Palladium nanoneedle “highways” for fast hydrogen transport in magnesium nanoparticle assembled films

The importance of hydrogen storage for mobile applications remains a timely subject with respect to a sustainable energy economy. Magnesium is a viable material for hydrogen storage by insertion, because of its low weight, abundance, and non-toxicity. A major obstacle for magnesium hydrides to be us...

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Published in	Journal of materials science Vol. 60; no. 12; pp. 5415 - 5426
Main Authors	Schieck, Katrina E., Pedicone, Luca, Crespi, Stefania, Di Vece, Marcel
Format	Journal Article
Language	English
Published	New York Springer US 01.03.2025 Springer Nature B.V
Subjects	Applications programs Atoms & subatomic particles Characterization and Evaluation of Materials Chemistry and Materials Science Classical Mechanics Composites & Nanocomposites Crystallography and Scattering Methods desorption Electric properties Glass substrates High temperature Hydrogen Hydrogen storage Hydrogenation Magnesium Materials Science Mobile computing Nanoparticles Nanostructured materials Oxidation Palladium Polymer Sciences renewable energy sources Roads & highways Solid Mechanics Storage systems temperature
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Abstract	The importance of hydrogen storage for mobile applications remains a timely subject with respect to a sustainable energy economy. Magnesium is a viable material for hydrogen storage by insertion, because of its low weight, abundance, and non-toxicity. A major obstacle for magnesium hydrides to be used for hydrogen storage is the high temperature for release, making it impracticable. However, nanoscale magnesium shows promising hydrogen desorption temperatures, which is employed in the form of nanoparticles in this work. A palladium “nanoneedle” network was used to speed up hydrogen transport to and from the magnesium nanoparticles in a matter of minutes. By using the optical changes that accompany the presence of hydrogen in magnesium, hydrogen transport was studied. The palladium nanoneedle “highways” improved the (de-) hydrogenation of magnesium nanoparticles by at least a factor two, which could be a template for further improvements in hydrogen storage systems.
AbstractList	The importance of hydrogen storage for mobile applications remains a timely subject with respect to a sustainable energy economy. Magnesium is a viable material for hydrogen storage by insertion, because of its low weight, abundance, and non-toxicity. A major obstacle for magnesium hydrides to be used for hydrogen storage is the high temperature for release, making it impracticable. However, nanoscale magnesium shows promising hydrogen desorption temperatures, which is employed in the form of nanoparticles in this work. A palladium “nanoneedle” network was used to speed up hydrogen transport to and from the magnesium nanoparticles in a matter of minutes. By using the optical changes that accompany the presence of hydrogen in magnesium, hydrogen transport was studied. The palladium nanoneedle “highways” improved the (de-) hydrogenation of magnesium nanoparticles by at least a factor two, which could be a template for further improvements in hydrogen storage systems.
Author	Pedicone, Luca Crespi, Stefania Schieck, Katrina E. Di Vece, Marcel
Author_xml	– sequence: 1 givenname: Katrina E. surname: Schieck fullname: Schieck, Katrina E. organization: Interdisciplinary Centre for Nanostructured Materials and Interfaces (CIMaINa) and Physics Department “Aldo Pontremoli”, Università degli Studi di Milano – sequence: 2 givenname: Luca surname: Pedicone fullname: Pedicone, Luca organization: Interdisciplinary Centre for Nanostructured Materials and Interfaces (CIMaINa) and Physics Department “Aldo Pontremoli”, Università degli Studi di Milano – sequence: 3 givenname: Stefania surname: Crespi fullname: Crespi, Stefania organization: Dipartimento Di Scienze Della Terra “Ardito Desio”, Università degli Studi di Milano – sequence: 4 givenname: Marcel orcidid: 0000-0002-0041-4348 surname: Di Vece fullname: Di Vece, Marcel email: marcel.divece@unimi.it organization: Interdisciplinary Centre for Nanostructured Materials and Interfaces (CIMaINa) and Physics Department “Aldo Pontremoli”, Università degli Studi di Milano
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Snippet	The importance of hydrogen storage for mobile applications remains a timely subject with respect to a sustainable energy economy. Magnesium is a viable...
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SubjectTerms	Applications programs Atoms & subatomic particles Characterization and Evaluation of Materials Chemistry and Materials Science Classical Mechanics Composites & Nanocomposites Crystallography and Scattering Methods desorption Electric properties Glass substrates High temperature Hydrogen Hydrogen storage Hydrogenation Magnesium Materials Science Mobile computing Nanoparticles Nanostructured materials Oxidation Palladium Polymer Sciences renewable energy sources Roads & highways Solid Mechanics Storage systems temperature
Title	Palladium nanoneedle “highways” for fast hydrogen transport in magnesium nanoparticle assembled films
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