Effects of the Discharge Parameters on the Efficiency and Stability of Ambient Metastable-Induced Desorption Ionization

Ionization efficiency is an important factor for ion sources in mass spectrometry and ion mobility spectrometry.Using helium as the discharge gas,acetone as the sample,and high-field asymmetric ion mobility spectrometry（FAIMS） as the ion detection method,this work investigates in detail the effects...

Full description

Saved in:
Bibliographic Details
Published inPlasma science & technology Vol. 17; no. 12; pp. 1048 - 1052
Main Author 张晓天 陈池来 刘友江 王泓伟 张乐华 孔德义 Mario CHAVARRIA
Format Journal Article
LanguageEnglish
Published 01.12.2015
Subjects
Desorption
Discharge
Ion mobility
Ionic mobility
Ionization
Mass spectrometry
Spectrometry
Spectroscopy
亚稳态
放电参数
环境
电离效率
离子迁移谱
稳定性
解吸
诱导
Online AccessGet full text
ISSN1009-0630
DOI10.1088/1009-0630/17/12/12

Cover

Abstract Ionization efficiency is an important factor for ion sources in mass spectrometry and ion mobility spectrometry.Using helium as the discharge gas,acetone as the sample,and high-field asymmetric ion mobility spectrometry（FAIMS） as the ion detection method,this work investigates in detail the effects of discharge parameters on the efficiency of ambient metastableinduced desorption ionization（AMDI） at atmospheric pressure.The results indicate that the discharge power and gas flow rate are both significantly correlated with the ionization efficiency.Specifically,an increase in the applied discharge power leads to a rapid increase in the ionization efficiency,which gradually reaches equilibrium due to ion saturation.Moreover,when the discharge voltage is fixed at 2.1 kV,a maximum efficiency can be achieved at the flow rate of 9.0 m/s.This study provides a foundation for the design and application of AMDI for on-line detection with mass spectrometry and ion mobility spectrometry.
AbstractList Ionization efficiency is an important factor for ion sources in mass spectrometry and ion mobility spectrometry.Using helium as the discharge gas,acetone as the sample,and high-field asymmetric ion mobility spectrometry（FAIMS） as the ion detection method,this work investigates in detail the effects of discharge parameters on the efficiency of ambient metastableinduced desorption ionization（AMDI） at atmospheric pressure.The results indicate that the discharge power and gas flow rate are both significantly correlated with the ionization efficiency.Specifically,an increase in the applied discharge power leads to a rapid increase in the ionization efficiency,which gradually reaches equilibrium due to ion saturation.Moreover,when the discharge voltage is fixed at 2.1 kV,a maximum efficiency can be achieved at the flow rate of 9.0 m/s.This study provides a foundation for the design and application of AMDI for on-line detection with mass spectrometry and ion mobility spectrometry.
Ionization efficiency is an important factor for ion sources in mass spectrometry and ion mobility spectrometry. Using helium as the discharge gas, acetone as the sample, and high-field asymmetric ion mobility spectrometry (FAIMS) as the ion detection method, this work investigates in detail the effects of discharge parameters on the efficiency of ambient metastable-induced desorption ionization (AMDI) at atmospheric pressure. The results indicate that the discharge power and gas flow rate are both significantly correlated with the ionization efficiency. Specifically, an increase in the applied discharge power leads to a rapid increase in the ionization efficiency, which gradually reaches equilibrium due to ion saturation. Moreover, when the discharge voltage is fixed at 2.1 kV, a maximum efficiency can be achieved at the flow rate of 9.0 m/s. This study provides a foundation for the design and application of AMDI for on-line detection with mass spectrometry and ion mobility spectrometry.
