Kinetics of the hydrogen absorption and desorption processes of hydrogen storage alloys: A review

High hydrogen absorption and desorption rates are two significant index parameters for the applications of hydrogen storage tanks. The analysis of the hydrogen absorption and desorption behavior using the isothermal kinetic models is an efficient way to investigate the kinetic mechanism. Multitudino...

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Published inInternational journal of minerals, metallurgy and materials Vol. 29; no. 1; pp. 32 - 48
Main Authors Li, Qian, Lin, Xi, Luo, Qun, Chen, Yu’an, Wang, Jingfeng, Jiang, Bin, Pan, Fusheng
Format Journal Article
LanguageEnglish
Published Beijing University of Science and Technology Beijing 01.01.2022
Springer Nature B.V
National Engineering Research Center for Magnesium Alloys, Chongqing University, Chongqing 400044, China
State Key Laboratory of Advanced Special Steels & Shanghai Key Laboratory of Advanced Ferrometallurgy & School of Materials Science and Engineering,Shanghai University, Shanghai 200444, China%School of Materials Science and Engineering, Shanghai Jiao Tong University, Shanghai 200240, China%State Key Laboratory of Advanced Special Steels & Shanghai Key Laboratory of Advanced Ferrometallurgy & School of Materials Science and Engineering,Shanghai University, Shanghai 200444, China%National Engineering Research Center for Magnesium Alloys, Chongqing University, Chongqing 400044, China
Subjects
Absorption
Alloys
Ceramics
Characterization and Evaluation of Materials
Chemical reactions
Chemisorption
Chemistry and Materials Science
Composites
Corrosion and Coatings
Desorption
Glass
Hydrogen
Hydrogen storage materials
Invited Review
Materials Science
Mathematical models
Measurement methods
Metallic Materials
Natural Materials
Nucleation
Parameters
Pressure effects
Storage tanks
Surfaces and Interfaces
Temperature effects
Thin Films
Tribology
metal hydrides
kinetic models
hydrogen desorption process
hydrogen absorption process
hydrogen storage
metal?hydrides
hydrogen?storage
hydrogen?desorption?process
hydrogen?absorption?process
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Abstract High hydrogen absorption and desorption rates are two significant index parameters for the applications of hydrogen storage tanks. The analysis of the hydrogen absorption and desorption behavior using the isothermal kinetic models is an efficient way to investigate the kinetic mechanism. Multitudinous kinetic models have been developed to describe the kinetic process. However, these kinetic models were deduced based on some assumptions and only appropriate for specific kinetic measurement methods and rate-controlling steps (RCSs), which sometimes lead to confusion during application. The kinetic analysis procedures using these kinetic models, as well as the key kinetic parameters, are unclear for many researchers who are unfamiliar with this field. These problems will prevent the kinetic models and their analysis methods from revealing the kinetic mechanism of hydrogen storage alloys. Thus, this review mainly focuses on the summarization of kinetic models based on different kinetic measurement methods and RCSs for the chemisorption, surface penetration, diffusion of hydrogen, nucleation and growth, and chemical reaction processes. The analysis procedures of kinetic experimental data are expounded, as well as the effects of temperature, hydrogen pressure, and particle radius. The applications of the kinetic models for different hydrogen storage alloys are also introduced.
AbstractList High hydrogen absorption and desorption rates are two significant index parameters for the applications of hydrogen storage tanks. The analysis of the hydrogen absorption and desorption behavior using the isothermal kinetic models is an efficient way to investigate the kinetic mechanism. Multitudinous kinetic models have been developed to describe the kinetic process. However, these kinetic models were deduced based on some assumptions and only appropriate for specific kinetic measurement methods and rate-controlling steps (RCSs), which sometimes lead to confusion during application. The kinetic analysis procedures using these kinetic models, as well as the key kinetic parameters, are unclear for many researchers who are unfamiliar with this field. These problems will prevent the kinetic models and their analysis methods from revealing the kinetic mechanism of hydrogen storage alloys. Thus, this review mainly focuses on the summarization of kinetic models based on different kinetic measurement methods and RCSs for the chemisorption, surface penetration, diffusion of hydrogen, nucleation and growth, and chemical reaction processes. The analysis procedures of kinetic experimental data are expounded, as well as the effects of temperature, hydrogen pressure, and particle radius. The applications of the kinetic models for different hydrogen storage alloys are also introduced.
