N-Alkoxymethylation of heterocyclic compounds with diethyl phosphite via cleavage of P–O bond
N-Alkoxymethylation of heterocyclic compounds with diethyl phosphite via cleavage of P–O bond was investigated and a series of N3-ethoxymethylated heterocyclic compounds were synthesized. A mechanism in which diethyl phosphite acts as an efficient surrogate of ethanol was proposed and supported by s...
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Published in | Tetrahedron Vol. 67; no. 13; pp. 2462 - 2467 |
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Main Authors | , , , , , |
Format | Journal Article |
Language | English |
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01.04.2011
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Abstract | N-Alkoxymethylation of heterocyclic compounds with diethyl phosphite via cleavage of P–O bond was investigated and a series of
N3-ethoxymethylated heterocyclic compounds were synthesized. A mechanism in which diethyl phosphite acts as an efficient surrogate of ethanol was proposed and supported by several evidences.
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AbstractList | N-Alkoxymethylation of heterocyclic compounds with diethyl phosphite via cleavage of P–O bond was investigated and a series of
N3-ethoxymethylated heterocyclic compounds were synthesized. A mechanism in which diethyl phosphite acts as an efficient surrogate of ethanol was proposed and supported by several evidences.
[Display omitted] N-Alkoxymethylation of heterocyclic compounds with diethyl phosphite via cleavage of P-O bond was investigated and a series of N3-ethoxymethylated heterocyclic compounds were synthesized. A mechanism in which diethyl phosphite acts as an efficient surrogate of ethanol was proposed and supported by several evidences. (C) 2011 Elsevier Ltd. All rights reserved. N-Alkoxymethylation of heterocyclic compounds with diethyl phosphite via cleavage of P-O bond was investigated and a series of N3-ethoxymethylated heterocyclic compounds were synthesized. A mechanism in which diethyl phosphite acts as an efficient surrogate of ethanol was proposed and supported by several evidences. |
Author | Da, Yu-Xia Ren, Rong-Guo Quan, Zheng-Jun Jia, Xiao-Dong Wang, Xi-Cun Zhang, Zhang |
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Keywords | GIDSJYAVUXNYDJ-UHFFFAOYSA-N N-Alkylation SXWPJKGXMOJYOP-UHFFFAOYSA-N YNUSNAMYYOEJON-UHFFFAOYSA-N WOFYKUQBJSSXNP-UHFFFAOYSA-N DRQQEKOMTUWUOT-UHFFFAOYSA-N P–O cleavage TUOSAVVUMNXEOZ-UHFFFAOYSA-N MTIWEZWOLZINJW-UHFFFAOYSA-N FEXSMYHVMRFNJF-UHFFFAOYSA-N BCLCTNFGMGONNN-UHFFFAOYSA-N VFILUPWGBQBLTG-UHFFFAOYSA-N YJBCMGOBQZRKEP-UHFFFAOYSA-N BBHQISMLUGXQOW-UHFFFAOYSA-N QFVKMKADINJBDL-UHFFFAOYSA-N MNSGOOCAMMSKGI-UHFFFAOYSA-N Diethyl phosphite N3-Substituted dihydropyrimidinones AVKMPYLSTJCGML-UHFFFAOYSA-N VAJJXKGFPILYBO-UHFFFAOYSA-N BECSINOJAUIXPT-UHFFFAOYSA-N XUWMZOOSKGGZNW-UHFFFAOYSA-N LGIKGKXCBQZOLN-UHFFFAOYSA-N BINOL P O cleavage BIGINELLI-TYPE ALPHA-AMINO ENANTIOSELECTIVE SYNTHESIS ACIDS EFFICIENT SYNTHESIS ALDEHYDES ASYMMETRIC HYDROPHOSPHONYLATION MICHAEL ADDITION PHOSPHONATES Ethanol Nitrogen heterocycle Alkoxycarbonylation Pyrimidone derivatives Alkylation Azides P―O cleavage Reaction mechanism Cleavage Chemical synthesis |
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Snippet | N-Alkoxymethylation of heterocyclic compounds with diethyl phosphite via cleavage of P–O bond was investigated and a series of
N3-ethoxymethylated heterocyclic... N-Alkoxymethylation of heterocyclic compounds with diethyl phosphite via cleavage of P-O bond was investigated and a series of N3-ethoxymethylated heterocyclic... |
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SubjectTerms | Bonding Chemistry Chemistry, Organic Cleavage Diethyl phosphite Ethanol Ethyl alcohol Exact sciences and technology Heterocyclic compounds Heterocyclic compounds with several n hetero atoms in the same ring, in separated rings or in fused rings Inorganic salts Kinetics and mechanisms N-Alkylation N3-Substituted dihydropyrimidinones Organic chemistry Physical Sciences Preparations and properties P–O cleavage Reactivity and mechanisms Science & Technology Tetrahedrons |
Title | N-Alkoxymethylation of heterocyclic compounds with diethyl phosphite via cleavage of P–O bond |
URI | https://dx.doi.org/10.1016/j.tet.2011.01.061 http://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcApp=Summon&SrcAuth=ProQuest&DestApp=WOS&DestLinkType=FullRecord&UT=000288841300012 https://search.proquest.com/docview/1744674058 |
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