Author 张晓天 陈池来 刘友江 王泓伟 张乐华 孔德义 Mario CHAVARRIA
AuthorAffiliation State Key Laboratory of Transducer Technology, Hefei Institute of Intelligent Machines, CAS, Hefei 230031, China College of Electronic Science and Applied Physics, University of Technology, Hefei 2300111 China Department of Automation, University of Science and Technology of China, Hefei 230027,China Microsystems Laboratory, Ecole Polytechnique Federale de Lausanne （EPFL）, CH-1015 Lausanne, Switzerland
Author_xml – sequence: 1
  fullname: 张晓天 陈池来 刘友江 王泓伟 张乐华 孔德义 Mario CHAVARRIA
BookMark eNp9kE1LAzEQhnNQsFX_gKfFk5e1-dikm6PUr4KiYO8hm520kW22TVKk_nqzWjx4EAYS5n2fYeYdoyPfe0DoguBrgut6QjCWJRYMT8h0QmiuIzT6bZ6gcYzvGPNK1myEPu6sBZNi0dsiraC4ddGsdFhC8aqDXkOCkDX_rWWrMw682Rfat8Vb0o3rXNoP7M26yUoqniHpmIUOyrlvdwba4hZiHzbJ5Snz3rtPPXzP0LHVXYTzw3uKFvd3i9lj-fTyMJ_dPJWGcZLKqrKNhdoya6aildQY1lJesyk3jWZcg8GaCdwwIUlLcd1ISkgrrDRUNJizU3T1M3YT-u0OYlLrfCB0nfbQ76IiNeUV5xJX2Vr_WE3oYwxglXHpe9cUtOsUwWqIVw1JqiFJRaaK0FwZpX_QTXBrHfb_Q5cHaNX75db55S8lhJBYSi7YF3bhjek
CitedBy_id crossref_primary_10_1039_C7AY00965H
crossref_primary_10_3390_mi10050286
Cites_doi 10.1021/ac8022108
10.1088/1009-0630/11/1/10
10.5059/yukigoseikyokaishi.69.171
10.1007/s00216-013-7316-0
10.1021/ac901122b
10.1088/1009-0630/15/9/02
10.1002/jms.1243
10.5194/acp-9-4177-2009
10.1021/ac802117u
10.1016/j.jasms.2007.07.027
10.1021/ac050162j
10.1021/ac801641a
10.1002/rcm.6198
10.1016/j.aca.2014.06.014
10.1007/s00216-012-6536-z
10.1103/PhysRev.11.316
ContentType Journal Article
DBID 2RA
92L
CQIGP
W92
~WA
AAYXX
CITATION
7U5
8FD
H8D
L7M
DOI 10.1088/1009-0630/17/12/12
DatabaseName 维普期刊资源整合服务平台
中文科技期刊数据库-CALIS站点
中文科技期刊数据库-7.0平台
中文科技期刊数据库-工程技术
中文科技期刊数据库- 镜像站点
CrossRef
Solid State and Superconductivity Abstracts
Technology Research Database
Aerospace Database
Advanced Technologies Database with Aerospace
DatabaseTitle CrossRef
Aerospace Database
Solid State and Superconductivity Abstracts
Technology Research Database
Advanced Technologies Database with Aerospace
DatabaseTitleList
Aerospace Database
DeliveryMethod fulltext_linktorsrc
Discipline Physics
DocumentTitleAlternate Effects of the Discharge Parameters on the Efficiency and Stability of Ambient Metastable-Induced Desorption Ionization
EndPage 1052
ExternalDocumentID 10_1088_1009_0630_17_12_12
666909956
GroupedDBID 02O
042
123
1JI
1WK
2B.
2C.
2RA
4.4
5B3
5VR
5VS
5ZH
7.M
7.Q
92E
92I
92L
92Q
93N
AAGCD
AAJIO
AAJKP
AALHV
AATNI
ABHWH
ABQJV
ACAFW
ACGFS
ACHIP
AEFHF
AENEX
AFUIB
AFYNE
AHSEE
AKPSB
ALMA_UNASSIGNED_HOLDINGS
BBWZM
CCEZO
CCVFK
CEBXE
CHBEP
CJUJL
CQIGP
CRLBU
CS3
CW9
DU5
EBS
EDWGO
EJD
EMSAF
EPQRW
EQZZN
FA0
HAK
IJHAN
IOP
IZVLO
JCGBZ
KNG
KOT
LAP
M45
N5L
N9A
NS0
NT-
NT.
