Defocused Wide‐field Imaging Unravels Structural and Temporal Heterogeneity in Complex Systems
Today's miniature devices and biological systems share the fact that their dynamics and properties cannot be understood in terms of macroscopic concepts, but require a thorough understanding of the nanoscale structuring. This structuring is often very heterogeneous, both in time and in space, a...
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| Published in | Advanced materials (Weinheim) Vol. 21; no. 10‐11; pp. 1079 - 1090 |
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| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
WILEY‐VCH Verlag
20.03.2009
Wiley-VCH Verlag |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Today's miniature devices and biological systems share the fact that their dynamics and properties cannot be understood in terms of macroscopic concepts, but require a thorough understanding of the nanoscale structuring. This structuring is often very heterogeneous, both in time and in space, and is difficult or impossible to resolve with traditional approaches. In this Progress Report, we will discuss how single‐molecule microscopy—and defocused wide‐field imaging in particular—can be used to shed light on these phenomena.
Revealing heterogeneity in macromolecular systems such as polymer matrices is difficult to achieve using traditional methods, but is highly suited to single‐molecule imaging. In this Progress Report we discuss some approaches that can provide detailed information on the structure and dynamics of such systems. In particular, we focus on a recent technique, defocused wide‐field imaging, which provides the position and orientation of a single molecule, and how this can be applied to explore phenomena such as polymer dynamics, nanoscale structuring, and energy transfer. |
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| AbstractList | Today's miniature devices and biological systems share the fact that their dynamics and properties cannot be understood in terms of macroscopic concepts, but require a thorough understanding of the nanoscale structuring. This structuring is often very heterogeneous, both in time and in space, and is difficult or impossible to resolve with traditional approaches. In this Progress Report, we will discuss how single-molecule microscopy - and defocused wide-field imaging in particular - can be used to shed light on these phenomena. Today's miniature devices and biological systems share the fact that their dynamics and properties cannot be understood in terms of macroscopic concepts, but require a thorough understanding of the nanoscale structuring. This structuring is often very heterogeneous, both in time and in space, and is difficult or impossible to resolve with traditional approaches. In this Progress Report, we will discuss how single‐molecule microscopy—and defocused wide‐field imaging in particular—can be used to shed light on these phenomena. Revealing heterogeneity in macromolecular systems such as polymer matrices is difficult to achieve using traditional methods, but is highly suited to single‐molecule imaging. In this Progress Report we discuss some approaches that can provide detailed information on the structure and dynamics of such systems. In particular, we focus on a recent technique, defocused wide‐field imaging, which provides the position and orientation of a single molecule, and how this can be applied to explore phenomena such as polymer dynamics, nanoscale structuring, and energy transfer. Abstract Today's miniature devices and biological systems share the fact that their dynamics and properties cannot be understood in terms of macroscopic concepts, but require a thorough understanding of the nanoscale structuring. This structuring is often very heterogeneous, both in time and in space, and is difficult or impossible to resolve with traditional approaches. In this Progress Report, we will discuss how single‐molecule microscopy—and defocused wide‐field imaging in particular—can be used to shed light on these phenomena. |
| Author | Uji‐i, Hiroshi Muls, Benoît Soumillion, Jean‐Philippe Müllen, Klaus Sliwa, Michel Deres, Ania Enderlein, Jörg Hofkens, Johan Dedecker, Peter Hotta, Jun‐ichi |
| Author_xml | – sequence: 1 givenname: Peter surname: Dedecker fullname: Dedecker, Peter – sequence: 2 givenname: Benoît surname: Muls fullname: Muls, Benoît – sequence: 3 givenname: Ania surname: Deres fullname: Deres, Ania – sequence: 4 givenname: Hiroshi surname: Uji‐i fullname: Uji‐i, Hiroshi – sequence: 5 givenname: Jun‐ichi surname: Hotta fullname: Hotta, Jun‐ichi – sequence: 6 givenname: Michel surname: Sliwa fullname: Sliwa, Michel – sequence: 7 givenname: Jean‐Philippe surname: Soumillion fullname: Soumillion, Jean‐Philippe – sequence: 8 givenname: Klaus surname: Müllen fullname: Müllen, Klaus – sequence: 9 givenname: Jörg surname: Enderlein fullname: Enderlein, Jörg – sequence: 10 givenname: Johan surname: Hofkens fullname: Hofkens, Johan email: johan.hofkens@chem.kuleuven.be |
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| Copyright | Copyright © 2009 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim Distributed under a Creative Commons Attribution 4.0 International License |
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| Keywords | Conjugated polymers Single-molecule imaging Nanostructuring Defocused wide-field imaging Fluorescence Chromophores Energy transfer Polyphenylene dendrimers |
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| Snippet | Today's miniature devices and biological systems share the fact that their dynamics and properties cannot be understood in terms of macroscopic concepts, but... Abstract Today's miniature devices and biological systems share the fact that their dynamics and properties cannot be understood in terms of macroscopic... |
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| SubjectTerms | Chemical Sciences Chromophores Conjugated polymers Defocused wide‐field imaging Energy transfer Fluorescence Nanostructuring or physical chemistry Polyphenylene dendrimers Single‐molecule imaging Theoretical and |
| Title | Defocused Wide‐field Imaging Unravels Structural and Temporal Heterogeneity in Complex Systems |
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