Surface interaction of tetrabromobisphenol A, bisphenol A and phenol with graphene-based materials in water: Adsorption mechanism and thermodynamic effects

•Graphene oxide (GO) adsorbed emerging compounds less than reduced GO (rGO).•Langmuir model and pseudo-second-order can describe adsorption well.•Endothermic and spontaneous adsorption with small change in entropy was observed.•Adsorption mechanism was governed by π – π interactions and hydrogen bon...

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Published inJournal of hazardous materials advances Vol. 9; p. 100227
Main Authors Catherine, Hepsiba Niruba, Tan, Kok-Hou, Shih, Yang-hsin, Doong, Ruey-an, Manu, Basavaraj, Ding, Jiann-yuan
Format Journal Article
LanguageEnglish
Published Elsevier B.V 01.02.2023
Subjects
Bisphenol A
Emerging contaminants
Graphene oxide
Phenol
Sorption
Temperature
Tetrabromobisphenol A
Sorption
Bisphenol A
Phenol
Temperature
Tetrabromobisphenol A
Graphene oxide
Emerging contaminants
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Abstract •Graphene oxide (GO) adsorbed emerging compounds less than reduced GO (rGO).•Langmuir model and pseudo-second-order can describe adsorption well.•Endothermic and spontaneous adsorption with small change in entropy was observed.•Adsorption mechanism was governed by π – π interactions and hydrogen bonding.•GO and rGO with organic pollutants can affect their fate in aquatic environment. Carbon-based materials, especially graphene nanocomposites (GNS) have attracted wide attention in recent years. In this study, graphene oxide (GO) and reduced graphene oxide (rGO) were prepared using the Improved Hummers method and were investigated for their adsorption behavior of emerging contaminants such as tetrabromobisphenol A (TBBPA), bisphenol A (BPA), and a conventional contaminant, phenol. The adsorption capacity seemed to slightly increase with increasing reduction degree of GO, highlighting its hydrophobic effect. The adsorption kinetics and isotherms were well delineated using pseudo-second-order and Langmuir equations respectively. At higher temperatures, the adsorption of these selected organic contaminants on GO and rGO slightly increased, also indicating the slight effect of temperature on the adsorption in the environment. From a thermodynamic analysis, the endothermic and spontaneous reaction was observed. The adsorption mechanisms included hydrophobicity, π- π interactions and π electron acceptor and donor ones. GNS can suspend in water even after adsorbing pollutants at the water interface. This would enhance the transport of these contaminants with nanomaterials in the environment. These findings are valuable to elucidate the interaction mechanism between phenol, BPA, and TBBPA on GNS while further understanding the physicochemical behavior of these organic contaminants in the environment. Summary: Adsorption capacities of emerging contaminants, BPA and TBBPA, as well as phenol on graphene oxide (GO) and reduced GO (rGO), were similar. Higher temperatures slightly increased the adsorption of these phenolic compounds on GO and rGO, which also indicated an endothermic and spontaneous process. [Display omitted]
AbstractList •Graphene oxide (GO) adsorbed emerging compounds less than reduced GO (rGO).•Langmuir model and pseudo-second-order can describe adsorption well.•Endothermic and spontaneous adsorption with small change in entropy was observed.•Adsorption mechanism was governed by π – π interactions and hydrogen bonding.•GO and rGO with organic pollutants can affect their fate in aquatic environment. Carbon-based materials, especially graphene nanocomposites (GNS) have attracted wide attention in recent years. In this study, graphene oxide (GO) and reduced graphene oxide (rGO) were prepared using the Improved Hummers method and were investigated for their adsorption behavior of emerging contaminants such as tetrabromobisphenol A (TBBPA), bisphenol A (BPA), and a conventional contaminant, phenol. The adsorption capacity seemed to slightly increase with increasing reduction degree of GO, highlighting its hydrophobic effect. The adsorption kinetics and isotherms were well delineated using pseudo-second-order and Langmuir equations respectively. At higher temperatures, the adsorption of these selected organic contaminants on GO and rGO slightly increased, also indicating the slight effect of temperature on the adsorption in the environment. From a thermodynamic analysis, the endothermic and spontaneous reaction was observed. The adsorption mechanisms included hydrophobicity, π- π interactions and π electron acceptor and donor ones. GNS can suspend in water even after adsorbing pollutants at the water interface. This would enhance the transport of these contaminants with nanomaterials in the environment. These findings are valuable to elucidate the interaction mechanism between phenol, BPA, and TBBPA on GNS while further understanding the physicochemical behavior of these organic contaminants in the environment. Summary: Adsorption capacities of emerging contaminants, BPA and TBBPA, as well as phenol on graphene oxide (GO) and reduced GO (rGO), were similar. Higher temperatures slightly increased the adsorption of these phenolic compounds on GO and rGO, which also indicated an endothermic and spontaneous process. [Display omitted]
ArticleNumber 100227
Author Ding, Jiann-yuan
Catherine, Hepsiba Niruba
Tan, Kok-Hou
Manu, Basavaraj
Doong, Ruey-an
Shih, Yang-hsin
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  givenname: Ruey-an
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  surname: Ding
  fullname: Ding, Jiann-yuan
  organization: Center of General Education, Wenzao Ursuline University of Languages, Kaohsiung, 80793, Taiwan
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crossref_primary_10_1080_03067319_2023_2300749
crossref_primary_10_1080_09603123_2023_2208536
crossref_primary_10_3390_w15081626
crossref_primary_10_3390_toxics11030232
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Copyright 2022
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Keywords Sorption
Bisphenol A
Phenol
Temperature
Tetrabromobisphenol A
Graphene oxide
Emerging contaminants
Language English
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Snippet •Graphene oxide (GO) adsorbed emerging compounds less than reduced GO (rGO).•Langmuir model and pseudo-second-order can describe adsorption well.•Endothermic...
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Publisher
StartPage 100227
SubjectTerms Bisphenol A
Emerging contaminants
Graphene oxide
Phenol
Sorption
Temperature
Tetrabromobisphenol A
Title Surface interaction of tetrabromobisphenol A, bisphenol A and phenol with graphene-based materials in water: Adsorption mechanism and thermodynamic effects
URI https://dx.doi.org/10.1016/j.hazadv.2022.100227
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