Local Diverse Polarization Optimized Comprehensive Energy‐Storage Performance in Lead‐Free Superparaelectrics
Lead‐free dielectric ceramics with ultrahigh energy‐storage performance are the core components used in next‐generation advanced pulse power capacitors. However, the low energy storage density largely hinders their development towards miniaturization, lightweight, and integration. Here, an effective...
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| Published in | Advanced materials (Weinheim) Vol. 34; no. 44; pp. e2205787 - n/a |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
Wiley Subscription Services, Inc
01.11.2022
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Lead‐free dielectric ceramics with ultrahigh energy‐storage performance are the core components used in next‐generation advanced pulse power capacitors. However, the low energy storage density largely hinders their development towards miniaturization, lightweight, and integration. Here, an effective strategy of constructing local diverse polarization is designed in superparaelectrics to realize an ultrahigh energy storage density of ≈10.59 J cm−3 as well as a large efficiency of ≈87.6%. The excellent comprehensive energy‐storage performance is mainly attributed to the design of ultrasmall polar nanoregions with local diverse polarization configuration, confirmed by scanning transmission electron microscopy, leading to the reduced heat loss, substantially enhanced polarization, and breakdown electric field compared to ceramics with single polarization configuration. Benefiting from these features, outstanding temperature/frequency/cycling stability and superior charge/discharge performance (power density ≈187.5 MW cm−3, discharge energy density ≈3.52 J cm−3, discharge rate ≈77 ns) are also achieved. This work demonstrates that local diverse polarization is a super strategy to design new dielectric materials with high energy‐storage performance.
Excellent energy‐storage properties with an ultrahigh recoverable energy storage density ≈10.59 J cm−3 and a large efficiency ≈87.6% are realized in lead‐free relaxor ferroelectrics, which is responsible by the local diverse polarization design, leading to the ultrasmall polar nanoregions, reduced heat loss, substantially enhanced polarization, and breakdown electric field compared to single polarization configuration. |
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| AbstractList | Lead‐free dielectric ceramics with ultrahigh energy‐storage performance are the core components used in next‐generation advanced pulse power capacitors. However, the low energy storage density largely hinders their development towards miniaturization, lightweight, and integration. Here, an effective strategy of constructing local diverse polarization is designed in superparaelectrics to realize an ultrahigh energy storage density of ≈10.59 J cm−3 as well as a large efficiency of ≈87.6%. The excellent comprehensive energy‐storage performance is mainly attributed to the design of ultrasmall polar nanoregions with local diverse polarization configuration, confirmed by scanning transmission electron microscopy, leading to the reduced heat loss, substantially enhanced polarization, and breakdown electric field compared to ceramics with single polarization configuration. Benefiting from these features, outstanding temperature/frequency/cycling stability and superior charge/discharge performance (power density ≈187.5 MW cm−3, discharge energy density ≈3.52 J cm−3, discharge rate ≈77 ns) are also achieved. This work demonstrates that local diverse polarization is a super strategy to design new dielectric materials with high energy‐storage performance. Lead-free dielectric ceramics with ultrahigh energy-storage performance are the core components used in next-generation advanced pulse power capacitors. However, the low energy storage density largely hinders their development towards miniaturization, lightweight, and integration. Here, an effective strategy of constructing local diverse polarization is designed in superparaelectrics to realize an ultrahigh energy storage density of ≈10.59 J cm-3 as well as a large efficiency of ≈87.6%. The excellent comprehensive energy-storage performance is mainly attributed to the design of ultrasmall polar nanoregions with local diverse polarization configuration, confirmed by scanning transmission electron microscopy, leading to the reduced heat loss, substantially enhanced polarization, and breakdown electric field compared to ceramics with single polarization configuration. Benefiting from these features, outstanding temperature/frequency/cycling stability and superior charge/discharge performance (power density ≈187.5 MW cm-3 , discharge energy density ≈3.52 J cm-3 , discharge rate ≈77 ns) are also achieved. This work demonstrates that local diverse polarization is a super strategy to design new dielectric materials with high energy-storage performance.Lead-free dielectric ceramics with ultrahigh energy-storage performance are the core components used in next-generation advanced pulse power capacitors. However, the low energy storage density largely hinders their development towards miniaturization, lightweight, and integration. Here, an effective strategy of constructing local diverse polarization is designed in superparaelectrics to realize an ultrahigh energy storage density of ≈10.59 J cm-3 as well as a large efficiency of ≈87.6%. The excellent comprehensive energy-storage performance is mainly attributed to the design of ultrasmall polar nanoregions with local diverse polarization configuration, confirmed by scanning transmission electron microscopy, leading to the reduced heat loss, substantially