Greatly Enhanced Accessibility and Reproducibility of Worm‐like Micelles by In Situ Crosslinking Polymerization‐Induced Self‐Assembly
Worm‐like micelles have attracted great interest due to their anisotropic structures. However, the experimental conditions for obtaining worm‐like micelles are very restricted, which usually causes seriously poor reproducibility. In this work, significantly enhanced accessibility of worm‐like micell...
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| Published in | Angewandte Chemie International Edition Vol. 61; no. 43; pp. e202211792 - n/a |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
Wiley Subscription Services, Inc
24.10.2022
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| Edition | International ed. in English |
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| Abstract | Worm‐like micelles have attracted great interest due to their anisotropic structures. However, the experimental conditions for obtaining worm‐like micelles are very restricted, which usually causes seriously poor reproducibility. In this work, significantly enhanced accessibility of worm‐like micelles is realized by in situ crosslinking polymerization‐induced self‐assembly (PISA). The reproducibility of worm‐like micelles is greatly improved due to the significantly enlarged experimental windows of worm‐like micelles in the morphology diagram. Moreover, the reliability of the methodology to enhance the accessibility of worm‐like micelles has been demonstrated in various in situ crosslinking PISA systems. The greatly enhanced accessibility and reproducibility of worm‐like micelles is undoubtedly cost‐effective especially in scale‐up production, which paves the way for further application of worm‐like micelles with various compositions and functionalities.
Greatly enhanced accessibility of worm‐like micelles (W) is realized by in situ crosslinking polymerization‐induced self‐assembly (PISA), leading to significantly improved reproducibility of worm‐like micelles. The reliability of the methodology has been demonstrated in various in situ crosslinking PISA systems with different formulations of monomers, macro RAFT agents, crosslinkers, solvents, and polymerization temperatures. |
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| AbstractList | Worm‐like micelles have attracted great interest due to their anisotropic structures. However, the experimental conditions for obtaining worm‐like micelles are very restricted, which usually causes seriously poor reproducibility. In this work, significantly enhanced accessibility of worm‐like micelles is realized by in situ crosslinking polymerization‐induced self‐assembly (PISA). The reproducibility of worm‐like micelles is greatly improved due to the significantly enlarged experimental windows of worm‐like micelles in the morphology diagram. Moreover, the reliability of the methodology to enhance the accessibility of worm‐like micelles has been demonstrated in various in situ crosslinking PISA systems. The greatly enhanced accessibility and reproducibility of worm‐like micelles is undoubtedly cost‐effective especially in scale‐up production, which paves the way for further application of worm‐like micelles with various compositions and functionalities. Worm-like micelles have attracted great interest due to their anisotropic structures. However, the experimental conditions for obtaining worm-like micelles are very restricted, which usually causes seriously poor reproducibility. In this work, significantly enhanced accessibility of worm-like micelles is realized by in situ crosslinking polymerization-induced self-assembly (PISA). The reproducibility of worm-like micelles is greatly improved due to the significantly enlarged experimental windows of worm-like micelles in the morphology diagram. Moreover, the reliability of the methodology to enhance the accessibility of worm-like micelles has been demonstrated in various in situ crosslinking PISA systems. The greatly enhanced accessibility and reproducibility of worm-like micelles is undoubtedly cost-effective especially in scale-up production, which paves the way for further application of worm-like micelles with various compositions and functionalities.Worm-like micelles have attracted great interest due to their anisotropic structures. However, the experimental conditions for obtaining worm-like micelles are very restricted, which usually causes seriously poor reproducibility. In this work, significantly enhanced accessibility of worm-like micelles is realized by in situ crosslinking polymerization-induced self-assembly (PISA). The reproducibility of worm-like micelles is greatly improved due to the significantly enlarged experimental windows of worm-like micelles in the morphology diagram. Moreover, the reliability of the methodology to enhance the accessibility of worm-like micelles has been demonstrated in various in situ crosslinking PISA systems. The greatly enhanced accessibility and reproducibility of worm-like micelles is undoubtedly cost-effective especially in scale-up production, which paves the way for further application of worm-like micelles with various compositions and functionalities. Worm‐like micelles have attracted great interest due to their anisotropic structures. However, the experimental conditions for obtaining worm‐like micelles are very restricted, which usually causes seriously poor reproducibility. In this work, significantly enhanced accessibility of worm‐like micelles is realized by in situ crosslinking polymerization‐induced self‐assembly (PISA). The reproducibility of worm‐like micelles is greatly improved due to the significantly enlarged experimental windows of worm‐like micelles in the morphology diagram. Moreover, the reliability of the methodology to enhance the accessibility of worm‐like micelles has been demonstrated in various in situ crosslinking PISA systems. The greatly enhanced accessibility and reproducibility of worm‐like micelles is undoubtedly cost‐effective especially in scale‐up production, which paves the way for further application of worm‐like micelles with various compositions and functionalities. Greatly enhanced accessibility of worm‐like micelles (W) is realized by in situ crosslinking polymerization‐induced self‐assembly (PISA), leading to significantly improved reproducibility of worm‐like micelles. The reliability of the methodology has been demonstrated in various in situ crosslinking PISA systems with different formulations of monomers, macro RAFT agents, crosslinkers, solvents, and polymerization temperatures. |
| Author | Zhang, Wen‐Jian Chang, Zi‐Xuan Bai, Wei Hong, Chun‐Yan |
| Author_xml | – sequence: 1 givenname: Wen‐Jian orcidid: 0000-0001-9039-3618 surname: Zhang fullname: Zhang, Wen‐Jian organization: Anhui University – sequence: 2 givenname: Zi‐Xuan surname: Chang fullname: Chang, Zi‐Xuan organization: University of Science and Technology of China – sequence: 3 givenname: Wei surname: Bai fullname: Bai, Wei email: Baiwei@ahu.edu.cn organization: Anhui University – sequence: 4 givenname: Chun‐Yan orcidid: 0000-0002-5295-4741 surname: Hong fullname: Hong, Chun‐Yan email: hongcy@ustc.edu.cn organization: University of Science and Technology of China |
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| Snippet | Worm‐like micelles have attracted great interest due to their anisotropic structures. However, the experimental conditions for obtaining worm‐like micelles are... Worm-like micelles have attracted great interest due to their anisotropic structures. However, the experimental conditions for obtaining worm-like micelles are... |
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| SubjectTerms | Accessibility Assembly Crosslinking In Situ Crosslinking Micelles Polymerization Polymerization-Induced Self-Assembly Reproducibility Worm-Like Micelles |
| Title | Greatly Enhanced Accessibility and Reproducibility of Worm‐like Micelles by In Situ Crosslinking Polymerization‐Induced Self‐Assembly |
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