Organic–Inorganic Hybridization Engineering of Polyperylenediimide Cathodes for Efficient Potassium Storage
Polyperylenediimide (PDI) is always subject to its modest conductivities, limited reversible active sites and inferior stability for potassium storage. To address these issues, herein, we firstly propose an organic–inorganic hybrid (PDI@Fe‐Sn@N‐Ti3C2Tx), where Fe/Sn single atoms are bound to the N‐d...
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| Published in | Angewandte Chemie International Edition Vol. 60; no. 44; pp. 23596 - 23601 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
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Weinheim
Wiley Subscription Services, Inc
25.10.2021
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| Edition | International ed. in English |
| Subjects | |
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| Abstract | Polyperylenediimide (PDI) is always subject to its modest conductivities, limited reversible active sites and inferior stability for potassium storage. To address these issues, herein, we firstly propose an organic–inorganic hybrid (PDI@Fe‐Sn@N‐Ti3C2Tx), where Fe/Sn single atoms are bound to the N‐doped MXenes (N‐Ti3C2Tx) via the unsaturated Fe/Sn–N3 bonds, and functionalized with PDI via d–π hybridization, forming a high conjugated δ skeleton. The resulted hybrid cathode endowed with enhanced electronic/ionic conductivities, lowered dissociation barriers of multiple redox centers and a stable cathode electrolyte interphase layer displays a 14‐electron involved high‐rate capacities and long cycle life. Moreover, it shows competitive performance in full cells even under different folding states and low operating temperatures.
Hierarchical organic–inorganic hybrid PDI@Fe‐Sn@N‐Ti3C2Tx is smartly designed and exhibits superb potassium‐storage properties, thanks to its unique properties including abundant contactable active sites, Fe/Sn–N3 bonds, electronic polarization, and strong coordination interactions, as shown by detailed experiments and theoretical calculations/simulations. |
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| AbstractList | Polyperylenediimide (PDI) is always subject to its modest conductivities, limited reversible active sites and inferior stability for potassium storage. To address these issues, herein, we firstly propose an organic–inorganic hybrid (PDI@Fe‐Sn@N‐Ti3C2Tx), where Fe/Sn single atoms are bound to the N‐doped MXenes (N‐Ti3C2Tx) via the unsaturated Fe/Sn–N3 bonds, and functionalized with PDI via d–π hybridization, forming a high conjugated δ skeleton. The resulted hybrid cathode endowed with enhanced electronic/ionic conductivities, lowered dissociation barriers of multiple redox centers and a stable cathode electrolyte interphase layer displays a 14‐electron involved high‐rate capacities and long cycle life. Moreover, it shows competitive performance in full cells even under different folding states and low operating temperatures. Polyperylenediimide (PDI) is always subject to its modest conductivities, limited reversible active sites and inferior stability for potassium storage. To address these issues, herein, we firstly propose an organic–inorganic hybrid (PDI@Fe‐Sn@N‐Ti3C2Tx), where Fe/Sn single atoms are bound to the N‐doped MXenes (N‐Ti3C2Tx) via the unsaturated Fe/Sn–N3 bonds, and functionalized with PDI via d–π hybridization, forming a high conjugated δ skeleton. The resulted hybrid cathode endowed with enhanced electronic/ionic conductivities, lowered dissociation barriers of multiple redox centers and a stable cathode electrolyte interphase layer displays a 14‐electron involved high‐rate capacities and long cycle life. Moreover, it shows competitive performance in full cells even under different folding states and low operating temperatures. Hierarchical organic–inorganic hybrid PDI@Fe‐Sn@N‐Ti3C2Tx is smartly designed and exhibits superb potassium‐storage properties, thanks to its unique properties including abundant contactable active sites, Fe/Sn–N3 bonds, electronic polarization, and strong coordination interactions, as shown by detailed experiments and theoretical calculations/simulations. Polyperylenediimide (PDI) is always subject to its modest conductivities, limited reversible active sites and inferior stability for potassium storage. To address these issues, herein, we firstly propose an organic–inorganic hybrid (PDI@Fe‐Sn@N‐Ti 3 C 2 T x ), where Fe/Sn single atoms are bound to the N‐doped MXenes (N‐Ti 3 C 2 T x ) via the unsaturated Fe/Sn–N 3 bonds, and functionalized with PDI via d–π hybridization, forming a high conjugated δ skeleton. The resulted hybrid cathode endowed with enhanced electronic/ionic conductivities, lowered dissociation barriers of multiple redox centers and a stable cathode electrolyte interphase layer displays a 14‐electron involved high‐rate capacities and long cycle life. Moreover, it shows competitive performance in full cells even under different folding states and low operating temperatures. Polyperylenediimide (PDI) is always subject to its modest conductivities, limited reversible active sites and inferior stability for potassium storage. To address these issues, herein, we firstly propose an organic-inorganic hybrid (PDI@Fe-Sn@N-Ti3 C2 Tx ), where Fe/Sn single atoms are bound to the N-doped MXenes (N-Ti3 C2 Tx ) via the unsaturated Fe/Sn-N3 bonds, and functionalized with PDI via d-π hybridization, forming a high conjugated δ skeleton. The resulted hybrid cathode endowed with enhanced electronic/ionic conductivities, lowered dissociation barriers of multiple redox centers and a stable cathode electrolyte interphase layer displays a 14-electron involved high-rate capacities and long cycle life. Moreover, it shows competitive performance in full cells even under different folding states and low operating temperatures.Polyperylenediimide (PDI) is always subject to its modest conductivities, limited reversible active sites and inferior stability for potassium storage. To address these issues, herein, we firstly propose an organic-inorganic hybrid (PDI@Fe-Sn@N-Ti3 C2 Tx ), where Fe/Sn single atoms are bound to the N-doped MXenes (N-Ti3 C2 Tx ) via the unsaturated Fe/Sn-N3 bonds, and functionalized with PDI via d-π hybridization, forming a high conjugated δ skeleton. The resulted hybrid cathode endowed with enhanced electronic/ionic conductivities, lowered dissociation barriers of multiple redox centers and a stable cathode electrolyte interphase layer displays a 14-electron involved high-rate capacities and long cycle life. Moreover, it shows competitive performance in full cells even under different folding states and low operating temperatures. |
| Author | Hou, Linrui Wang, Yuyan Han, Pinyu Zhang, Yamin Yuan, Changzhou Liu, Fusheng Qin, Guohui |
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| SubjectTerms | Cathodes Electrolytic cells Fe/Sn single atoms Hybridization Low temperature N-doped MXenes Operating temperature organic–inorganic hybrid polyperylenediimide cathode Potassium potassium-ion batteries Shelf life |
| Title | Organic–Inorganic Hybridization Engineering of Polyperylenediimide Cathodes for Efficient Potassium Storage |
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