DSC study of antioxidant activity of selected p-phenylenediamines in styrene-butadiene rubber
The antioxidant activity of selected N,N′-substituted p -phenylenediamines (PPDs) in styrene-butadiene rubber (SBR) has been studied by differential scanning calorimetry under non-isothermal conditions. The kinetic parameters describing temperature dependence of induction period have been obtained....
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| Published in | Journal of thermal analysis and calorimetry Vol. 97; no. 2; pp. 535 - 540 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
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Dordrecht
Springer Netherlands
01.08.2009
Springer |
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| Abstract | The antioxidant activity of selected N,N′-substituted
p
-phenylenediamines (PPDs) in styrene-butadiene rubber (SBR) has been studied by differential scanning calorimetry under non-isothermal conditions. The kinetic parameters describing temperature dependence of induction period have been obtained. Protection factors and antioxidant effectiveness have been calculated to characterize the stabilizing effect of the antioxidants under study. It is shown that all antioxidants under study exhibit stabilizing effect on SBR. The obtained values were used to compare the stabilizing effect of the same antioxidants in polyisoprene (PI) rubber. The order of stability for SBR matrix samples differs from that for PI samples. It is shown that the stabilization effect of the antioxidant depends much on the polymer matrix. |
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| AbstractList | The antioxidant activity of selected N,N'-substituted p-phenylenediamines (PPDs) in styrene-butadiene rubber (SBR) has been studied by differential scanning calorimetry under non-isothermal conditions. The kinetic parameters describing temperature dependence of induction period have been obtained. Protection factors and antioxidant effectiveness have been calculated to characterize the stabilizing effect of the antioxidants under study. It is shown that all antioxidants under study exhibit stabilizing effect on SBR. The obtained values were used to compare the stabilizing effect of the same antioxidants in polyisoprene (PI) rubber. The order of stability for SBR matrix samples differs from that for PI samples. It is shown that the stabilization effect of the antioxidant depends much on the polymer matrix. The antioxidant activity of selected N,N′-substituted p -phenylenediamines (PPDs) in styrene-butadiene rubber (SBR) has been studied by differential scanning calorimetry under non-isothermal conditions. The kinetic parameters describing temperature dependence of induction period have been obtained. Protection factors and antioxidant effectiveness have been calculated to characterize the stabilizing effect of the antioxidants under study. It is shown that all antioxidants under study exhibit stabilizing effect on SBR. The obtained values were used to compare the stabilizing effect of the same antioxidants in polyisoprene (PI) rubber. The order of stability for SBR matrix samples differs from that for PI samples. It is shown that the stabilization effect of the antioxidant depends much on the polymer matrix. |
| Author | Lehocký, P. Šimon, P. Chochulová, A. Cibulková, Zuzana Kosár, K. |
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| CitedBy_id | crossref_primary_10_1002_pc_22666 crossref_primary_10_1016_j_polymdegradstab_2016_06_013 crossref_primary_10_1016_j_polymdegradstab_2020_109438 crossref_primary_10_1016_j_scitotenv_2022_154675 crossref_primary_10_4028_www_scientific_net_AMM_152_154_28 crossref_primary_10_1016_j_cplett_2015_09_013 crossref_primary_10_1016_j_cplett_2015_09_035 crossref_primary_10_1007_s10973_015_4893_5 crossref_primary_10_1016_j_foodchem_2013_11_011 crossref_primary_10_1016_j_polymdegradstab_2017_07_027 crossref_primary_10_1016_j_polymdegradstab_2020_109196 crossref_primary_10_1016_j_cplett_2017_05_036 crossref_primary_10_1016_j_tca_2018_08_009 crossref_primary_10_1007_s10965_024_04006_3 crossref_primary_10_1016_j_polymdegradstab_2012_06_012 crossref_primary_10_1016_j_polymdegradstab_2015_01_019 crossref_primary_10_1002_vnl_21901 crossref_primary_10_1007_s10973_014_4167_7 crossref_primary_10_1007_s10973_011_1963_1 crossref_primary_10_1134_S1070363216020262 crossref_primary_10_1007_s10973_014_4382_2 crossref_primary_10_1016_j_polymdegradstab_2016_02_028 crossref_primary_10_1007_s10973_011_1322_2 |
