Construction of 3D marigold-like direct Z-scheme heterojunction In2O3/CdS with boosted photocatalytic degradation of antibiotics under visible light
In the present work, a 3D marigold-like direct Z-scheme heterojunction photocatalyst of In2O3/CdS was fabricated through in-situ growth technology. Both characterization and experiment results show that the as-synthetised In2O3/CdS possesses outstanding reusability and stability, and high separation...
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| Published in | Colloid and interface science communications Vol. 51; p. 100674 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.11.2022
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| Subjects | |
| Online Access | Get full text |
| ISSN | 2215-0382 2215-0382 |
| DOI | 10.1016/j.colcom.2022.100674 |
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| Abstract | In the present work, a 3D marigold-like direct Z-scheme heterojunction photocatalyst of In2O3/CdS was fabricated through in-situ growth technology. Both characterization and experiment results show that the as-synthetised In2O3/CdS possesses outstanding reusability and stability, and high separation rates of photogenerated e−/h+ pairs. The catalyst of In2O3/CdS has a satisfactory degradation efficiency of 84.8% for doxycycline hydrochloride and 79.0% for levofloxacin within 60 min. Doxycycline hydrochloride and levofloxacin are eventually destroyed and decomposed by •O2−, •OH and h+ radicals resulted from In2O3/CdS under vis-light. And the contribution of free radicals follow the order of •O2− > •OH > h+. The transfer path of e−/h+ and the generation of •O2−and •OH in the In2O3/CdS are attributed to the formation of Z-scheme heterojunction. Generally, the heterojunction formation between In2O3 and CdS is more conducive to the improvement of photocatalytic performance. The as-synthetised heterojunction In2O3/CdS is a quite promising photocatalyst in water pollution controlling.
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•3D direct Z-scheme heterojunction In2O3/CdS was obtained by in-situ growth method.•In2O3/CdS can effectively degrade two different antibiotics under vis-light.•Z-scheme heterojunction promotes the transfer of e−/h+ and formation of •O2− and •OH.•Antibiotics of DH and LV can be completely mineralized by heterojunction In2O3/CdS. |
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| AbstractList | In the present work, a 3D marigold-like direct Z-scheme heterojunction photocatalyst of In2O3/CdS was fabricated through in-situ growth technology. Both characterization and experiment results show that the as-synthetised In2O3/CdS possesses outstanding reusability and stability, and high separation rates of photogenerated e−/h+ pairs. The catalyst of In2O3/CdS has a satisfactory degradation efficiency of 84.8% for doxycycline hydrochloride and 79.0% for levofloxacin within 60 min. Doxycycline hydrochloride and levofloxacin are eventually destroyed and decomposed by •O2−, •OH and h+ radicals resulted from In2O3/CdS under vis-light. And the contribution of free radicals follow the order of •O2− > •OH > h+. The transfer path of e−/h+ and the generation of •O2−and •OH in the In2O3/CdS are attributed to the formation of Z-scheme heterojunction. Generally, the heterojunction formation between In2O3 and CdS is more conducive to the improvement of photocatalytic performance. The as-synthetised heterojunction In2O3/CdS is a quite promising photocatalyst in water pollution controlling.
[Display omitted]
•3D direct Z-scheme heterojunction In2O3/CdS was obtained by in-situ growth method.•In2O3/CdS can effectively degrade two different antibiotics under vis-light.•Z-scheme heterojunction promotes the transfer of e−/h+ and formation of •O2− and •OH.•Antibiotics of DH and LV can be completely mineralized by heterojunction In2O3/CdS. |
| ArticleNumber | 100674 |
| Author | Wang, Ting Huang, Tianyin Guo, Yongfu Zheng, Xinyu Zeng, Zheng Yang, Jingjing Pan, Ziwei |
| Author_xml | – sequence: 1 givenname: Ting surname: Wang fullname: Wang, Ting organization: Department of Municipal Engineering, Suzhou University of Science and Technology, Suzhou 215009, China – sequence: 2 givenname: Zheng surname: Zeng fullname: Zeng, Zheng organization: Department of Municipal Engineering, Suzhou University of Science and Technology, Suzhou 215009, China – sequence: 3 givenname: Jingjing surname: Yang fullname: Yang, Jingjing organization: Department of Municipal Engineering, Suzhou University of Science and Technology, Suzhou 215009, China – sequence: 4 givenname: Ziwei surname: Pan fullname: Pan, Ziwei organization: Department of Municipal Engineering, Suzhou University of Science and Technology, Suzhou 215009, China – sequence: 5 givenname: Xinyu surname: Zheng fullname: Zheng, Xinyu organization: Department of Municipal Engineering, Suzhou University of Science and Technology, Suzhou 215009, China – sequence: 6 givenname: Yongfu surname: Guo fullname: Guo, Yongfu email: yongfuguo@163.com organization: Department of Municipal Engineering, Suzhou University of Science and Technology, Suzhou 215009, China – sequence: 7 givenname: Tianyin surname: Huang fullname: Huang, Tianyin organization: Department of Municipal Engineering, Suzhou University of Science and Technology, Suzhou 215009, China |
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| Keywords | Degradation Antibiotics Indium oxide Z-scheme heterojunction Photocatalysis |
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| Snippet | In the present work, a 3D marigold-like direct Z-scheme heterojunction photocatalyst of In2O3/CdS was fabricated through in-situ growth technology. Both... |
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| SubjectTerms | Antibiotics Degradation Indium oxide Photocatalysis Z-scheme heterojunction |
| Title | Construction of 3D marigold-like direct Z-scheme heterojunction In2O3/CdS with boosted photocatalytic degradation of antibiotics under visible light |
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