Correlation of type II adsorption isotherms of water contaminants using modified BET equations

The BET equation is commonly used to describe type II sigmoid isotherms of water contaminants. However, there are some type II isotherms that do not agree with the BET equation. In this paper, three modified BET equations (Aguerre–Suarez–Viollaz, Pantuso–Tolaba–Aguerre, and Aranovich–Donohue) are ev...

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Published inColloid and interface science communications Vol. 46; p. 100557
Main Authors Brião, Giani de Vargas, da Silva, Meuris Gurgel Carlos, Vieira, Melissa Gurgel Adeodato, Chu, Khim Hoong
Format Journal Article
LanguageEnglish
Published Elsevier B.V 01.01.2022
Subjects
Aranovich–Donohue isotherm
Multilayer adsorption
S-shaped
Sigmoid
Type II
Type II
Aranovich–Donohue isotherm
Multilayer adsorption
S-shaped
Sigmoid
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Abstract The BET equation is commonly used to describe type II sigmoid isotherms of water contaminants. However, there are some type II isotherms that do not agree with the BET equation. In this paper, three modified BET equations (Aguerre–Suarez–Viollaz, Pantuso–Tolaba–Aguerre, and Aranovich–Donohue) are evaluated against published isotherm data of dysprosium, reactive blue 5G, and naphthenic acid. In the cases studied, the three modified BET equations are shown to outperform the original BET equation. The Aranovich–Donohue equation is a promising isotherm model, offering accurate data correlations and statistically significant parameter estimates. In particular, it is very effective in tracing the atypical curve shapes of the reactive blue 5G and naphthenic acid isotherms. Although the Aranovich–Donohue equation has not attracted much attention, it is a practical alternative to the widely used BET equation for correlating adsorption isotherms of water contaminants. [Display omitted] •The BET equation fits intricate type II isotherms poorly.•The Aranovich–Donohue equation outperforms the BET equation in correlating atypical type II isotherms.•The Aranovich–Donohue parameter estimates are statistically significant.
AbstractList The BET equation is commonly used to describe type II sigmoid isotherms of water contaminants. However, there are some type II isotherms that do not agree with the BET equation. In this paper, three modified BET equations (Aguerre–Suarez–Viollaz, Pantuso–Tolaba–Aguerre, and Aranovich–Donohue) are evaluated against published isotherm data of dysprosium, reactive blue 5G, and naphthenic acid. In the cases studied, the three modified BET equations are shown to outperform the original BET equation. The Aranovich–Donohue equation is a promising isotherm model, offering accurate data correlations and statistically significant parameter estimates. In particular, it is very effective in tracing the atypical curve shapes of the reactive blue 5G and naphthenic acid isotherms. Although the Aranovich–Donohue equation has not attracted much attention, it is a practical alternative to the widely used BET equation for correlating adsorption isotherms of water contaminants. [Display omitted] •The BET equation fits intricate type II isotherms poorly.•The Aranovich–Donohue equation outperforms the BET equation in correlating atypical type II isotherms.•The Aranovich–Donohue parameter estimates are statistically significant.
ArticleNumber 100557
Author Brião, Giani de Vargas
da Silva, Meuris Gurgel Carlos
Vieira, Melissa Gurgel Adeodato
Chu, Khim Hoong
Author_xml – sequence: 1
  givenname: Giani de Vargas
  surname: Brião
  fullname: Brião, Giani de Vargas
  organization: School of Chemical Engineering, University of Campinas (UNICAMP), Cidade Universitária Zeferino Vaz, 13083-852, Campinas, São Paulo, Brazil
– sequence: 2
  givenname: Meuris Gurgel Carlos
  surname: da Silva
  fullname: da Silva, Meuris Gurgel Carlos
  organization: School of Chemical Engineering, University of Campinas (UNICAMP), Cidade Universitária Zeferino Vaz, 13083-852, Campinas, São Paulo, Brazil
– sequence: 3
  givenname: Melissa Gurgel Adeodato
  surname: Vieira
  fullname: Vieira, Melissa Gurgel Adeodato
  organization: School of Chemical Engineering, University of Campinas (UNICAMP), Cidade Universitária Zeferino Vaz, 13083-852, Campinas, São Paulo, Brazil
– sequence: 4
  givenname: Khim Hoong
  surname: Chu
  fullname: Chu, Khim Hoong
  email: khimchu@gmail.com
  organization: Honeychem Research, Newtown, Wellington 6021, New Zealand
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Keywords Type II
Aranovich–Donohue isotherm
Multilayer adsorption
S-shaped
Sigmoid
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Snippet The BET equation is commonly used to describe type II sigmoid isotherms of water contaminants. However, there are some type II isotherms that do not agree with...
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StartPage 100557
SubjectTerms Aranovich–Donohue isotherm
Multilayer adsorption
S-shaped
Sigmoid
Type II
Title Correlation of type II adsorption isotherms of water contaminants using modified BET equations
URI https://dx.doi.org/10.1016/j.colcom.2021.100557
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