Impact of solid-electrolyte interphase layer thickness on lithium-ion battery cell surface temperature
The widely used non-destructive battery characterization techniques, such as voltage, capacity, and impedance measurements, often fail to fully characterise a discarded lithium-ion battery when reuse of spent battery is envisaged. Here we propose a tool that uses the surface temperature of a pouch c...
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| Published in | Journal of power sources Vol. 525; p. 231126 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
30.03.2022
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| Subjects | |
| Online Access | Get full text |
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| Abstract | The widely used non-destructive battery characterization techniques, such as voltage, capacity, and impedance measurements, often fail to fully characterise a discarded lithium-ion battery when reuse of spent battery is envisaged. Here we propose a tool that uses the surface temperature of a pouch cell to measure the thickness of the solid-electrolyte-interphase (SEI) layer, which is often attributed as one of the main causes of lithium-ion battery degradation at 0.1C–1C discharge rates in ambient conditions. A 2D multiphysics coupled electrochemical-thermal continuum model and a 3D thermal model have been developed to investigate the changes in the surface temperature of a lithium-ion pouch cell with varying SEI layer thicknesses. Present modelling results show that the cell surface temperature changes due to significant SEI layer heat generation at several discharge rates. Furthermore, the temperature change has also been subject to different cooling conditions and particle sizes. The present results provide a reference to making decisions on battery reuse by providing a correlation between the SEI layer thickness with the surface temperature of the cell and inform future research on thermal runaway as a thicker SEI layer can decrease the onset temperature of thermal runaway.
•Battery temperature changes due to significant solid-electrolyte-interphase heat.•Anode particle size changed the thermal impact of the solid-electrolyte-interphase.•Thermal impact of the solid-electrolyte-interphase depends on depth-of-discharge. |
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| AbstractList | The widely used non-destructive battery characterization techniques, such as voltage, capacity, and impedance measurements, often fail to fully characterise a discarded lithium-ion battery when reuse of spent battery is envisaged. Here we propose a tool that uses the surface temperature of a pouch cell to measure the thickness of the solid-electrolyte-interphase (SEI) layer, which is often attributed as one of the main causes of lithium-ion battery degradation at 0.1C–1C discharge rates in ambient conditions. A 2D multiphysics coupled electrochemical-thermal continuum model and a 3D thermal model have been developed to investigate the changes in the surface temperature of a lithium-ion pouch cell with varying SEI layer thicknesses. Present modelling results show that the cell surface temperature changes due to significant SEI layer heat generation at several discharge rates. Furthermore, the temperature change has also been subject to different cooling conditions and particle sizes. The present results provide a reference to making decisions on battery reuse by providing a correlation between the SEI layer thickness with the surface temperature of the cell and inform future research on thermal runaway as a thicker SEI layer can decrease the onset temperature of thermal runaway.
•Battery temperature changes due to significant solid-electrolyte-interphase heat.•Anode particle size changed the thermal impact of the solid-electrolyte-interphase.•Thermal impact of the solid-electrolyte-interphase depends on depth-of-discharge. |
| ArticleNumber | 231126 |
| Author | Andriunas, Ignas Wade, Neal Milojevic, Zoran Das, Prodip K. |
| Author_xml | – sequence: 1 givenname: Ignas orcidid: 0000-0001-7483-7733 surname: Andriunas fullname: Andriunas, Ignas email: ignas.andriunas@outlook.com organization: School of Engineering, Newcastle University, Newcastle upon Tyne, NE1 7RU, UK – sequence: 2 givenname: Zoran surname: Milojevic fullname: Milojevic, Zoran organization: School of Engineering, Newcastle University, Newcastle upon Tyne, NE1 7RU, UK – sequence: 3 givenname: Neal surname: Wade fullname: Wade, Neal organization: School of Engineering, Newcastle University, Newcastle upon Tyne, NE1 7RU, UK – sequence: 4 givenname: Prodip K. orcidid: 0000-0001-9096-3721 surname: Das fullname: Das, Prodip K. organization: School of Engineering, Newcastle University, Newcastle upon Tyne, NE1 7RU, UK |
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| Keywords | Lithium-ion battery Temperature Heat Modelling Pouch cell Solid-electrolyte-interphase |
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| SubjectTerms | Heat Lithium-ion battery Modelling Pouch cell Solid-electrolyte-interphase Temperature |
| Title | Impact of solid-electrolyte interphase layer thickness on lithium-ion battery cell surface temperature |
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