Theoretical and experimental investigations of coherent phonon dynamics in sapphire crystal using femtosecond time-resolved coherent anti-Stokes Raman scattering
We report on the theoretical and the experimental investigations of the coherent phonon dynamics in sapphire crystal using the femtosecond time-resolved coherent anti-Stokes Raman scattering （fs-CARS） technique. The temporal chirped white-light continuum （WLC） is used for the Stokes pulse, therefore...
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| Published in | Chinese physics B Vol. 20; no. 12; pp. 315 - 321 |
|---|---|
| Main Author | |
| Format | Journal Article |
| Language | English |
| Published |
IOP Publishing
01.12.2011
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1674-1056 2058-3834 |
| DOI | 10.1088/1674-1056/20/12/126301 |
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| Abstract | We report on the theoretical and the experimental investigations of the coherent phonon dynamics in sapphire crystal using the femtosecond time-resolved coherent anti-Stokes Raman scattering （fs-CARS） technique. The temporal chirped white-light continuum （WLC） is used for the Stokes pulse, therefore we can perform the selective excitation of the phonon modes without using a complicated laser system. The expected quantum beat phenomenon is clearly observed. The theoretical formulas consist very well with the experimental results. The dephasing times of the excited phonon modes, the wavenumber difference, and the phase shift between the simultaneously excited modes are obtained and discussed. This work opens up a way to study directly high-frequency coherent phonon dynamics in bulk crystals on a femtosecond time scale and is especially helpful for understanding the nature of coherent phonons. |
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| AbstractList | We report on the theoretical and the experimental investigations of the coherent phonon dynamics in sapphire crystal using the femtosecond time-resolved coherent anti-Stokes Raman scattering （fs-CARS） technique. The temporal chirped white-light continuum （WLC） is used for the Stokes pulse, therefore we can perform the selective excitation of the phonon modes without using a complicated laser system. The expected quantum beat phenomenon is clearly observed. The theoretical formulas consist very well with the experimental results. The dephasing times of the excited phonon modes, the wavenumber difference, and the phase shift between the simultaneously excited modes are obtained and discussed. This work opens up a way to study directly high-frequency coherent phonon dynamics in bulk crystals on a femtosecond time scale and is especially helpful for understanding the nature of coherent phonons. |
| Author | 杜鑫 张明福 何兴 孟庆琨 宋云飞 杨延强 韩杰才 |
| AuthorAffiliation | Centre for Condensed Matter Science and Technology, Department of Physics, Harbin Institute of Technology, Harbin 150080, China College of Foundation Science, Harbin University of Commerce, Harbin 150028, China Centre for Composite Materials, Harbin Institute of Technology, Harbin 150080, China |
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| Cites_doi | 10.1016/S1386-1425(98)00312-6 10.1063/1.104462 10.1002/(SICI)1097-4555(200001/02)31:1/2<33::AID-JRS494>3.0.CO;2-H 10.1016/S0026-2692(01)00087-8 10.1364/OE.18.022937 10.1002/jrs.741 10.1016/S0009-2614(97)01262-1 10.7498/aps.59.5406 10.1063/1.1567827 10.1088/1674-1056/20/1/014206 10.1103/PhysRevLett.79.5102 10.1088/1674-1056/19/4/043201 10.1063/1.1554765 10.1103/PhysRevLett.77.3661 10.1002/crat.200711066 10.1103/PhysRevB.45.768 10.1063/1.1818741 10.1088/1674-1056/18/4/029 10.1021/jp9832589 10.1002/jrs.1482 10.1021/jp972213p 10.1103/PhysRevB.58.5448 10.1103/PhysRevLett.65.764 10.1063/1.1578179 10.1103/RevModPhys.50.607 |
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| DocumentTitleAlternate | Theoretical and experimental investigations of coherent phonon dynamics in sapphire crystal using femtosecond time-resolved coherent anti-Stokes Raman scattering |
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| Notes | We report on the theoretical and the experimental investigations of the coherent phonon dynamics in sapphire crystal using the femtosecond time-resolved coherent anti-Stokes Raman scattering （fs-CARS） technique. The temporal chirped white-light continuum （WLC） is used for the Stokes pulse, therefore we can perform the selective excitation of the phonon modes without using a complicated laser system. The expected quantum beat phenomenon is clearly observed. The theoretical formulas consist very well with the experimental results. The dephasing times of the excited phonon modes, the wavenumber difference, and the phase shift between the simultaneously excited modes are obtained and discussed. This work opens up a way to study directly high-frequency coherent phonon dynamics in bulk crystals on a femtosecond time scale and is especially helpful for understanding the nature of coherent phonons. 11-5639/O4 coherent phonon, femtosecond time-resolved coherent anti-Stokes Raman scattering, dephasing, quantum beat |
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| References | 23 24 25 26 Yin J (18) 2011; 20 10 Yu L Y (27) 2010; 59 12 13 14 Wang Y H (11) 2009; 18 15 16 17 19 Mukamel S (21) 1995 1 2 3 4 5 6 7 8 9 Zhang S A (22) 2010; 19 Shen Y R (20) 1984 |
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| Title | Theoretical and experimental investigations of coherent phonon dynamics in sapphire crystal using femtosecond time-resolved coherent anti-Stokes Raman scattering |
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