Theoretical aspects of 2D electrochemical phase formation
Two-dimensional electrochemical phase formation as a result of nucleation, growth, and overlap of disk-shaped nuclei of a new phase on the electrode surface is analyzed. This problem is considered based on the Kolmogorov-Johnson-Mehl-Avrami (KJMA) theory. General formulae applicable for any type of...
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| Published in | Journal of solid state electrochemistry Vol. 25; no. 2; pp. 689 - 694 |
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| Main Authors | , , |
| Format | Journal Article |
| Language | English |
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Berlin/Heidelberg
Springer Berlin Heidelberg
01.02.2021
Springer Nature B.V |
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| Abstract | Two-dimensional electrochemical phase formation as a result of nucleation, growth, and overlap of disk-shaped nuclei of a new phase on the electrode surface is analyzed. This problem is considered based on the Kolmogorov-Johnson-Mehl-Avrami (KJMA) theory. General formulae applicable for any type of two-dimensional crystallization are derived. The theory of the double-pulse potentiostatic method is considered. Theoretical expressions are obtained for potentiostatic current density transients in the case of two-dimensional electrocrystallization at different durations and magnitudes of the first and second pulses (nucleation and growth pulses, respectively). The maxima of the current density transients are analyzed to obtain information about the mechanisms and parameters of nucleation and growth. The morphology of a continuous deposit layer is discussed in terms of Voronoi cells. |
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| AbstractList | Two-dimensional electrochemical phase formation as a result of nucleation, growth, and overlap of disk-shaped nuclei of a new phase on the electrode surface is analyzed. This problem is considered based on the Kolmogorov-Johnson-Mehl-Avrami (KJMA) theory. General formulae applicable for any type of two-dimensional crystallization are derived. The theory of the double-pulse potentiostatic method is considered. Theoretical expressions are obtained for potentiostatic current density transients in the case of two-dimensional electrocrystallization at different durations and magnitudes of the first and second pulses (nucleation and growth pulses, respectively). The maxima of the current density transients are analyzed to obtain information about the mechanisms and parameters of nucleation and growth. The morphology of a continuous deposit layer is discussed in terms of Voronoi cells. |
| Author | Zaikov, Yury P. Grishenkova, Olga V. Isaev, Vladimir A. |
| Author_xml | – sequence: 1 givenname: Vladimir A. orcidid: 0000-0001-5487-0536 surname: Isaev fullname: Isaev, Vladimir A. email: v.isaev@ihte.uran.ru, v.a.isaev@mail.ru organization: Institute of High Temperature Electrochemistry, Ural Branch of the Russian Academy of Sciences – sequence: 2 givenname: Olga V. orcidid: 0000-0001-5880-1634 surname: Grishenkova fullname: Grishenkova, Olga V. organization: Institute of High Temperature Electrochemistry, Ural Branch of the Russian Academy of Sciences – sequence: 3 givenname: Yury P. orcidid: 0000-0001-6138-3955 surname: Zaikov fullname: Zaikov, Yury P. organization: Institute of High Temperature Electrochemistry, Ural Branch of the Russian Academy of Sciences, Ural Federal University |
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| Keywords | 2D deposit layer Electrodeposition Nucleation Growth |
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| Title | Theoretical aspects of 2D electrochemical phase formation |
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