Metal-organic framework structure-property relationships for high-performance multifunctional polymer nanocomposite applications

Metal-organic frameworks (MOFs) have emerged as a new class of crystalline nanomaterials with ultrahigh porosities and high internal surface areas. Recently, these MOF structures with their extraordinary inherent properties have become potential candidates for specific technologies in areas such as...

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Published inJournal of materials chemistry. A, Materials for energy and sustainability Vol. 9; no. 8; pp. 4348 - 4378
Main Authors Unnikrishnan, Vishnu, Zabihi, Omid, Ahmadi, Mojtaba, Li, Quanxiang, Blanchard, Patrick, Kiziltas, Alper, Naebe, Minoo
Format Journal Article
LanguageEnglish
Published Cambridge Royal Society of Chemistry 02.03.2021
Subjects
Aerospace industry
Boron
Boron nitride
chemistry
Composite structures
coordination polymers
Defense industry
Graphene
Hybrid composites
Hybridization
Industrial applications
Mechanical properties
Metal-organic frameworks
Nanocomposites
Nanomaterials
Nanotechnology
polymer nanocomposites
Polymers
Porous materials
Substrates
Synthesis
Online AccessGet full text
ISSN2050-7488
2050-7496
2050-7496
DOI10.1039/d0ta11255k

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Abstract Metal-organic frameworks (MOFs) have emerged as a new class of crystalline nanomaterials with ultrahigh porosities and high internal surface areas. Recently, these MOF structures with their extraordinary inherent properties have become potential candidates for specific technologies in areas such as the automotive, defence, and aerospace industries. Conversely, polymeric materials are common in a wide variety of industrial applications due to their unique properties and versatile performance. The idea of hybridising MOFs and polymers purely for their distinct superior properties has led to the concept of hybrid composite structures, which exhibit the inherent properties of the two different materials. However, MOFs by themselves have always been considered as labile reinforcements for polymers to afford multifunctional nanocomposites. Therefore, to improve the interactions between MOFs and polymers, it is imperative to understand the factors affecting the inherent MOF properties. This review briefly presents approaches for the synthesis, functionalisation, and post-synthesis modification of MOFs, and the opportunities and challenges for the utilisation of MOFs in high-performance, multifunctional polymer nanocomposites are comprehensively reviewed. In this regard, a wide range of properties related to multifunctional polymer nanocomposites, with a focus on mechanical properties and flame retardancy, are presented. Recent trends in the hybridisation of MOFs with various substrates and other two-dimensional nanomaterials such as graphene and boron nitrides are also discussed. This review highlights the potential of MOFs as versatile porous materials for the development of novel hybrid fillers which could represent remarkable advances in the field of high-performance multifunctional composites. Metal-organic frameworks (MOFs) have emerged as a new class of crystalline nanomaterials with ultrahigh porosities and high internal surface areas.
AbstractList Metal–organic frameworks (MOFs) have emerged as a new class of crystalline nanomaterials with ultrahigh porosities and high internal surface areas. Recently, these MOF structures with their extraordinary inherent properties have become potential candidates for specific technologies in areas such as the automotive, defence, and aerospace industries. Conversely, polymeric materials are common in a wide variety of industrial applications due to their unique properties and versatile performance. The idea of hybridising MOFs and polymers purely for their distinct superior properties has led to the concept of hybrid composite structures, which exhibit the inherent properties of the two different materials. However, MOFs by themselves have always been considered as labile reinforcements for polymers to afford multifunctional nanocomposites. Therefore, to improve the interactions between MOFs and polymers, it is imperative to understand the factors affecting the inherent MOF properties. This review briefly presents approaches for the synthesis, functionalisation, and post-synthesis modification of MOFs, and the opportunities and challenges for the utilisation of MOFs in high-performance, multifunctional polymer nanocomposites are comprehensively reviewed. In this regard, a wide range of properties related to multifunctional polymer nanocomposites, with a focus on mechanical properties and flame retardancy, are presented. Recent trends in the hybridisation of MOFs with various substrates and other two-dimensional nanomaterials such as graphene and boron nitrides are also discussed. This review highlights the potential of MOFs as versatile porous materials for the development of novel hybrid fillers which could represent remarkable advances in the field of high-performance multifunctional composites.
Metal-organic frameworks (MOFs) have emerged as a new class of crystalline nanomaterials with ultrahigh porosities and high internal surface areas. Recently, these MOF structures with their extraordinary inherent properties have become potential candidates for specific technologies in areas such as the automotive, defence, and aerospace industries. Conversely, polymeric materials are common in a wide variety of industrial applications due to their unique properties and versatile performance. The idea of hybridising MOFs and polymers purely for their distinct superior properties has led to the concept of hybrid composite structures, which exhibit the inherent properties of the two different materials. However, MOFs by themselves have always been considered as labile reinforcements for polymers to afford multifunctional nanocomposites. Therefore, to improve the interactions between MOFs and polymers, it is imperative to understand the factors affecting the inherent MOF properties. This review briefly presents approaches for the synthesis, functionalisation, and post-synthesis modification of MOFs, and the opportunities and challenges for the utilisation of MOFs in high-performance, multifunctional polymer nanocomposites are comprehensively reviewed. In this regard, a wide range of properties related to multifunctional polymer nanocomposites, with a focus on mechanical properties and flame retardancy, are presented. Recent trends in the hybridisation of MOFs with various substrates and other two-dimensional nanomaterials such as graphene and boron nitrides are also discussed. This review highlights the potential of MOFs as versatile porous materials for the development of novel hybrid fillers which could represent remarkable advances in the field of high-performance multifunctional composites. Metal-organic frameworks (MOFs) have emerged as a new class of crystalline nanomaterials with ultrahigh porosities and high internal surface areas.
Author Blanchard, Patrick
Unnikrishnan, Vishnu
Li, Quanxiang
Zabihi, Omid
Ahmadi, Mojtaba
Kiziltas, Alper
Naebe, Minoo
AuthorAffiliation Deakin University
Ford Motor Company
Institute for Frontier Materials
Research and Product Development
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PublicationCentury 2000
PublicationDate 20210302
PublicationDateYYYYMMDD 2021-03-02
PublicationDate_xml – month: 3
  year: 2021
  text: 20210302
  day: 2
PublicationDecade 2020
PublicationPlace Cambridge
PublicationPlace_xml – name: Cambridge
PublicationTitle Journal of materials chemistry. A, Materials for energy and sustainability
PublicationYear 2021
Publisher Royal Society of Chemistry
Publisher_xml – name: Royal Society of Chemistry
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Snippet Metal-organic frameworks (MOFs) have emerged as a new class of crystalline nanomaterials with ultrahigh porosities and high internal surface areas. Recently,...
Metal–organic frameworks (MOFs) have emerged as a new class of crystalline nanomaterials with ultrahigh porosities and high internal surface areas. Recently,...
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SubjectTerms Aerospace industry
Boron
Boron nitride
chemistry
Composite structures
coordination polymers
Defense industry
Graphene
Hybrid composites
Hybridization
Industrial applications
Mechanical properties
Metal-organic frameworks
Nanocomposites
Nanomaterials
Nanotechnology
polymer nanocomposites
Polymers
Porous materials
Substrates
Synthesis
Title Metal-organic framework structure-property relationships for high-performance multifunctional polymer nanocomposite applications
URI https://www.proquest.com/docview/2494900840
https://www.proquest.com/docview/2551990780
Volume 9
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