Highly electroluminescent devices made with a conveniently synthesized triazole-triphenylamine derivative

The convenient synthesis of (3-(4- tert-Butylphenyl)-4-phenyl-5-(4′-diphenylaminostilben-4-yl)-1,2,4-triazole) is described. This molecule, labeled TAZ-TPA is composed of triphenylamine (known to transport holes) and triazole (known to transport electrons) moieties. TAZ-TPA is easily obtained as a t...

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Published inThin solid films Vol. 466; no. 1; pp. 209 - 216
Main Authors Maindron, T., Wang, Y., Dodelet, J.P., Miyatake, K., Hlil, A.R., Hay, A.S., Tao, Y., D'Iorio, M.
Format Journal Article
LanguageEnglish
Published Lausanne Elsevier B.V 01.11.2004
Elsevier Science
Subjects
Amorphous material
Condensed matter: electronic structure, electrical, magnetic, and optical properties
Cross-disciplinary physics: materials science; rheology
Electroluminescence
Exact sciences and technology
Luminescence
Materials science
Methods of deposition of films and coatings; film growth and epitaxy
Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation
Optoelectronic devices
Organic light emitting devices
Other luminescence and radiative recombination
Physics
Vacuum deposition
Amorphous material
Optoelectronic devices
Organic light emitting devices
Luminescence
Amines
Scattering
Photoluminescence
Light emitting diodes
Electroluminescence
Crystal growth from vapors
Experimental study
Thin films
Thickness
Cyclic voltammetry
Absorbance
Triazoles
Size effect
IV characteristic
Vacuum evaporation
Organic compounds
Illuminance
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Abstract The convenient synthesis of (3-(4- tert-Butylphenyl)-4-phenyl-5-(4′-diphenylaminostilben-4-yl)-1,2,4-triazole) is described. This molecule, labeled TAZ-TPA is composed of triphenylamine (known to transport holes) and triazole (known to transport electrons) moieties. TAZ-TPA is easily obtained as a thin solid film by vacuum evaporation. Devices made with TAZ-TPA as electron transport and electroluminescent layer, in conjunction with an aryl amine hole transport layer, luminesce strongly in the blue green (the luminescence peaks at 484 nm). They are characterized by a 4±0.5 V turn on voltage, a maximum luminance of 10 900±1100 Cd/m 2 and a photometric efficiency of 2.2±0.2 Cd/A. From the dependence of the luminance vs. the thickness of the TAZ-TPA layer, it is deduced that the hole and electron diffusion lengths in TAZ-TPA are 60±12 nm and 100±12 nm, respectively. Adding 1 wt.% rubrene in the hole transport layer improves the maximum luminance to 16 100±1600 Cd/m 2 without practically altering the electroluminescent spectrum of the device.
AbstractList The convenient synthesis of (3-(4-tert-Butylphenyl)-4-phenyl-5-(4'-diphenylaminostilben-4-yl)-1 ,2,4-triazole) is described. This molecule, labeled TAZ-TPA is composed of triphenylamine (known to transport holes) and triazole (known to transport electrons) moieties. TAZ-TPA is easily obtained as a thin solid film by vacuum evaporation. Devices made with TAZ-TPA as electron transport and electroluminescent layer, in conjunction with an aryl amine hole transport layer, luminesce strongly in the blue green (the luminescence peaks at 484 nm). They are characterized by a 4 +/- 0.5 V turn on voltage, a maximum luminance of 10900 +/- 1100 Cd/sq m and a photometric efficiency of 2.2 +/- 0.2 Cd/A. From the dependence of the luminance vs. the thickness of the TAZ-TPA layer, it is deduced that the hole and electron diffusion lengths in TAZ-TPA are 60 +/- 12 nm and 100 +/- 12 nm, respectively. Adding 1 wt.% rubrene in the hole transport layer improves the maximum luminance to 16100 +/- 1600 Cd/sq m without practically altering the electroluminescent spectrum of the device.
The convenient synthesis of (3-(4- tert-Butylphenyl)-4-phenyl-5-(4′-diphenylaminostilben-4-yl)-1,2,4-triazole) is described. This molecule, labeled TAZ-TPA is composed of triphenylamine (known to transport holes) and triazole (known to transport electrons) moieties. TAZ-TPA is easily obtained as a thin solid film by vacuum evaporation. Devices made with TAZ-TPA as electron transport and electroluminescent layer, in conjunction with an aryl amine hole transport layer, luminesce strongly in the blue green (the luminescence peaks at 484 nm). They are characterized by a 4±0.5 V turn on voltage, a maximum luminance of 10 900±1100 Cd/m 2 and a photometric efficiency of 2.2±0.2 Cd/A. From the dependence of the luminance vs. the thickness of the TAZ-TPA layer, it is deduced that the hole and electron diffusion lengths in TAZ-TPA are 60±12 nm and 100±12 nm, respectively. Adding 1 wt.% rubrene in the hole transport layer improves the maximum luminance to 16 100±1600 Cd/m 2 without practically altering the electroluminescent spectrum of the device.
Author Maindron, T.
Dodelet, J.P.
Hay, A.S.
Tao, Y.
Wang, Y.
Miyatake, K.
Hlil, A.R.
D'Iorio, M.
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Issue 1
Keywords Amorphous material
Optoelectronic devices
Organic light emitting devices
Luminescence
Amines
Scattering
Photoluminescence
Light emitting diodes
Electroluminescence
Crystal growth from vapors
Experimental study
Thin films
Thickness
Cyclic voltammetry
Absorbance
Triazoles
Size effect
IV characteristic
Vacuum evaporation
Organic compounds
Illuminance
Language English
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Elsevier Science
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Snippet The convenient synthesis of (3-(4- tert-Butylphenyl)-4-phenyl-5-(4′-diphenylaminostilben-4-yl)-1,2,4-triazole) is described. This molecule, labeled TAZ-TPA is...
The convenient synthesis of (3-(4-tert-Butylphenyl)-4-phenyl-5-(4'-diphenylaminostilben-4-yl)-1 ,2,4-triazole) is described. This molecule, labeled TAZ-TPA is...
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SubjectTerms Amorphous material
Condensed matter: electronic structure, electrical, magnetic, and optical properties
Cross-disciplinary physics: materials science; rheology
Electroluminescence
Exact sciences and technology
Luminescence
Materials science
Methods of deposition of films and coatings; film growth and epitaxy
Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation
Optoelectronic devices
Organic light emitting devices
Other luminescence and radiative recombination
Physics
Vacuum deposition
Title Highly electroluminescent devices made with a conveniently synthesized triazole-triphenylamine derivative
URI https://dx.doi.org/10.1016/j.tsf.2004.01.119
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