Evaluation of magnetic material IIP@GO-Fe3O4 based on Kesambi wood (Schleichera oleosa) as a potential adsorbent for the removal of Cr(VI) from aqueous solutions

Magnetic composite material modified ion imprinting polymer (IIP@GO-Fe3O4) based on GO from kesambi wood (Schleichera oleosa)was successfully synthesized by using a precipitation method. The physico-chemical characterization uses XRD, FTIR, BET-BJH and SEM-EDX. IIP@GO-Fe3O4 was applied to adsorb Cr(...

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Published inReactive & functional polymers Vol. 166; p. 105000
Main Authors Neolaka, Yantus A.B., Lawa, Yosep, Naat, Johnson, Riwu, Arsel A.P., Lindu, Yeskiel E., Darmokoesoemo, Handoko, Widyaningrum, Bernadeta Ayu, Iqbal, Munawar, Kusuma, Heri Septya
Format Journal Article
LanguageEnglish
Published Amsterdam Elsevier B.V 01.09.2021
Elsevier BV
Subjects
Adsorbents
Adsorption
Adsorptivity
Aqueous solutions
Chemical precipitation
Composite materials
Graphene-oxide magnetic (GO-Fe3O4)
Hexavalent chromium
Imprinting polymer
Iron oxides
Magnetic materials
Polymer matrix composites
Polymers
Selectivity
Studies
Wastewater
Water sampling
Hexavalent chromium
Imprinting polymer
Adsorption
Wastewater
Graphene-oxide magnetic (GO-Fe3O4)
Online AccessGet full text
ISSN1381-5148
1873-166X
DOI10.1016/j.reactfunctpolym.2021.105000

