Lithiophilic N-doped carbon bowls induced Li deposition in layered graphene film for advanced lithium metal batteries
Lithium (Li) metal with high theoretical capacity and low electrochemical potential is the most ideal anode for next-generation high-energy batteries. However, the practical implementation of Li anode has been hindered by dendritic growth and volume expansion during cycling, which results in low Cou...
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| Published in | Nano research Vol. 15; no. 1; pp. 352 - 360 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Beijing
Tsinghua University Press
01.01.2022
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Lithium (Li) metal with high theoretical capacity and low electrochemical potential is the most ideal anode for next-generation high-energy batteries. However, the practical implementation of Li anode has been hindered by dendritic growth and volume expansion during cycling, which results in low Coulombic efficiency (CE), short lifespan, and safety hazards. Here, we report a highly stable and dendrite-free Li metal anode by utilizing N-doped hollow porous bowl-like hard carbon/reduced graphene nanosheets (CB@rGO) hybrids as three-dimensional (3D) conductive and lithiophilic scaffold host. The lithiophilic carbon bowl (CB) mainly works as excellent guides during the Li plating process, whereas the rGO layer with high conductivity and mechanical stability maintains the integrity of the composite by confining the volume change in long-range order during cycling. Moreover, the local current density can be reduced due to the 3D conductive framework. Therefore, CB@rGO presents a low lithium metal nucleation overpotential of 18 mV, high CE of 98%, and stable cycling without obvious voltage fluctuation for over 600 cycles at a current density of 1 mA·cm
−2
. Our study not only provides a good CB@rGO host and pre-Lithiated CB@rGO composite anode electrode, but also brings a new strategy of designing 3D electrodes for those active materials suffering from severe volume expansion. |
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| AbstractList | Lithium (Li) metal with high theoretical capacity and low electrochemical potential is the most ideal anode for next-generation high-energy batteries. However, the practical implementation of Li anode has been hindered by dendritic growth and volume expansion during cycling, which results in low Coulombic efficiency (CE), short lifespan, and safety hazards. Here, we report a highly stable and dendrite-free Li metal anode by utilizing N-doped hollow porous bowl-like hard carbon/reduced graphene nanosheets (CB@rGO) hybrids as three-dimensional (3D) conductive and lithiophilic scaffold host. The lithiophilic carbon bowl (CB) mainly works as excellent guides during the Li plating process, whereas the rGO layer with high conductivity and mechanical stability maintains the integrity of the composite by confining the volume change in long-range order during cycling. Moreover, the local current density can be reduced due to the 3D conductive framework. Therefore, CB@rGO presents a low lithium metal nucleation overpotential of 18 mV, high CE of 98%, and stable cycling without obvious voltage fluctuation for over 600 cycles at a current density of 1 mA·cm
−2
. Our study not only provides a good CB@rGO host and pre-Lithiated CB@rGO composite anode electrode, but also brings a new strategy of designing 3D electrodes for those active materials suffering from severe volume expansion. Lithium (Li) metal with high theoretical capacity and low electrochemical potential is the most ideal anode for next-generation high-energy batteries. However, the practical implementation of Li anode has been hindered by dendritic growth and volume expansion during cycling, which results in low Coulombic efficiency (CE), short lifespan, and safety hazards. Here, we report a highly stable and dendrite-free Li metal anode by utilizing N-doped hollow porous bowl-like hard carbon/reduced graphene nanosheets (CB@rGO) hybrids as three-dimensional (3D) conductive and lithiophilic scaffold host. The lithiophilic carbon bowl (CB) mainly works as excellent guides during the Li plating process, whereas the rGO layer with high conductivity and mechanical stability maintains the integrity of the composite by confining the volume change in long-range order during cycling. Moreover, the local current density can be reduced due to the 3D conductive framework. Therefore, CB@rGO presents a low lithium metal nucleation overpotential of 18 mV, high CE of 98%, and stable cycling without obvious voltage fluctuation for over 600 cycles at a current density of 1 mA·cm−2. Our study not only provides a good CB@rGO host and pre-Lithiated CB@rGO composite anode electrode, but also brings a new strategy of designing 3D electrodes for those active materials suffering from severe volume expansion. |
| Author | Wu, Hong-Hui He, Xin Świętosławski, Michał Gao, Biao Feng, Xiaoyu Zhang, Qiaobao |
| Author_xml | – sequence: 1 givenname: Xiaoyu surname: Feng fullname: Feng, Xiaoyu organization: Department of Materials Science and Engineering, College of Materials, Xiamen University, The State Key Laboratory of Refractories and Metallurgy and Institute of Advanced Materials and Nanotechnology, Wuhan University of Science and Technology – sequence: 2 givenname: Hong-Hui surname: Wu fullname: Wu, Hong-Hui organization: School of Materials Science and Engineering, University of Science and Technology Beijing – sequence: 3 givenname: Biao surname: Gao fullname: Gao, Biao organization: The State Key Laboratory of Refractories and Metallurgy and Institute of Advanced Materials and Nanotechnology, Wuhan University of Science and Technology – sequence: 4 givenname: Michał surname: Świętosławski fullname: Świętosławski, Michał organization: Faculty of Chemistry, Jagiellonian University – sequence: 5 givenname: Xin surname: He fullname: He, Xin email: xinhe@scu.edu.cn organization: School of Chemical Engineering, Sichuan University – sequence: 6 givenname: Qiaobao surname: Zhang fullname: Zhang, Qiaobao email: zhangqiaobao@xmu.edu.cn organization: Department of Materials Science and Engineering, College of Materials, Xiamen University |
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| Copyright | Tsinghua University Press and Springer-Verlag GmbH Germany, part of Springer Nature 2021 Tsinghua University Press and Springer-Verlag GmbH Germany, part of Springer Nature 2021. |
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| Keywords | bowl-like carbon/reduced graphene nanosheets hybrids lithium metal battery Li metal host dendrite inhibition |
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| Title | Lithiophilic N-doped carbon bowls induced Li deposition in layered graphene film for advanced lithium metal batteries |
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