High hydrogen absorption and desorption rates are two significant index parameters for the applications of hydrogen storage tanks. The analysis of the hydrogen absorption and desorption behavior using the isothermal kinetic models is an efficient way to investigate the kin-etic mechanism. Multitudinous kinetic models have been developed to describe the kinetic process. However, these kinetic models were de-duced based on some assumptions and only appropriate for specific kinetic measurement methods and rate-controlling steps (RCSs), which sometimes lead to confusion during application. The kinetic analysis procedures using these kinetic models, as well as the key kinetic paramet-ers, are unclear for many researchers who are unfamiliar with this field. These problems will prevent the kinetic models and their analysis methods from revealing the kinetic mechanism of hydrogen storage alloys. Thus, this review mainly focuses on the summarization of kinetic models based on different kinetic measurement methods and RCSs for the chemisorption, surface penetration, diffusion of hydrogen, nucle-ation and growth, and chemical reaction processes. The analysis procedures of kinetic experimental data are expounded, as well as the effects of temperature, hydrogen pressure, and particle radius. The applications of the kinetic models for different hydrogen storage alloys are also in-troduced.
Author Li, Qian
Jiang, Bin
Wang, Jingfeng
Luo, Qun
Chen, Yu’an
Pan, Fusheng
Lin, Xi
AuthorAffiliation National Engineering Research Center for Magnesium Alloys, Chongqing University, Chongqing 400044, China;State Key Laboratory of Advanced Special Steels & Shanghai Key Laboratory of Advanced Ferrometallurgy & School of Materials Science and Engineering,Shanghai University, Shanghai 200444, China%School of Materials Science and Engineering, Shanghai Jiao Tong University, Shanghai 200240, China%State Key Laboratory of Advanced Special Steels & Shanghai Key Laboratory of Advanced Ferrometallurgy & School of Materials Science and Engineering,Shanghai University, Shanghai 200444, China%National Engineering Research Center for Magnesium Alloys, Chongqing University, Chongqing 400044, China
AuthorAffiliation_xml – name: National Engineering Research Center for Magnesium Alloys, Chongqing University, Chongqing 400044, China;State Key Laboratory of Advanced Special Steels & Shanghai Key Laboratory of Advanced Ferrometallurgy & School of Materials Science and Engineering,Shanghai University, Shanghai 200444, China%School of Materials Science and Engineering, Shanghai Jiao Tong University, Shanghai 200240, China%State Key Laboratory of Advanced Special Steels & Shanghai Key Laboratory of Advanced Ferrometallurgy & School of Materials Science and Engineering,Shanghai University, Shanghai 200444, China%National Engineering Research Center for Magnesium Alloys, Chongqing University, Chongqing 400044, China
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– sequence: 4
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Issue 1
Keywords metal hydrides
kinetic models
hydrogen desorption process
hydrogen absorption process
hydrogen storage
metal?hydrides
hydrogen?storage
hydrogen?desorption?process
hydrogen?absorption?process
Language English
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PublicationTitle International journal of minerals, metallurgy and materials
PublicationTitleAbbrev Int J Miner Metall Mater
PublicationTitle_FL International Journal of Minerals, Metallurgy and Materials
PublicationYear 2022
Publisher University of Science and Technology Beijing
Springer Nature B.V
National Engineering Research Center for Magnesium Alloys, Chongqing University, Chongqing 400044, China
State Key Laboratory of Advanced Special Steels & Shanghai Key Laboratory of Advanced Ferrometallurgy & School of Materials Science and Engineering,Shanghai University, Shanghai 200444, China%School of Materials Science and Engineering, Shanghai Jiao Tong University, Shanghai 200240, China%State Key Laboratory of Advanced Special Steels & Shanghai Key Laboratory of Advanced Ferrometallurgy & School of Materials Science and Engineering,Shanghai University, Shanghai 200444, China%National Engineering Research Center for Magnesium Alloys, Chongqing University, Chongqing 400044, China
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– name: State Key Laboratory of Advanced Special Steels & Shanghai Key Laboratory of Advanced Ferrometallurgy & School of Materials Science and Engineering,Shanghai University, Shanghai 200444, China%School of Materials Science and Engineering, Shanghai Jiao Tong University, Shanghai 200240, China%State Key Laboratory of Advanced Special Steels & Shanghai Key Laboratory of Advanced Ferrometallurgy & School of Materials Science and Engineering,Shanghai University, Shanghai 200444, China%National Engineering Research Center for Magnesium Alloys, Chongqing University, Chongqing 400044, China
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Snippet High hydrogen absorption and desorption rates are two significant index parameters for the applications of hydrogen storage tanks. The analysis of the hydrogen...
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SubjectTerms Absorption
Alloys
Ceramics
Characterization and Evaluation of Materials
Chemical reactions
Chemisorption
Chemistry and Materials Science
Composites
Corrosion and Coatings
Desorption
Glass
Hydrogen
Hydrogen storage materials
Invited Review
Materials Science
Mathematical models
Measurement methods
Metallic Materials
Natural Materials
Nucleation
Parameters
Pressure effects
Storage tanks
Surfaces and Interfaces
Temperature effects
Thin Films
Tribology
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Title Kinetics of the hydrogen absorption and desorption processes of hydrogen storage alloys: A review
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