Cover

Abstract Magnetic composite material modified ion imprinting polymer (IIP@GO-Fe3O4) based on GO from kesambi wood (Schleichera oleosa)was successfully synthesized by using a precipitation method. The physico-chemical characterization uses XRD, FTIR, BET-BJH and SEM-EDX. IIP@GO-Fe3O4 was applied to adsorb Cr(VI) from the water sample by utilizing the batch system. Various adsorption parameters for Cr(VI) such as adsorbent mass, pH, contact time and temperature were optimized in this investigation. The Cr(VI) maximum adsorption occurred when the adsorbent mass usage 0.04 g, pH 2, 40 min of contacts and at the temperature of 323 K. In this study ten kinetic and eight isothermal adsorption models were used to investigate the adsorption mechanism of Cr(VI) onto IIP@GO-Fe3O4. The kinetic modelling shows that the adsorption of Cr(VI) onto IIP@GO-Fe3O4 corresponds to the pseudo-second-order (PSO) model, while the adsorption isotherm corresponds to the Dubinin-Radushkevich (DKR) model with an adsorption capacity of 8.502 mg/g. The thermodynamic study has shown that the adsorption process can take place at a temperature of 323 K. The result showed that a higher adsorption selectivity on IIP@GO-Fe3O4 compares to NIP@GO-Fe3O4. The adsorbent materials gave better reusability because their adsorptive capacity remained at the same level (although it was used at least ten times). [Display omitted] •IIP@GO-Fe3O4 based on kesambi wood (Schleichera oleosa) was successfully synthesized;•The magnetic composite material showed good adsorption ability of Cr(VI);•The kinetic and isotherm modellings are based on the pseudo-second-order (PSO) and Dubinin-Radushkevich (DKR) models;•The IIP@GO-Fe3O4 material has a high adsorption selectivity toward Cr(VI);•The material IIP@GO-Fe3O4 has shown a sufficient reusability factor for the adsorption of Cr(VI)
AbstractList Magnetic composite material modified ion imprinting polymer (IIP@GO-Fe3O4) based on GO from kesambi wood (Schleichera oleosa) was successfully synthesized by using a precipitation method. The physico-chemical characterization uses XRD, FTIR, BET-BJH and SEM-EDX. IIP@GO-Fe3O4 was applied to adsorb Cr(VI) from the water sample by utilizing the batch system. Various adsorption parameters for Cr(VI) such as adsorbent mass, pH, contact time and temperature were optimized in this investigation. The Cr(VI) maximum adsorption occurred when the adsorbent mass usage 0.04 g, pH 2, 40 min of contacts and at the temperature of 323 K. In this study ten kinetic and eight isothermal adsorption models were used to investigate the adsorption mechanism of Cr(VI) onto IIP@GO-Fe3O4. The kinetic modelling shows that the adsorption of Cr(VI) onto IIP@GO-Fe3O4 corresponds to the pseudo-second-order (PSO) model, while the adsorption isotherm corresponds to the Dubinin-Radushkevich (DKR) model with an adsorption capacity of 8.502 mg/g. The thermodynamic study has shown that the adsorption process can take place at a temperature of 323 K. The result showed that a higher adsorption selectivity on IIP@GO-Fe3O4 compares to NIP@GO-Fe3O4. The adsorbent materials gave better reusability because their adsorptive capacity remained at the same level (although it was used at least ten times).
Magnetic composite material modified ion imprinting polymer (IIP@GO-Fe3O4) based on GO from kesambi wood (Schleichera oleosa)was successfully synthesized by using a precipitation method. The physico-chemical characterization uses XRD, FTIR, BET-BJH and SEM-EDX. IIP@GO-Fe3O4 was applied to adsorb Cr(VI) from the water sample by utilizing the batch system. Various adsorption parameters for Cr(VI) such as adsorbent mass, pH, contact time and temperature were optimized in this investigation. The Cr(VI) maximum adsorption occurred when the adsorbent mass usage 0.04 g, pH 2, 40 min of contacts and at the temperature of 323 K. In this study ten kinetic and eight isothermal adsorption models were used to investigate the adsorption mechanism of Cr(VI) onto IIP@GO-Fe3O4. The kinetic modelling shows that the adsorption of Cr(VI) onto IIP@GO-Fe3O4 corresponds to the pseudo-second-order (PSO) model, while the adsorption isotherm corresponds to the Dubinin-Radushkevich (DKR) model with an adsorption capacity of 8.502 mg/g. The thermodynamic study has shown that the adsorption process can take place at a temperature of 323 K. The result showed that a higher adsorption selectivity on IIP@GO-Fe3O4 compares to NIP@GO-Fe3O4. The adsorbent materials gave better reusability because their adsorptive capacity remained at the same level (although it was used at least ten times). [Display omitted] •IIP@GO-Fe3O4 based on kesambi wood (Schleichera oleosa) was successfully synthesized;•The magnetic composite material showed good adsorption ability of Cr(VI);•The kinetic and isotherm modellings are based on the pseudo-second-order (PSO) and Dubinin-Radushkevich (DKR) models;•The IIP@GO-Fe3O4 material has a high adsorption selectivity toward Cr(VI);•The material IIP@GO-Fe3O4 has shown a sufficient reusability factor for the adsorption of Cr(VI)
ArticleNumber 105000
Author Iqbal, Munawar
Riwu, Arsel A.P.
Widyaningrum, Bernadeta Ayu
Lawa, Yosep
Lindu, Yeskiel E.
Naat, Johnson
Darmokoesoemo, Handoko
Neolaka, Yantus A.B.
Kusuma, Heri Septya
Author_xml – sequence: 1
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  organization: Department of Chemical Education, Faculty of Education and Teachers Training, University of Nusa Cendana, Kupang, Nusa Tenggara Timur, 85001, Indonesia
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  surname: Lawa
  fullname: Lawa, Yosep
  organization: Department of Chemical Education, Faculty of Education and Teachers Training, University of Nusa Cendana, Kupang, Nusa Tenggara Timur, 85001, Indonesia
– sequence: 3
  givenname: Johnson
  surname: Naat
  fullname: Naat, Johnson
  organization: Department of Chemical Education, Faculty of Education and Teachers Training, University of Nusa Cendana, Kupang, Nusa Tenggara Timur, 85001, Indonesia
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  surname: Riwu
  fullname: Riwu, Arsel A.P.
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  givenname: Yeskiel E.
  surname: Lindu
  fullname: Lindu, Yeskiel E.
  organization: Analytical Chemistry Research Group, Department of Chemical Education, Faculty of Education and Teachers Training, University of Nusa Cendana, Kupang 85001, Nusa Tenggara Timur, Indonesia
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  surname: Darmokoesoemo
  fullname: Darmokoesoemo, Handoko
  email: handoko.darmokoesoemo@gmail.com
  organization: Department of Chemistry, Faculty of Science and Technology, Airlangga University, Mulyorejo, Surabaya 60115, Indonesia
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  givenname: Bernadeta Ayu
  surname: Widyaningrum
  fullname: Widyaningrum, Bernadeta Ayu
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  givenname: Heri Septya
  surname: Kusuma
  fullname: Kusuma, Heri Septya
  email: heriseptyakusuma@gmail.com
  organization: Department of Chemical Engineering, Faculty of Industrial Technology, Universitas Pembangunan Nasional "Veteran" Yogyakarta, Indonesia
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Keywords Hexavalent chromium
Imprinting polymer
Adsorption
Wastewater
Graphene-oxide magnetic (GO-Fe3O4)
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Snippet Magnetic composite material modified ion imprinting polymer (IIP@GO-Fe3O4) based on GO from kesambi wood (Schleichera oleosa)was successfully synthesized by...
Magnetic composite material modified ion imprinting polymer (IIP@GO-Fe3O4) based on GO from kesambi wood (Schleichera oleosa) was successfully synthesized by...
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SubjectTerms Adsorbents
Adsorption
Adsorptivity
Aqueous solutions
Chemical precipitation
Composite materials
Graphene-oxide magnetic (GO-Fe3O4)
Hexavalent chromium
Imprinting polymer
Iron oxides
Magnetic materials
Polymer matrix composites
Polymers
Selectivity
Studies
Wastewater
Water sampling
Title Evaluation of magnetic material IIP@GO-Fe3O4 based on Kesambi wood (Schleichera oleosa) as a potential adsorbent for the removal of Cr(VI) from aqueous solutions
URI https://dx.doi.org/10.1016/j.reactfunctpolym.2021.105000
https://www.proquest.com/docview/2581066870
Volume 166
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