Cobalt Single‐Atom Reverse Hydrogen Spillover for Efficient Electrochemical Water Dissociation and Dechlorination

• Published in: Angewandte Chemie International Edition Vol. 63; no. 19; pp. e202401386 - n/a
• Main Authors: Zheng, Qian, Xu, Hengyue, Yao, Yancai, Dai, Jie, Wang, Jiaxian, Hou, Wei, Zhao, Long, Zou, Xingyue, Zhan, Guangming, Wang, Ruizhao, Wang, Kaiyuan, Zhang, Lizhi
• Format: Journal Article
• Language: English
• Published: Weinheim Wiley Subscription Services, Inc 06.05.2024
• Edition: International ed. in English
• Subjects: Catalysis; Chloramphenicol; Chloromycetin; Cobalt; Dechlorination; Direct reduction; Electrocatalysts; Electrocatalytic Hydrodechlorination; Electrochemistry; Electrodes; Hydrogen; Hydrogen Spillover; Recombination; Single-atom Monolithic Electrode; Titanium; Titanium oxides; Water Dissociation

Efficient water dissociation to atomic hydrogen (H*) with restrained recombination of H* is crucial for improving the H* utilization for electrochemical dechlorination, but is currently limited by the lack of feasible electrodes. Herein, we developed a monolithic single‐atom electrode with Co single...