Behaviors of dewaterability and heavy metals of waste activated sludge conditioned by heat-activated peroxymonosulfate oxidation

In this work, heat-activated peroxymonosulfate (heat-PMS) oxidation was used to condition waste activated sludge. The results showed that the optimal temperature and PMS dosage for sludge dewatering were 75 °C and 150 mg/g-volatile solids (VS), and the addition of rice husk (100–400 mg/g-VS) was fav...

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Published inChemical papers Vol. 74; no. 2; pp. 641 - 650
Main Authors Huang, Zaichun, Liu, Changgeng, Zhu, Xuejun, Xiang, Guoqi, Zeng, Chenghua, Zhong, Yuquan
Format Journal Article
LanguageEnglish
Published Cham Springer International Publishing 01.02.2020
Springer Nature B.V
Subjects
Activated sludge
Biochemistry
Biotechnology
Chemistry
Chemistry and Materials Science
Chemistry/Food Science
Conditioning
Heavy metals
Industrial Chemistry/Chemical Engineering
Leaching
Materials Science
Medicinal Chemistry
Moisture content
Original Paper
Oxidation
Sludge
Solubilization
Suction
Toxicity
Heat/peroxymonosulfate
Waste activated sludge
Advanced oxidation
Dewatering
Heavy metals
Online AccessGet full text

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Abstract In this work, heat-activated peroxymonosulfate (heat-PMS) oxidation was used to condition waste activated sludge. The results showed that the optimal temperature and PMS dosage for sludge dewatering were 75 °C and 150 mg/g-volatile solids (VS), and the addition of rice husk (100–400 mg/g-VS) was favorable to further enhance sludge dewaterability. Under optimal conditions, the capillary suction time reduction and water content of sludge cake were 82.4% and 65.8%, respectively. The significant improvement of sludge dewaterability was ascribed to the releases of extracellular polymeric substances (EPS)-bound water and cell water caused by the significant breakdown of tightly bound EPS, as well as the skeleton effect. In addition, heat-PMS oxidation has been demonstrated with the merits of improving the immobilization of heavy metals (HMs) and weakening their environmental risk. After conditioning, HMs solubilization was enhanced significantly and their leaching toxicity decreased obviously. Meanwhile, HMs were transformed into more stable forms. Therefore, heat-PMS oxidation might be a potential and desirable technology for sludge conditioning with respect to the enhancement of sludge dewaterability and the decrease of HMs environmental risk.
AbstractList In this work, heat-activated peroxymonosulfate (heat-PMS) oxidation was used to condition waste activated sludge. The results showed that the optimal temperature and PMS dosage for sludge dewatering were 75 °C and 150 mg/g-volatile solids (VS), and the addition of rice husk (100–400 mg/g-VS) was favorable to further enhance sludge dewaterability. Under optimal conditions, the capillary suction time reduction and water content of sludge cake were 82.4% and 65.8%, respectively. The significant improvement of sludge dewaterability was ascribed to the releases of extracellular polymeric substances (EPS)-bound water and cell water caused by the significant breakdown of tightly bound EPS, as well as the skeleton effect. In addition, heat-PMS oxidation has been demonstrated with the merits of improving the immobilization of heavy metals (HMs) and weakening their environmental risk. After conditioning, HMs solubilization was enhanced significantly and their leaching toxicity decreased obviously. Meanwhile, HMs were transformed into more stable forms. Therefore, heat-PMS oxidation might be a potential and desirable technology for sludge conditioning with respect to the enhancement of sludge dewaterability and the decrease of HMs environmental risk.
In this work, heat-activated peroxymonosulfate (heat-PMS) oxidation was used to condition waste activated sludge. The results showed that the optimal temperature and PMS dosage for sludge dewatering were 75 °C and 150 mg/g-volatile solids (VS), and the addition of rice husk (100–400 mg/g-VS) was favorable to further enhance sludge dewaterability. Under optimal conditions, the capillary suction time reduction and water content of sludge cake were 82.4% and 65.8%, respectively. The significant improvement of sludge dewaterability was ascribed to the releases of extracellular polymeric substances (EPS)-bound water and cell water caused by the significant breakdown of tightly bound EPS, as well as the skeleton effect. In addition, heat-PMS oxidation has been demonstrated with the merits of improving the immobilization of heavy metals (HMs) and weakening their environmental risk. After conditioning, HMs solubilization was enhanced significantly and their leaching toxicity decreased obviously. Meanwhile, HMs were transformed into more stable forms. Therefore, heat-PMS oxidation might be a potential and desirable technology for sludge conditioning with respect to the enhancement of sludge dewaterability and the decrease of HMs environmental risk.
Author Liu, Changgeng
Xiang, Guoqi
Zeng, Chenghua
Huang, Zaichun
Zhong, Yuquan
Zhu, Xuejun
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Issue 2
Keywords Heat/peroxymonosulfate
Waste activated sludge
Advanced oxidation
Dewatering
Heavy metals
Language English
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Snippet In this work, heat-activated peroxymonosulfate (heat-PMS) oxidation was used to condition waste activated sludge. The results showed that the optimal...
In this work, heat-activated peroxymonosulfate (heat-PMS) oxidation was used to condition waste activated sludge. The results showed that the optimal...
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SubjectTerms Activated sludge
Biochemistry
Biotechnology
Chemistry
Chemistry and Materials Science
Chemistry/Food Science
Conditioning
Heavy metals
Industrial Chemistry/Chemical Engineering
Leaching
Materials Science
Medicinal Chemistry
Moisture content
Original Paper
Oxidation
Sludge
Solubilization
Suction
Toxicity
Title Behaviors of dewaterability and heavy metals of waste activated sludge conditioned by heat-activated peroxymonosulfate oxidation
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https://www.proquest.com/docview/2343286846
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