Infrared laser ablation of glassy As2Se3
In this study, we report the first measurements of wavelength and pulse length dependence of ablation thresholds in glassy As2Se3. Ablation yields, obtained from time-of-flight spectra were compared to laser intensity curves to obtain laser ablation thresholds. The wavelength dependence of the ablat...
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Published in | Journal of non-crystalline solids Vol. 352; no. 23-25; pp. 2430 - 2433 |
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Main Authors | , , , , |
Format | Journal Article Conference Proceeding |
Language | English |
Published |
Amsterdam
Elsevier B.V
15.07.2006
Elsevier |
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Abstract | In this study, we report the first measurements of wavelength and pulse length dependence of ablation thresholds in glassy As2Se3. Ablation yields, obtained from time-of-flight spectra were compared to laser intensity curves to obtain laser ablation thresholds. The wavelength dependence of the ablation thresholds were obtained by tuning the Vanderbilt–Keck free electron laser in the range of 3.2–5μm. Pulse dependence of the ablation thresholds were obtained with a 5μs macropulse in the wavelength range 3.2–5μm and with macropulses ranging from 200 to 1000ns at the wavelength of 3.5μm. The wavelength dependence of the ablation threshold did not indicate that impurity absorption was a major factor in the ablation process in glassy As2Se3. The ablation threshold decreased with wavelengths corresponding to higher photon energies. In addition, a sharp increase in ablation threshold was observed with decrease in the macropulse length. Optical images of ablation craters at intensities above the threshold reveal significant melting on the sample surface. We will discuss the wavelength and pulse length dependence of the laser ablation threshold in glassy As2Se3 in terms of a multi-photon process and a cumulative heating process. |
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AbstractList | In this study, we report the first measurements of wavelength and pulse length dependence of ablation thresholds in glassy As2Se3. Ablation yields, obtained from time-of-flight spectra were compared to laser intensity curves to obtain laser ablation thresholds. The wavelength dependence of the ablation thresholds were obtained by tuning the Vanderbilt–Keck free electron laser in the range of 3.2–5μm. Pulse dependence of the ablation thresholds were obtained with a 5μs macropulse in the wavelength range 3.2–5μm and with macropulses ranging from 200 to 1000ns at the wavelength of 3.5μm. The wavelength dependence of the ablation threshold did not indicate that impurity absorption was a major factor in the ablation process in glassy As2Se3. The ablation threshold decreased with wavelengths corresponding to higher photon energies. In addition, a sharp increase in ablation threshold was observed with decrease in the macropulse length. Optical images of ablation craters at intensities above the threshold reveal significant melting on the sample surface. We will discuss the wavelength and pulse length dependence of the laser ablation threshold in glassy As2Se3 in terms of a multi-photon process and a cumulative heating process. |
Author | Sanghera, J. Aggarwal, I. Tolk, N. Adair, J. Hari, P. |
Author_xml | – sequence: 1 givenname: P. surname: Hari fullname: Hari, P. email: hari@utulsa.edu organization: Department of Physics and Engineering Physics, University of Tulsa, Tulsa, OK 74104, USA – sequence: 2 givenname: J. surname: Adair fullname: Adair, J. organization: Department of Physics and Astronomy, Vanderbilt University, Nashville, TN 37235, USA – sequence: 3 givenname: N. surname: Tolk fullname: Tolk, N. organization: Department of Physics and Astronomy, Vanderbilt University, Nashville, TN 37235, USA – sequence: 4 givenname: J. surname: Sanghera fullname: Sanghera, J. organization: Naval Research Laboratory, Washington, DC 20375, USA – sequence: 5 givenname: I. surname: Aggarwal fullname: Aggarwal, I. organization: Naval Research Laboratory, Washington, DC 20375, USA |
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CitedBy_id | crossref_primary_10_1002_rcm_4607 crossref_primary_10_1016_j_materresbull_2014_12_027 crossref_primary_10_1021_acs_jpcc_7b10894 crossref_primary_10_1063_1_3587616 crossref_primary_10_7567_1347_4065_ab3368 crossref_primary_10_1016_j_optcom_2017_10_056 crossref_primary_10_1016_j_jallcom_2018_11_058 crossref_primary_10_1038_s41598_017_06592_3 |
Cites_doi | 10.1103/PhysRevB.61.11998 |
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Keywords | 78.66.Jg Chalcogenides 79.20.Ds Infra-red fibers Lasers 73.61.Jc Multi-photon processes Radiation matter interactions Heat treatments Chalcogenide glasses Fibers Laser pulse Laser radiation Time of flight spectra Infrared radiation Laser ablation technique |
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References | Wood (bib2) 1986 Mott, Davis (bib8) 1971 Becker, Johnson, Edwards (bib3) 1994; 65 Borisova (bib7) 1990 Nishii, Yamashita (bib1) 2000 Brau (bib4) 1990 Li, Drabold (bib6) 2000; 61 Kokorina (bib5) 1996 Nishii (10.1016/j.jnoncrysol.2006.03.044_bib1) 2000 Kokorina (10.1016/j.jnoncrysol.2006.03.044_bib5) 1996 Li (10.1016/j.jnoncrysol.2006.03.044_bib6) 2000; 61 Wood (10.1016/j.jnoncrysol.2006.03.044_bib2) 1986 Brau (10.1016/j.jnoncrysol.2006.03.044_bib4) 1990 Borisova (10.1016/j.jnoncrysol.2006.03.044_bib7) 1990 Becker (10.1016/j.jnoncrysol.2006.03.044_bib3) 1994; 65 Mott (10.1016/j.jnoncrysol.2006.03.044_bib8) 1971 |
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SubjectTerms | Chalcogenides Condensed matter: electronic structure, electrical, magnetic, and optical properties Electron and ion emission by liquids and solids; impact phenomena Exact sciences and technology Impact phenomena (including electron spectra and sputtering) Infra-red fibers Laser-beam impact phenomena Lasers Physics |
Title | Infrared laser ablation of glassy As2Se3 |
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