Solvation sheath reorganization enables divalent metal batteries with fast interfacial charge transfer kinetics
Divalent rechargeable metal batteries such as those based on magnesium and calcium are of interest because of the abundance of these elements and their lower tendency to form dendrites, but practical demonstrations are lacking. Hou et al . used methoxyethyl amine chelants in which the ligands attach...
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| Published in | Science (American Association for the Advancement of Science) Vol. 374; no. 6564; pp. 172 - 178 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
The American Association for the Advancement of Science
08.10.2021
AAAS |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Divalent rechargeable metal batteries such as those based on magnesium and calcium are of interest because of the abundance of these elements and their lower tendency to form dendrites, but practical demonstrations are lacking. Hou
et al
. used methoxyethyl amine chelants in which the ligands attach to the metal atom in more than one place, modulating the solvation structure of the metal ions to enable a facile charge-transfer reaction (see the Perspective by Zuo and Yin). In full battery cells, these components lead to high efficiency and energy density. Theoretical calculations were used to understand the solvation structures. —MSL
Chelating ligands promote fast charge-transfer kinetics for Mg and Ca batteries with substantially lowered overpotentials.
Rechargeable magnesium and calcium metal batteries (RMBs and RCBs) are promising alternatives to lithium-ion batteries because of the high crustal abundance and capacity of magnesium and calcium. Yet, they are plagued by sluggish kinetics and parasitic reactions. We found a family of methoxyethyl-amine chelants that greatly promote interfacial charge transfer kinetics and suppress side reactions on both the cathode and metal anode through solvation sheath reorganization, thus enabling stable and highly reversible cycling of the RMB and RCB full cells with energy densities of 412 and 471 watt-hours per kilogram, respectively. This work provides a versatile electrolyte design strategy for divalent metal batteries. |
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| AbstractList | Rechargeable magnesium and calcium metal batteries (RMBs and RCBs) are promising alternatives to lithium-ion batteries because of the high crustal abundance and capacity of magnesium and calcium. Yet, they are plagued by sluggish kinetics and parasitic reactions. We found a family of methoxyethyl-amine chelants that greatly promote interfacial charge transfer kinetics and suppress side reactions on both the cathode and metal anode through solvation sheath reorganization, thus enabling stable and highly reversible cycling of the RMB and RCB full cells with energy densities of 412 and 471 watt-hours per kilogram, respectively. This work provides a versatile electrolyte design strategy for divalent metal batteries. Divalent rechargeable metal batteries such as those based on magnesium and calcium are of interest because of the abundance of these elements and their lower tendency to form dendrites, but practical demonstrations are lacking. Hou et al . used methoxyethyl amine chelants in which the ligands attach to the metal atom in more than one place, modulating the solvation structure of the metal ions to enable a facile charge-transfer reaction (see the Perspective by Zuo and Yin). In full battery cells, these components lead to high efficiency and energy density. Theoretical calculations were used to understand the solvation structures. —MSL Chelating ligands promote fast charge-transfer kinetics for Mg and Ca batteries with substantially lowered overpotentials. Rechargeable magnesium and calcium metal batteries (RMBs and RCBs) are promising alternatives to lithium-ion batteries because of the high crustal abundance and capacity of magnesium and calcium. Yet, they are plagued by sluggish kinetics and parasitic reactions. We found a family of methoxyethyl-amine chelants that greatly promote interfacial charge transfer kinetics and suppress side reactions on both the cathode and metal anode through solvation sheath reorganization, thus enabling stable and highly reversible cycling of the RMB and RCB full cells with energy densities of 412 and 471 watt-hours per kilogram, respectively. This work provides a versatile electrolyte design strategy for divalent metal batteries. Rechargeable magnesium and calcium metal batteries (RMBs and RCBs) are promising alternatives to lithium-ion batteries because of the high crustal abundance and capacity of magnesium and calcium. Yet, they are plagued by sluggish kinetics and parasitic reactions. We found a family of methoxyethyl-amine chelants that greatly promote interfacial charge transfer kinetics and suppress side reactions on both the cathode and metal anode through solvation sheath reorganization, thus enabling stable and highly reversible cycling of the RMB and RCB full cells with energy densities of 412 and 471 watt-hours per kilogram, respectively. This work provides a versatile electrolyte design strategy for divalent metal batteries.Rechargeable magnesium and calcium metal batteries (RMBs and RCBs) are promising alternatives to lithium-ion batteries because of the high crustal abundance and capacity of magnesium and calcium. Yet, they are plagued by sluggish kinetics and parasitic reactions. We found a family of methoxyethyl-amine chelants that greatly promote interfacial charge transfer kinetics and suppress side reactions on both the cathode and metal anode through solvation sheath reorganization, thus enabling stable and highly reversible cycling of