luminescent Materials and Devices, School of Materials Science and Engineering, South China University of Technology, Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques, Guangdong Engineering Technology Research and Development Center of Special Optical Fiber Materials and Devices – sequence: 6 givenname: Yankun surname: Qi fullname: Qi, Yankun organization: State Key Laboratory of Luminescent Materials and Devices, School of Materials Science and Engineering, South China University of Technology, Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques, Guangdong Engineering Technology Research and Development Center of Special Optical Fiber Materials and Devices – sequence: 7 givenname: Shichao surname: Lv fullname: Lv, Shichao email: lvshichao@scut.edu.cn organization: State Key Laboratory of Luminescent Materials and Devices, School of Materials Science and Engineering, South China University of Technology, Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques, Guangdong Engineering Technology Research and Development Center of Special Optical Fiber Materials and Devices – sequence: 8 givenname: Jianrong surname: Qiu fullname: Qiu, Jianrong organization: College of Optical Science and Engineering, State Key Laboratory of Modern Optical Instrumentation, Zhejiang University – sequence: 9 givenname: Yurong surname: Yan fullname: Yan, Yurong email: yryan@scut.edu.cn organization: Key Lab Guangdong High Property & Functional Polymer Materials, School of Materials Science and Engineering, South China University of Technology – sequence: 10 givenname: Shifeng orcidid: 0000-0003-4609-763X surname: Zhou fullname: Zhou, Shifeng email: zhoushifeng@scut.edu.cn organization: State Key Laboratory of Luminescent Materials and Devices, School of Materials Science and Engineering, South China University of Technology, Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques, Guangdong Engineering Technology Research and Development Center of Special Optical Fiber Materials and Devices |
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Cites_doi | 10.1109/TNS2.1960.4315731 10.1016/0029-554X(79)90729-8 10.1038/s41467-019-10351-5 10.1063/1.371107 10.1002/advs.202003728 10.3390/polym12051070 10.1021/acsphotonics.8b00769 10.1016/j.nima.2010.06.196 10.1002/advs.202102439 10.1063/1.5091805 10.1021/cm00045a002 10.1021/acsenergylett.1c00007 10.1201/9781315375199 10.1002/adma.201707251 10.1021/acsami.0c02589 10.1201/9781439819401 10.1021/acsanm.2c01561 10.1038/nphoton.2015.216 10.1002/adma.201802348 10.1016/j.energy.2019.116144 10.1002/adma.201904911 10.3390/s110505112 10.1039/D1MA00569C 10.1016/S0168-9002(00)01031-7 10.1016/j.mattod.2019.11.006 10.1038/s41427-021-00308-w 10.1002/pssb.200304296 10.1016/0029-554X(81)90511-5 10.3390/s21041051 10.1109/TNS.1975.4327617 |
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SubjectTerms | Chemistry and Materials Science Crosslinking Density Electron microscopes Energy Fabrics Materials Engineering Materials Science Melt spinning Nanoscale Science and Technology Polymer Sciences Polymers Radiation absorption Radiation detectors Radiation sources Renewable and Green Energy Research Article Rheological properties Scintillating fibers Smart materials Software Styrenes Temperature Textile Engineering Textiles X ray imagery X-rays |
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Title | Super-elastic Scintillating Fibers and Fabrics for Efficient and Visual Radiation Detection |
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