Coordination-driven strategy towards crystalline hybrid photochromic materials via the marriage of a non-photochromic extended dipyridine unit and zincophosphate
The coordinative linkage of supramolecular zincophosphate building units and an extended dipyridine unit, 1,4-di(pyridine-4-yl)benzene (bpyb), generates two hybrid photochromic frames. The structural and photochromic diversities were mainly attributable to the distinct coordination mode of bpyb in t...
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| Published in | Journal of materials chemistry. C, Materials for optical and electronic devices Vol. 7; no. 13; pp. 3920 - 3923 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Cambridge
Royal Society of Chemistry
2019
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| Subjects | |
| Online Access | Get full text |
| ISSN | 2050-7526 2050-7534 |
| DOI | 10.1039/C9TC00851A |
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| Abstract | The coordinative linkage of supramolecular zincophosphate building units and an extended dipyridine unit, 1,4-di(pyridine-4-yl)benzene (bpyb), generates two hybrid photochromic frames. The structural and photochromic diversities were mainly attributable to the distinct coordination mode of bpyb in the resultant structure. Different from most of the reported photochromic materials driven by photochromically active units, the crystalline hybrid photochromic materials in this work are decorated by non-photochromic bpyb. The metal-assisted phosphate-to-bpyb charge transfer is responsible for the photochromism. Our work provides a new perspective to develop photochromic hybrid materials based on non-photochromic moieties. |
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| AbstractList | The coordinative linkage of supramolecular zincophosphate building units and an extended dipyridine unit, 1,4-di(pyridine-4-yl)benzene (bpyb), generates two hybrid photochromic frames. The structural and photochromic diversities were mainly attributable to the distinct coordination mode of bpyb in the resultant structure. Different from most of the reported photochromic materials driven by photochromically active units, the crystalline hybrid photochromic materials in this work are decorated by non-photochromic bpyb. The metal-assisted phosphate-to-bpyb charge transfer is responsible for the photochromism. Our work provides a new perspective to develop photochromic hybrid materials based on non-photochromic moieties. |
| Author | Wang, Guo-Ming Han, Song-De Wei, Qi Ge, Bang-Di Li, Jin-Hua |
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| Title | Coordination-driven strategy towards crystalline hybrid photochromic materials via the marriage of a non-photochromic extended dipyridine unit and zincophosphate |
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