Electron-Deficient Acridone Derivatives as a New Functional Core Towards Low-Bandgap Metallopolyynes
The synthesis, thermal, and photoluminescence properties of novel platinum metallopolyynes of electron‐deficient acridone derivatives with electronically tunable bandgaps and their molecular model complexes are described. Polymer P2 has an optical bandgap (Eg) of 2.10 eV which is much lowered than t...
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| Published in | Macromolecular chemistry and physics Vol. 208; no. 10; pp. 1129 - 1136 |
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| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
WILEY-VCH Verlag
21.05.2007
WILEY‐VCH Verlag Wiley |
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| Abstract | The synthesis, thermal, and photoluminescence properties of novel platinum metallopolyynes of electron‐deficient acridone derivatives with electronically tunable bandgaps and their molecular model complexes are described. Polymer P2 has an optical bandgap (Eg) of 2.10 eV which is much lowered than that of P1 (2.60 eV). The incorporation of electron‐accepting dicyanomethylene units on the acridone ring in the main chain creates a strong π‐conjugated system that features unique donor‐acceptor interactions and intramolecular charge‐transfer states. |
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| AbstractList | The synthesis, thermal, and photoluminescence properties of novel platinum metallopolyynes of electron‐deficient acridone derivatives with electronically tunable bandgaps and their molecular model complexes are described. Polymer P2 has an optical bandgap (Eg) of 2.10 eV which is much lowered than that of P1 (2.60 eV). The incorporation of electron‐accepting dicyanomethylene units on the acridone ring in the main chain creates a strong π‐conjugated system that features unique donor‐acceptor interactions and intramolecular charge‐transfer states. Abstract The synthesis, thermal, and photoluminescence properties of novel platinum metallopolyynes of electron‐deficient acridone derivatives with electronically tunable bandgaps and their molecular model complexes are described. Polymer P2 has an optical bandgap ( E g ) of 2.10 eV which is much lowered than that of P1 (2.60 eV). The incorporation of electron‐accepting dicyanomethylene units on the acridone ring in the main chain creates a strong π ‐conjugated system that features unique donor‐acceptor interactions and intramolecular charge‐transfer states. magnified image The synthesis, thermal, and photoluminescence properties of novel platinum metallopolyynes of electron-deficient acridone derivatives with electronically tunable bandgaps and their molecular model complexes are described. Polymer P2 has an optical bandgap (E-g) of 2.10 eV which is much lowered than that of P1 (2.60 eV). The incorporation of electron-accepting dicyanomethylene units on the acridone ring in the main chain creates a strong pi-conjugated system that features unique donor-acceptor interactions and intramolecular charge-transfer states. [GRAPHICS] The synthesis, thermal, and photoluminescence properties of novel platinum metallopolyynes of electron-deficient acridone derivatives with electronically tunable bandgaps and their molecular model complexes are described. Polymer P2 has an optical bandgap (Eg) of 2.10 eV which is much lowered than that of P1 (2.60 eV). The incorporation of electron-accepting dicyanomethylene units on the acridone ring in the main chain creates a strong -conjugated system that features unique donor-acceptor interactions and intramolecular charge-transfer states. . |
| Author | Chow, Wing-Cheong Zhou, Gui-Jiang Wong, Wai-Yeung |
| Author_xml | – sequence: 1 givenname: Wing-Cheong surname: Chow fullname: Chow, Wing-Cheong organization: Department of Chemistry, Hong Kong Baptist University, Waterloo Road, Kowloon Tong, Hong Kong, China – sequence: 2 givenname: Gui-Jiang surname: Zhou fullname: Zhou, Gui-Jiang organization: Department of Chemistry, Hong Kong Baptist University, Waterloo Road, Kowloon Tong, Hong Kong, China – sequence: 3 givenname: Wai-Yeung surname: Wong fullname: Wong, Wai-Yeung email: rwywong@hkbu.edu.hk organization: Department of Chemistry, Hong Kong Baptist University, Waterloo Road, Kowloon Tong, Hong Kong, China |
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| Keywords | synthesis acridone photoluminescence METAL DIYNES cyano groups ENERGY-GAP COPOLYMERS INTRAMOLECULAR CHARGE-TRANSFER EUROPIUM(III) LUMINESCENCE metallopolymers NMR FLUORENE SERIES CONJUGATED POLYMERS platinum(II) polyynes OPTICAL SPECTROSCOPY donor-acceptor compounds UNITS |
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| Snippet | The synthesis, thermal, and photoluminescence properties of novel platinum metallopolyynes of electron‐deficient acridone derivatives with electronically... The synthesis, thermal, and photoluminescence properties of novel platinum metallopolyynes of electron-deficient acridone derivatives with electronically... Abstract The synthesis, thermal, and photoluminescence properties of novel platinum metallopolyynes of electron‐deficient acridone derivatives with... |
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| SubjectTerms | acridone cyano groups donor-acceptor compounds metallopolymers NMR photoluminescence Physical Sciences platinum(II) polyynes Polymer Science Science & Technology synthesis |
| Title | Electron-Deficient Acridone Derivatives as a New Functional Core Towards Low-Bandgap Metallopolyynes |
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