P2P
PJBAE
Q02
R4D
RIN
RNS
RO9
ROL
RPA
RW3
S3P
SY9
T37
TCJ
TGP
W28
W92
~WA
-SA
-S~
AAYXX
ACARI
ADEQX
AERVB
AGQPQ
AOAED
ARNYC
CAJEA
CITATION
Q--
U1G
U5K
7U5
8FD
AEINN
H8D
L7M
ID FETCH-LOGICAL-c351t-44fbfe8f3fc76d92cc3d258375cba35aec0a360b3691d208b9211d6f9c26b053
ISSN 1009-0630
IngestDate Tue Aug 05 11:05:54 EDT 2025
Thu Apr 24 23:02:37 EDT 2025
Tue Jul 01 03:44:31 EDT 2025
Wed Feb 14 10:23:46 EST 2024
IsDoiOpenAccess false
IsOpenAccess true
IsPeerReviewed true
IsScholarly true
Issue 12
Language English
License http://iopscience.iop.org/info/page/text-and-data-mining
http://iopscience.iop.org/page/copyright
LinkModel OpenURL
MergedId FETCHMERGED-LOGICAL-c351t-44fbfe8f3fc76d92cc3d258375cba35aec0a360b3691d208b9211d6f9c26b053
Notes ZHANG Xiaotian, CHEN Chilai, LIU Youjiang , WANG Hongwei, ZHANG Lehua ,KONG Deyi ,Mario CHAVARRIA（ 1State Key Laboratory of Transducer Technology, Hefei Institute of Intelligent Machines, CAS, Hefei 230031, China; 2College of Electronic Science and Applied Physics, University of Technology, Hefei 2300111 China ;3Department of Automation, University of Science and Technology of China, Hefei 230027,China ;4Microsystems Laboratory, Ecole Polytechnique Federale de Lausanne （EPFL）, CH-1015 Lausanne, Switzerland）
34-1187/TL
ambient helium ionization asymmetric desorption metastable saturation acetone reaches unexpected
Ionization efficiency is an important factor for ion sources in mass spectrometry and ion mobility spectrometry.Using helium as the discharge gas,acetone as the sample,and high-field asymmetric ion mobility spectrometry（FAIMS） as the ion detection method,this work investigates in detail the effects of discharge parameters on the efficiency of ambient metastableinduced desorption ionization（AMDI） at atmospheric pressure.The results indicate that the discharge power and gas flow rate are both significantly correlated with the ionization efficiency.Specifically,an increase in the applied discharge power leads to a rapid increase in the ionization efficiency,which gradually reaches equilibrium due to ion saturation.Moreover,when the discharge voltage is fixed at 2.1 kV,a maximum efficiency can be achieved at the flow rate of 9.0 m/s.This study provides a foundation for the design and application of AMDI for on-line detection with mass spectrometry and ion mobility spectrometry.
ObjectType-Article-1
SourceType-Scholarly Journals-1
ObjectType-Feature-2
content type line 23
OpenAccessLink https://infoscience.epfl.ch/handle/20.500.14299/123969
PQID 1825455904
PQPubID 23500
PageCount 5
ParticipantIDs proquest_miscellaneous_1825455904
crossref_citationtrail_10_1088_1009_0630_17_12_12
crossref_primary_10_1088_1009_0630_17_12_12
chongqing_primary_666909956
ProviderPackageCode CITATION
AAYXX
PublicationCentury 2000
PublicationDate 2015-12-01
PublicationDateYYYYMMDD 2015-12-01
PublicationDate_xml – month: 12
  year: 2015
  text: 2015-12-01
  day: 01
PublicationDecade 2010
PublicationTitle Plasma science & technology
PublicationTitleAlternate Plasma Science ＆ Technology
PublicationYear 2015
References 11
Jin D (7) 2009; 11
13
14
15
17
18
Ran Chen (16) 2013; 15
1
2
3
4
Zhu W C (12) 2009; 42
5
6
8
9
Lu X (10) 2012; 21
References_xml – ident: 11
  doi: 10.1021/ac8022108
– volume: 11
  start-page: 48
  year: 2009
  ident: 7
  publication-title: Plasma Sci. & Technol.
  doi: 10.1088/1009-0630/11/1/10
– ident: 5
  doi: 10.5059/yukigoseikyokaishi.69.171
– ident: 8
  doi: 10.1007/s00216-013-7316-0
– volume: 21
  issn: 0963-0252
  year: 2012
  ident: 10
  publication-title: Plasma Sources Sci. Tech.
– ident: 14
  doi: 10.1021/ac901122b
– volume: 15
  start-page: 845
  year: 2013
  ident: 16
  publication-title: Plasma Sci. Technol.
  doi: 10.1088/1009-0630/15/9/02
– ident: 4
  doi: 10.1002/jms.1243
– ident: 17
  doi: 10.5194/acp-9-4177-2009
– ident: 13
  doi: 10.1021/ac802117u
– ident: 3
  doi: 10.1016/j.jasms.2007.07.027
– ident: 1
  doi: 10.1021/ac050162j
– ident: 2
  doi: 10.1021/ac801641a
– volume: 42
  issn: 1361-6463
  year: 2009
  ident: 12
  publication-title: Journal of Physics
– ident: 15
  doi: 10.1002/rcm.6198
– ident: 18
  doi: 10.1016/j.aca.2014.06.014
– ident: 9
  doi: 10.1007/s00216-012-6536-z
– ident: 6
  doi: 10.1103/PhysRev.11.316
SSID ssj0054983
Score 2.009829
Snippet Ionization efficiency is an important factor for ion sources in mass spectrometry and ion mobility spectrometry.Using helium as the discharge gas,acetone as...
Ionization efficiency is an important factor for ion sources in mass spectrometry and ion mobility spectrometry. Using helium as the discharge gas, acetone as...
