Magnetic order, spin dynamics and transport properties of the pyrochlore iridate Y2Ir2O7

In the present paper, we report the bulk magnetization, electron-spin-resonance spectra and transport properties of Y2Ir2O7. It is found that Y2Ir2O7 exhibits a magnetic transition at Tc=150K and coexistence of antiferromagnetic and ferromagnetic component due to geometrical frustration. The antifer...

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Published inSolid state communications Vol. 179; pp. 1 - 5
Main Authors Liu, Hui, Tong, Wei, Ling, Langsheng, Zhang, Shile, Zhang, Ranran, Zhang, Lei, Pi, Li, Zhang, Changjin, Zhang, Yuheng
Format Journal Article
LanguageEnglish
Published Elsevier Ltd 01.02.2014
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Abstract In the present paper, we report the bulk magnetization, electron-spin-resonance spectra and transport properties of Y2Ir2O7. It is found that Y2Ir2O7 exhibits a magnetic transition at Tc=150K and coexistence of antiferromagnetic and ferromagnetic component due to geometrical frustration. The antiferromagnetic order is due to Ir–O–Ir superexchange interactions and the ferromagnetic component is caused by canting of the moments from the antiferromagnetic state. The behavior of spin dynamics confirms that antiferromagnetic ordering with all-in/all-out structure is responsible for the existence of ferromagnetic component. The resistivity reveals that this compound is a semiconductor and the variable-range hopping process dominates the transport mechanism. •Y2Ir2O7 exhibits coexistence of antiferromagnetic and ferromagnetic component due to geometrical frustration.•AFM ordering with all-in/all-out structure is responsible for the existence of FM component.•This compound is a semiconductor and the variable-range hopping process dominates the transport mechanism in the range of the whole temperature measured.
AbstractList In the present paper, we report the bulk magnetization, electron-spin-resonance spectra and transport properties of Y2Ir2O7. It is found that Y2Ir2O7 exhibits a magnetic transition at Tc=150K and coexistence of antiferromagnetic and ferromagnetic component due to geometrical frustration. The antiferromagnetic order is due to Ir–O–Ir superexchange interactions and the ferromagnetic component is caused by canting of the moments from the antiferromagnetic state. The behavior of spin dynamics confirms that antiferromagnetic ordering with all-in/all-out structure is responsible for the existence of ferromagnetic component. The resistivity reveals that this compound is a semiconductor and the variable-range hopping process dominates the transport mechanism. •Y2Ir2O7 exhibits coexistence of antiferromagnetic and ferromagnetic component due to geometrical frustration.•AFM ordering with all-in/all-out structure is responsible for the existence of FM component.•This compound is a semiconductor and the variable-range hopping process dominates the transport mechanism in the range of the whole temperature measured.
Author Tong, Wei
Zhang, Yuheng
Pi, Li
Ling, Langsheng
Liu, Hui
Zhang, Shile
Zhang, Ranran
Zhang, Lei
Zhang, Changjin
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D. Variable-range hopping
A. Pyrochlore
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Snippet In the present paper, we report the bulk magnetization, electron-spin-resonance spectra and transport properties of Y2Ir2O7. It is found that Y2Ir2O7 exhibits...
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SubjectTerms A. Pyrochlore
D. Geometrical frustration
D. Spin–orbit coupling
D. Variable-range hopping
Title Magnetic order, spin dynamics and transport properties of the pyrochlore iridate Y2Ir2O7
URI https://dx.doi.org/10.1016/j.ssc.2013.11.004
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