| Cites_doi | 10.1007/s10973-005-7204-z 10.1016/j.polymdegradstab.2005.02.007 10.1016/S0168-583X(01)00970-3 10.1007/s10973-005-0660-3 10.1016/S0014-3057(01)00248-8 10.1023/A:1010148810569 10.1016/S0141-3910(01)00017-9 10.1016/j.polymdegradstab.2004.10.004 10.1016/S0141-3910(03)00210-6 10.1007/s11746-000-0103-8 10.1016/S0142-9418(99)00030-6 10.1023/A:1013950426882 10.1081/SCC-200032408 10.1093/comjnl/7.4.308 |
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| Keywords | protection factor N,N′-substituted antioxidants DSC induction periods antioxidant effectiveness oxidation p-phenylenediamines styrenebutadiene rubber Differential scanning calorimetry SBR Thermooxidative degradation Antioxidant Induction period Diamine Oxidation Thermal analysis Rubber Aromatic amine N,N'-substituted |
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| References | PospíšilJ.HorákJ.PilaìJ.BillinghamN. C.ZweifelH.Polym. Degrad. Stab.20038214510.1016/S0141-3910(03)00210-6 SigmundováI.UhlárJ.TomaSynth. Commun.200434366710.1081/SCC-200032408 CataldoF.Eur. Polym. J.20023888510.1016/S0014-3057(01)00248-81:CAS:528:DC%2BD38Xhslersb0%3D ParraD. F.do Rosario MatosJ.J. Therm. Anal. Cal.20026728710.1023/A:10139504268821:CAS:528:DC%2BD38Xit1Cnu7c%3D CibulkováZ.ŠimonP.LehockýP.BalkoJ.J. Therm. Anal. Cal.20058035710.1007/s10973-005-0660-3 Abdel-AzizM. M.BasfarA. A.Polym. Test.20001959110.1016/S0142-9418(99)00030-61:CAS:528:DC%2BD3cXjtFyqsbY%3D CataldoF.Polym. Degrad. Stab.20017278710.1016/S0141-3910(01)00017-9 ŠimonP.J. Therm. Anal. Cal.20068426310.1007/s10973-005-7204-z ŠimonP.KučmaA.J. Therm. Anal. Cal.199956110710.1023/A:1010148810569 NelderJ. A.MeadR.Computer J.19657308 GregorováA.CibulkováZ.KošíkováB.ŠimonP.Polym. Degrad. Stab.20058955310.1016/j.polymdegradstab.2005.02.007 ŠimonP.KolmanNiklováI.SchmidtJ. Am. Oil Chem. Soc.20007763910.1007/s11746-000-0103-8 Abdel-AzizM. M.BasfarA. A.Nucl. Instrum. Methods Phys. Res. B200118534610.1016/S0168-583X(01)00970-31:CAS:528:DC%2BD3MXptFOltbg%3D CibulkováZ.ŠimonP.LehockýP.BalkoJ.Polym. Degrad. Stab.20058747910.1016/j.polymdegradstab.2004.10.004 J. Pospíšil (9628_CR1) 2003; 82 F. Cataldo (9628_CR2) 2002; 38 F. Cataldo (9628_CR3) 2001; 72 I. Sigmundová (9628_CR13) 2004; 34 Z. Cibulková (9628_CR11) 2005; 87 M. M. Abdel-Aziz (9628_CR4) 2001; 185 Z. Cibulková (9628_CR12) 2005; 80 P. Šimon (9628_CR9) 2000; 77 P. Šimon (9628_CR8) 1999; 56 A. Gregorová (9628_CR10) 2005; 89 M. M. Abdel-Aziz (9628_CR5) 2000; 19 P. Šimon (9628_CR7) 2006; 84 D. F. Parra (9628_CR6) 2002; 67 J. A. Nelder (9628_CR14) 1965; 7 |
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p
-phenylenediamines (PPDs) in styrene-butadiene rubber (SBR) has been studied by differential scanning... The antioxidant activity of selected N,N'-substituted p-phenylenediamines (PPDs) in styrene-butadiene rubber (SBR) has been studied by differential scanning... |
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| SubjectTerms | Analytical Chemistry Antioxidants Applied sciences Calorimetry Chemical reactions and properties Chemistry Chemistry and Materials Science Degradation Differential scanning calorimetry Exact sciences and technology Inorganic Chemistry Mathematical analysis Measurement Science and Instrumentation Organic polymers Physical Chemistry Physicochemistry of polymers Polyimide resins Polymer Sciences Rubber Stabilization Temperature dependence |
| Title | DSC study of antioxidant activity of selected p-phenylenediamines in styrene-butadiene rubber |
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