Experimental evidence for ultrashort-lived spin polarons in EuSe
We investigated the time evolution of the density of giant spin polarons in a magnetic semiconductor. Spin polarons (SPs) were photoexcited and observed using time-resolved Faraday rotation. We find the existence of two types of SPs, a short-lived spin polaron with a lifetime of around τsl = 0.5 ns...
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| Published in | AIP advances Vol. 14; no. 2; pp. 025006 - 025006-4 |
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| Main Authors | , |
| Format | Journal Article |
| Language | English |
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Melville
American Institute of Physics
01.02.2024
AIP Publishing LLC |
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| Abstract | We investigated the time evolution of the density of giant spin polarons in a magnetic semiconductor. Spin polarons (SPs) were photoexcited and observed using time-resolved Faraday rotation. We find the existence of two types of SPs, a short-lived spin polaron with a lifetime of around τsl = 0.5 ns and a long-lived spin polaron with a lifetime of τll = 0.45 ± 0.03 µs, at T = 5 K. The stark difference of three order of magnitude between these lifetimes suggests that in the long lived SP the electron-hole pair is relaxed and its recombination is forbidden. The short-lived SP is probably associated with SP recombination before such relaxation has occured. An extraordinary finding is that the magnitude of τsl, as well as its decrease with increasing temperature, reproduces exactly the characteristic time for SP growth. This suggests that the thermal fluctuations, responsible for SP magnetic moment growth, are also responsible for increasing the recombination probability of SPs. |
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| AbstractList | We investigated the time evolution of the density of giant spin polarons in a magnetic semiconductor. Spin polarons (SPs) were photoexcited and observed using time-resolved Faraday rotation. We find the existence of two types of SPs, a short-lived spin polaron with a lifetime of around τsl = 0.5 ns and a long-lived spin polaron with a lifetime of τll = 0.45 ± 0.03 µs, at T = 5 K. The stark difference of three order of magnitude between these lifetimes suggests that in the long lived SP the electron-hole pair is relaxed and its recombination is forbidden. The short-lived SP is probably associated with SP recombination before such relaxation has occured. An extraordinary finding is that the magnitude of τsl, as well as its decrease with increasing temperature, reproduces exactly the characteristic time for SP growth. This suggests that the thermal fluctuations, responsible for SP magnetic moment growth, are also responsible for increasing the recombination probability of SPs. We investigated the time evolution of the density of giant spin polarons in a magnetic semiconductor. Spin polarons (SPs) were photoexcited and observed using time-resolved Faraday rotation. We find the existence of two types of SPs, a short-lived spin polaron with a lifetime of around τsl = 0.5 ns and a long-lived spin polaron with a lifetime of τll = 0.45 ± 0.03 µs, at T = 5 K. The stark difference of three order of magnitude between these lifetimes suggests that in the long lived SP the electron-hole pair is relaxed and its recombination is forbidden. The short-lived SP is probably associated with SP recombination before such relaxation has occured. An extraordinary finding is that the magnitude of τsl, as well as its decrease with increasing temperature, reproduces exactly the characteristic time for SP growth. This suggests that the thermal fluctuations, responsible for SP magnetic moment growth, are also responsible for increasing the recombination probability of SPs. |
| Author | van Kooten, S. C. P. Henriques, A. B. |
| Author_xml | – sequence: 1 givenname: S. C. P. surname: van Kooten fullname: van Kooten, S. C. P. organization: Laboratório de Magneto-Óptica—LMO, Instituto de Física, Universidade de São Paulo, 05508-090 São Paulo, Brazil – sequence: 2 givenname: A. B. surname: Henriques fullname: Henriques, A. B. organization: Laboratório de Magneto-Óptica—LMO, Instituto de Física, Universidade de São Paulo, 05508-090 São Paulo, Brazil |
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| Cites_doi | 10.1103/physrevb.105.224427 10.1016/0370-1573(86)90139-0 10.1038/nature03564 10.1103/physrevb.90.165202 10.1103/revmodphys.82.2731 10.1038/nature20807 10.1103/revmodphys.89.025006 10.1063/1.3634030 10.1103/physrevb.93.201201 10.1103/physrevlett.120.217203 10.1103/physrevlett.76.4250 10.1063/5.0079384 10.1103/physrevb.95.045205 10.1063/1.5116150 10.1063/1.5143311 10.1063/1.3602927 10.1038/nmat2593 |
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| SubjectTerms | Faraday effect Holes (electron deficiencies) Magnetic moments Magnetic semiconductors Polarons |
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| Title | Experimental evidence for ultrashort-lived spin polarons in EuSe |
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