Electrocatalytic oxygen evolution reaction (OER) on mixed nanoporous RuIr borides
Efficient water splitting for commercial electrolysis devices is predicated on the development of materials, specifically for the catalytic electrodes, that exhibit an optimal balance between activity and stability. Complicating the development of electrocatalytic materials, particularly for oxygen-...
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| Published in | Journal of applied electrochemistry Vol. 51; no. 7; pp. 1101 - 1108 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Dordrecht
Springer Netherlands
01.07.2021
Springer Nature B.V |
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| Abstract | Efficient water splitting for commercial electrolysis devices is predicated on the development of materials, specifically for the catalytic electrodes, that exhibit an optimal balance between activity and stability. Complicating the development of electrocatalytic materials, particularly for oxygen-evolving anodes in acidic polymer electrolyte membrane electrolyzers, is an inverse relationship between activity and stability. Here the development of a nanostructured oxygen evolution reaction (OER) electrocatalyst for low-pH water splitting is demonstrated. Dealloying of mixed RuIr borides is used to form a high aspect ratio electrocatalytic material that exhibits low OER overpotentials matching that of RuO
x
and electrolytic stability matching that of IrO
x
.
Graphic abstract |
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| AbstractList | Efficient water splitting for commercial electrolysis devices is predicated on the development of materials, specifically for the catalytic electrodes, that exhibit an optimal balance between activity and stability. Complicating the development of electrocatalytic materials, particularly for oxygen-evolving anodes in acidic polymer electrolyte membrane electrolyzers, is an inverse relationship between activity and stability. Here the development of a nanostructured oxygen evolution reaction (OER) electrocatalyst for low-pH water splitting is demonstrated. Dealloying of mixed RuIr borides is used to form a high aspect ratio electrocatalytic material that exhibits low OER overpotentials matching that of RuOx and electrolytic stability matching that of IrOx.Graphic abstract Efficient water splitting for commercial electrolysis devices is predicated on the development of materials, specifically for the catalytic electrodes, that exhibit an optimal balance between activity and stability. Complicating the development of electrocatalytic materials, particularly for oxygen-evolving anodes in acidic polymer electrolyte membrane electrolyzers, is an inverse relationship between activity and stability. Here the development of a nanostructured oxygen evolution reaction (OER) electrocatalyst for low-pH water splitting is demonstrated. Dealloying of mixed RuIr borides is used to form a high aspect ratio electrocatalytic material that exhibits low OER overpotentials matching that of RuO x and electrolytic stability matching that of IrO x . Graphic abstract |
| Author | Snyder, Joshua Intikhab, Saad Barsoum, Michel W. Natu, Varun Chatterjee, Swarnendu Sokol, Maxim Li, Yawei |
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| Keywords | PEM electrolysis Nanoporous metals Oxygen evolution reaction Dealloying |
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| SubjectTerms | Borides Chemistry Chemistry and Materials Science Electrocatalysts Electrochemistry Electrolysis High aspect ratio Hydrogen production Industrial Chemistry/Chemical Engineering Matching Oxygen evolution reactions Physical Chemistry Short Communication Stability Water splitting |
| Title | Electrocatalytic oxygen evolution reaction (OER) on mixed nanoporous RuIr borides |
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