the RMB and RCB full cells with energy densities of 412 and 471 watt-hours per kilogram, respectively. This work provides a versatile electrolyte design strategy for divalent metal batteries. Efficient, rechargeable Mg and Ca batteries Divalent rechargeable metal batteries such as those based on magnesium and calcium are of interest because of the abundance of these elements and their lower tendency to form dendrites, but practical demonstrations are lacking. Houet al. used methoxyethyl amine chelants in which the ligands attach to the metal atom in more than one place, modulating the solvation structure of the metal ions to enable a facile charge-transfer reaction (see the Perspective by Zuo and Yin). In full battery cells, these components lead to high efficiency and energy density. Theoretical calculations were used to understand the solvation structures. —MSL Efficient, rechargeable Mg and Ca batteriesDivalent rechargeable metal batteries such as those based on magnesium and calcium are of interest because of the abundance of these elements and their lower tendency to form dendrites, but practical demonstrations are lacking. Hou et al. used methoxyethyl amine chelants in which the ligands attach to the metal atom in more than one place, modulating the solvation structure of the metal ions to enable a facile charge-transfer reaction (see the Perspective by Zuo and Yin). In full battery cells, these components lead to high efficiency and energy density. Theoretical calculations were used to understand the solvation structures. —MSLRechargeable magnesium and calcium metal batteries (RMBs and RCBs) are promising alternatives to lithium-ion batteries because of the high crustal abundance and capacity of magnesium and calcium. Yet, they are plagued by sluggish kinetics and parasitic reactions. We found a family of methoxyethyl-amine chelants that greatly promote interfacial charge transfer kinetics and suppress side reactions on both the cathode and metal anode through solvation sheath reorganization, thus enabling stable and highly reversible cycling of the RMB and RCB full cells with energy densities of 412 and 471 watt-hours per kilogram, respectively. This work provides a versatile electrolyte design strategy for divalent metal batteries. |
| Author | Wang, Chunsheng Gaskell, Karen Hou, Singyuk Sun, Ruimin Ji, Xiao Wang, Peng-fei Wang, Luning Xu, Jijian Borodin, Oleg |
| Author_xml | – sequence: 1 givenname: Singyuk orcidid: 0000-0002-6444-7632 surname: Hou fullname: Hou, Singyuk organization: Department of Chemical and Biomolecular Engineering, University of Maryland, College Park, MD 20740, USA – sequence: 2 givenname: Xiao orcidid: 0000-0002-7043-5945 surname: Ji fullname: Ji, Xiao organization: Department of Chemical and Biomolecular Engineering, University of Maryland, College Park, MD 20740, USA – sequence: 3 givenname: Karen orcidid: 0000-0003-4389-5994 surname: Gaskell fullname: Gaskell, Karen organization: Department of Chemistry and Biochemistry, University of Maryland, College Park, MD 20742, USA – sequence: 4 givenname: Peng-fei orcidid: 0000-0001-9882-5059 surname: Wang fullname: Wang, Peng-fei organization: Department of Chemical and Biomolecular Engineering, University of Maryland, College Park, MD 20740, USA – sequence: 5 givenname: Luning orcidid: 0000-0002-6656-7013 surname: Wang fullname: Wang, Luning organization: Department of Chemistry and Biochemistry, University of Maryland, College Park, MD 20742, USA – sequence: 6 givenname: Jijian orcidid: 0000-0001-7727-0488 surname: Xu fullname: Xu, Jijian organization: Department of Chemical and Biomolecular Engineering, University of Maryland, College Park, MD 20740, USA – sequence: 7 givenname: Ruimin orcidid: 0000-0002-4464-1016 surname: Sun fullname: Sun, Ruimin organization: Department of Chemical and Biomolecular Engineering, University of Maryland, College Park, MD 20740, USA – sequence: 8 givenname: Oleg orcidid: 0000-0002-9428-5291 surname: Borodin fullname: Borodin, Oleg organization: Battery Science Branch, Sensors and Electron Devices Directorate, US Army Combat Capabilities Development Command Army Research Laboratory, Adelphi, MD 20783, USA – sequence: 9 givenname: Chunsheng orcidid: 0000-0002-8626-6381 surname: Wang fullname: Wang, Chunsheng organization: Department of Chemical and Biomolecular Engineering, University of Maryland, College Park, MD 20740, USA |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/34618574$$D View this record in MEDLINE/PubMed https://www.osti.gov/biblio/1980726$$D View this record in Osti.gov |
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| Snippet | Divalent rechargeable metal batteries such as those based on magnesium and calcium are of interest because of the abundance of these elements and their lower... Rechargeable magnesium and calcium metal batteries (RMBs and RCBs) are promising alternatives to lithium-ion batteries because of the high crustal abundance... Efficient, rechargeable Mg and Ca batteriesDivalent rechargeable metal batteries such as those based on magnesium and calcium are of interest because of the... Efficient, rechargeable Mg and Ca batteries Divalent rechargeable metal batteries such as those based on magnesium and calcium are of interest because of the... |
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| SubjectTerms | Abundance Calcium Charge transfer Dendrites Electrolytic cells Flux density Kinetics Lithium Lithium-ion batteries Magnesium Metal ions Metals Rechargeable batteries Science & Technology - Other Topics Sheaths Side reactions Solvation |
| Title | Solvation sheath reorganization enables divalent metal batteries with fast interfacial charge transfer kinetics |
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