SourceID proquest
crossref
chongqing
SourceType Aggregation Database
Enrichment Source
Index Database
Publisher
StartPage 1048
SubjectTerms Desorption
Discharge
Ion mobility
Ionic mobility
Ionization
Mass spectrometry
Spectrometry
Spectroscopy
亚稳态
放电参数
环境
电离效率
离子迁移谱
稳定性
解吸
诱导
Title Effects of the Discharge Parameters on the Efficiency and Stability of Ambient Metastable-Induced Desorption Ionization
URI http://lib.cqvip.com/qk/84262X/201512/666909956.html
https://www.proquest.com/docview/1825455904
Volume 17
hasFullText 1
inHoldings 1
isFullTextHit
isPrint
link http://utb.summon.serialssolutions.com/2.0.0/link/0/eLvHCXMwnV3_a9UwEA_bRPQX8SvOqVQw-EOpa_olTX5s3_rYhKmMKfutJG06BvNVtzcE_3rv0vTLcAwVHiXcXe_a3uc1l-YuIeRtK0NlFIJXp1mQ8FAEyrQ8EFzHRqlMh3Y7n8OPfP9L8uEkPdnYfDfLWrpa6_f1rxvrSv7Hq0ADv2KV7D94dlQKBGiDf-EIHobjX_m4nJIxMH7cO7u0Cx8ZiAsx5woXznSTAbiD8pn9G_frLUGMabNi7fx6_k1jVaR_aNYKgkV9bgLc0QMzA2BY2l30b5WDbqjZnAe0tMxovkeFtA1Oi4KWKVJkSMuEFtCILSujkjkWiCFLUFHSklORY7oFNOSC5ktaLmmxoDKnJQgUtGCWBWIZ6gFDYsy-RX0gm_dnS2sKLCQ0lz4tJZKEQB4ocUJgPfVRChhS2MYSzfRCculbI-VAiq3OxF7R0p_ZA5K09wgK4PZLf7jtxAqVtMickJBYEHXW-Yv9_Gt-dHSQz7-0sHSWtdJ3DnYiibt5JPe_iGZvfxjailkkAaFrdGMvBW92-8HEqcO2XfggsoepZx7zJWGMKUOsQd4kd6Iss_kIB58-DyEHjPFFX0niNLrqMLCzO9J2WbbLIrv16j3oWVenPyA2uh6NXQ9GbIR1_JA8cEMjL-9x_ohsmNVjctemKNeXT8hPh3avaz1AtDei3ZvQ7nUry5vQ7gHavRHteK5Du_cn2r0J7d6E9qfkeFkeL_YDt21IUMcpWwdJ0urWiDZu64w3MqrruIlSEWdprVWcKlOHKuahjrlkTRQKLSPGGt7KOuIa-qRnZGvVrcxz4kWKs0YJ0yQNT1imdSuNEaZuaoiKVcO2yc74JKvv_eow1eirbcKGZ1vVbsF93PflvLKJH0LgeuGyQt9ULKtYBL9t4o_nDApvk34zuKyCXgGn-tTKdFeXFcMPP2kqw-TFrde4Q-5PSH9JttYXV-YVRNlr_doi7DfWhaqZ
linkProvider IOP Publishing
openUrl ctx_ver=Z39.88-2004&ctx_enc=info%3Aofi%2Fenc%3AUTF-8&rfr_id=info%3Asid%2Fsummon.serialssolutions.com&rft_val_fmt=info%3Aofi%2Ffmt%3Akev%3Amtx%3Ajournal&rft.genre=article&rft.atitle=Effects+of+the+Discharge+Parameters+on+the+Efficiency+and+Stability+of+Ambient+Metastable-Induced+Desorption+Ionization&rft.jtitle=%E7%AD%89%E7%A6%BB%E5%AD%90%E4%BD%93%E7%A7%91%E5%AD%A6%E4%B8%8E%E6%8A%80%E6%9C%AF%EF%BC%9A%E8%8B%B1%E6%96%87%E7%89%88&rft.au=%E5%BC%A0%E6%99%93%E5%A4%A9+%E9%99%88%E6%B1%A0%E6%9D%A5+%E5%88%98%E5%8F%8B%E6%B1%9F+%E7%8E%8B%E6%B3%93%E4%BC%9F+%E5%BC%A0%E4%B9%90%E5%8D%8E+%E5%AD%94%E5%BE%B7%E4%B9%89+Mario+CHAVARRIA&rft.date=2015-12-01&rft.issn=1009-0630&rft.issue=12&rft.spage=1048&rft.epage=1052&rft_id=info:doi/10.1088%2F1009-0630%2F17%2F12%2F12&rft.externalDocID=666909956
thumbnail_s http://utb.summon.serialssolutions.com/2.0.0/image/custom?url=http%3A%2F%2Fimage.cqvip.com%2Fvip1000%2Fqk%2F84262X%2F84262X.jpg