enhanced polarization, and breakdown electric field compared to ceramics with single polarization configuration. Benefiting from these features, outstanding temperature/frequency/cycling stability and superior charge/discharge performance (power density ≈187.5 MW cm-3 , discharge energy density ≈3.52 J cm-3 , discharge rate ≈77 ns) are also achieved. This work demonstrates that local diverse polarization is a super strategy to design new dielectric materials with high energy-storage performance. Lead‐free dielectric ceramics with ultrahigh energy‐storage performance are the core components used in next‐generation advanced pulse power capacitors. However, the low energy storage density largely hinders their development towards miniaturization, lightweight, and integration. Here, an effective strategy of constructing local diverse polarization is designed in superparaelectrics to realize an ultrahigh energy storage density of ≈10.59 J cm −3 as well as a large efficiency of ≈87.6%. The excellent comprehensive energy‐storage performance is mainly attributed to the design of ultrasmall polar nanoregions with local diverse polarization configuration, confirmed by scanning transmission electron microscopy, leading to the reduced heat loss, substantially enhanced polarization, and breakdown electric field compared to ceramics with single polarization configuration. Benefiting from these features, outstanding temperature/frequency/cycling stability and superior charge/discharge performance (power density ≈187.5 MW cm −3 , discharge energy density ≈3.52 J cm −3 , discharge rate ≈77 ns) are also achieved. This work demonstrates that local diverse polarization is a super strategy to design new dielectric materials with high energy‐storage performance. Lead‐free dielectric ceramics with ultrahigh energy‐storage performance are the core components used in next‐generation advanced pulse power capacitors. However, the low energy storage density largely hinders their development towards miniaturization, lightweight, and integration. Here, an effective strategy of constructing local diverse polarization is designed in superparaelectrics to realize an ultrahigh energy storage density of ≈10.59 J cm−3 as well as a large efficiency of ≈87.6%. The excellent comprehensive energy‐storage performance is mainly attributed to the design of ultrasmall polar nanoregions with local diverse polarization configuration, confirmed by scanning transmission electron microscopy, leading to the reduced heat loss, substantially enhanced polarization, and breakdown electric field compared to ceramics with single polarization configuration. Benefiting from these features, outstanding temperature/frequency/cycling stability and superior charge/discharge performance (power density ≈187.5 MW cm−3, discharge energy density ≈3.52 J cm−3, discharge rate ≈77 ns) are also achieved. This work demonstrates that local diverse polarization is a super strategy to design new dielectric materials with high energy‐storage performance. Excellent energy‐storage properties with an ultrahigh recoverable energy storage density ≈10.59 J cm−3 and a large efficiency ≈87.6% are realized in lead‐free relaxor ferroelectrics, which is responsible by the local diverse polarization design, leading to the ultrasmall polar nanoregions, reduced heat loss, substantially enhanced polarization, and breakdown electric field compared to single polarization configuration. |
| Author | Deng, Shiqing Chen, Liang Wu, Jie Chen, Jun Yu, Huifen Liu, Hui Zhang, Zhifei Wang, Na Qi, He |
| Author_xml | – sequence: 1 givenname: Liang orcidid: 0000-0002-4951-2205 surname: Chen fullname: Chen, Liang organization: University of Science and Technology Beijing – sequence: 2 givenname: Na surname: Wang fullname: Wang, Na organization: University of Science and Technology Beijing – sequence: 3 givenname: Zhifei surname: Zhang fullname: Zhang, Zhifei organization: University of Science and Technology Beijing – sequence: 4 givenname: Huifen surname: Yu fullname: Yu, Huifen organization: University of Science and Technology Beijing – sequence: 5 givenname: Jie surname: Wu fullname: Wu, Jie organization: University of Science and Technology Beijing – sequence: 6 givenname: Shiqing surname: Deng fullname: Deng, Shiqing organization: University of Science and Technology Beijing – sequence: 7 givenname: Hui surname: Liu fullname: Liu, Hui organization: University of Science and Technology Beijing – sequence: 8 givenname: He orcidid: 0000-0002-3094-3574 surname: Qi fullname: Qi, He email: qiheustb@ustb.edu.cn organization: University of Science and Technology Beijing – sequence: 9 givenname: Jun surname: Chen fullname: Chen, Jun email: junchen@ustb.edu.cn organization: University of Science and Technology Beijing |
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| Snippet | Lead‐free dielectric ceramics with ultrahigh energy‐storage performance are the core components used in next‐generation advanced pulse power capacitors.... Lead-free dielectric ceramics with ultrahigh energy-storage performance are the core components used in next-generation advanced pulse power capacitors.... |
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| SubjectTerms | Ceramics Charge density Configurations Dielectrics Discharge Electric fields Energy storage Flux density Frequency stability Heat loss lead‐free dielectric ceramics local diverse polarization Materials science Miniaturization Polarization relaxor ferroelectrics Scanning transmission electron microscopy superparaelectrics |
| Title | Local Diverse Polarization Optimized Comprehensive Energy‐Storage Performance in Lead‐Free Superparaelectrics |
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