Stainless Steel Screen Modified with a Self-Healing Hydrogel for Efficient Gravity-Driven Oil–Water Separation

Due to their low oil adhesion and selective oil–water separation, screens with superhydrophilicity and underwater superoleophobicity have attracted significant attention. However, oil–water separation materials with high efficiency and low cost are still urgently in demand. Here, inspired by natural...

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Published in	Journal of polymers and the environment Vol. 30; no. 5; pp. 2165 - 2175
Main Authors	Li, Bo, Li, Hong, Chen, Ke, Liang, Chen, Luo, Yanping, Xiao, Wenqian, Liu, Xue, Liao, Xiaoling
Format	Journal Article
Language	English
Published	New York Springer US 01.05.2022 Springer Nature B.V
Subjects	adhesion Chemistry Chemistry and Materials Science Coatings Efficiency environment Environmental Chemistry Environmental Engineering/Biotechnology gravity Hydrogels Hydrophilicity Industrial Chemistry/Chemical Engineering Materials Science Mussels Oil oils Original Paper Polyacrylamide Polymer Sciences Separation Stainless steel Stainless steels Underwater Oil–water separation Hydrogel coating Self-healing Underwater superhydrophobicity Superhydrophilic
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Abstract	Due to their low oil adhesion and selective oil–water separation, screens with superhydrophilicity and underwater superoleophobicity have attracted significant attention. However, oil–water separation materials with high efficiency and low cost are still urgently in demand. Here, inspired by natural marine mussels, we prepared a self-healing hydrogel-coated screen to achieve highly efficient oil–water separation. Polydopamine (PDA) was incorporated into polyacrylamide (PAM) and uniformly coated on a stainless steel screen to prepare a self-healing hydrogel-coated screen. The results showed that the PDA-PAM hydrogel coating firmly adhered to the stainless steel screen and exhibited superhydrophilicity and underwater superoleophobicity. Regarding the PDA-PAM hydrogel-modified screen with a coating time of 7 min, different types of oil–water mixtures could be driven by gravity to achieve a highly efficient oil–water separation rate of over 97%, and the water flux could reach 91,673 L m −2 h −1 . After ten cycles, the separation efficiency did not decrease significantly, suggesting that the self-healing hydrogel-coated screen has excellent stability and recycling performance. This inexpensive novel filter screen with high efficiency has a wide range of potential application in the field of oil–water separation.
AbstractList	Due to their low oil adhesion and selective oil–water separation, screens with superhydrophilicity and underwater superoleophobicity have attracted significant attention. However, oil–water separation materials with high efficiency and low cost are still urgently in demand. Here, inspired by natural marine mussels, we prepared a self-healing hydrogel-coated screen to achieve highly efficient oil–water separation. Polydopamine (PDA) was incorporated into polyacrylamide (PAM) and uniformly coated on a stainless steel screen to prepare a self-healing hydrogel-coated screen. The results showed that the PDA-PAM hydrogel coating firmly adhered to the stainless steel screen and exhibited superhydrophilicity and underwater superoleophobicity. Regarding the PDA-PAM hydrogel-modified screen with a coating time of 7 min, different types of oil–water mixtures could be driven by gravity to achieve a highly efficient oil–water separation rate of over 97%, and the water flux could reach 91,673 L m−2 h−1. After ten cycles, the separation efficiency did not decrease significantly, suggesting that the self-healing hydrogel-coated screen has excellent stability and recycling performance. This inexpensive novel filter screen with high efficiency has a wide range of potential application in the field of oil–water separation. Due to their low oil adhesion and selective oil–water separation, screens with superhydrophilicity and underwater superoleophobicity have attracted significant attention. However, oil–water separation materials with high efficiency and low cost are still urgently in demand. Here, inspired by natural marine mussels, we prepared a self-healing hydrogel-coated screen to achieve highly efficient oil–water separation. Polydopamine (PDA) was incorporated into polyacrylamide (PAM) and uniformly coated on a stainless steel screen to prepare a self-healing hydrogel-coated screen. The results showed that the PDA-PAM hydrogel coating firmly adhered to the stainless steel screen and exhibited superhydrophilicity and underwater superoleophobicity. Regarding the PDA-PAM hydrogel-modified screen with a coating time of 7 min, different types of oil–water mixtures could be driven by gravity to achieve a highly efficient oil–water separation rate of over 97%, and the water flux could reach 91,673 L m⁻² h⁻¹. After ten cycles, the separation efficiency did not decrease significantly, suggesting that the self-healing hydrogel-coated screen has excellent stability and recycling performance. This inexpensive novel filter screen with high efficiency has a wide range of potential application in the field of oil–water separation. Due to their low oil adhesion and selective oil–water separation, screens with superhydrophilicity and underwater superoleophobicity have attracted significant attention. However, oil–water separation materials with high efficiency and low cost are still urgently in demand. Here, inspired by natural marine mussels, we prepared a self-healing hydrogel-coated screen to achieve highly efficient oil–water separation. Polydopamine (PDA) was incorporated into polyacrylamide (PAM) and uniformly coated on a stainless steel screen to prepare a self-healing hydrogel-coated screen. The results showed that the PDA-PAM hydrogel coating firmly adhered to the stainless steel screen and exhibited superhydrophilicity and underwater superoleophobicity. Regarding the PDA-PAM hydrogel-modified screen with a coating time of 7 min, different types of oil–water mixtures could be driven by gravity to achieve a highly efficient oil–water separation rate of over 97%, and the water flux could reach 91,673 L m −2 h −1 . After ten cycles, the separation efficiency did not decrease significantly, suggesting that the self-healing hydrogel-coated screen has excellent stability and recycling performance. This inexpensive novel filter screen with high efficiency has a wide range of potential application in the field of oil–water separation.
Author	Li, Bo Liang, Chen Liao, Xiaoling Li, Hong Liu, Xue Luo, Yanping Xiao, Wenqian Chen, Ke
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SubjectTerms	adhesion Chemistry Chemistry and Materials Science Coatings Efficiency environment Environmental Chemistry Environmental Engineering/Biotechnology gravity Hydrogels Hydrophilicity Industrial Chemistry/Chemical Engineering Materials Science Mussels Oil oils Original Paper Polyacrylamide Polymer Sciences Separation Stainless steel Stainless steels Underwater
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Title	Stainless Steel Screen Modified with a Self-Healing Hydrogel for Efficient Gravity-Driven Oil–Water Separation
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