Hierarchical Cu(OH)2@MnO2 core-shell nanorods array in situ generated on three-dimensional copper foam for high-performance supercapacitors
[Display omitted] Manganese dioxide (MnO2) with high theoretical capacity (1380 F g−1), high natural abundance and low cost has been considered as one of the most competitive active materials for preparing the electrode of supercapacitors. However, the poor electrical conductivity limits its broad a...
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| Published in | Journal of colloid and interface science Vol. 563; pp. 394 - 404 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Inc
15.03.2020
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| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
Manganese dioxide (MnO2) with high theoretical capacity (1380 F g−1), high natural abundance and low cost has been considered as one of the most competitive active materials for preparing the electrode of supercapacitors. However, the poor electrical conductivity limits its broad applications. To solve this problem, we design a hierarchical Cu(OH)2@MnO2 core-shell nanorods array on copper foam (CF), in which the one-dimensional (1D) Cu(OH)2 nanorod core provides the scaffold for the growth of MnO2 nanosheets and a short ion and electronic diffusion pathway and the two-dimensional (2D) MnO2 nanosheets shell provides enormous active sites due to their large surface area. The obtained Cu(OH)2@MnO2/CF nanorods array displays an excellent areal capacitance of 708.62 mF cm−2 at the current density of 2 mA cm−2 (283.45 F g−1 at 0.8 A g−1). Additionally, the assembled Cu(OH)2@MnO2/CF//activated carbon (AC) asymmetric supercapacitor shows an outstanding energy density of 18.36 Wh kg−1 at a power density of 750 W kg−1. Two such capacitors connected in series can light up a red LED bulb for over fifteen minutes. |
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| AbstractList | [Display omitted]
Manganese dioxide (MnO2) with high theoretical capacity (1380 F g−1), high natural abundance and low cost has been considered as one of the most competitive active materials for preparing the electrode of supercapacitors. However, the poor electrical conductivity limits its broad applications. To solve this problem, we design a hierarchical Cu(OH)2@MnO2 core-shell nanorods array on copper foam (CF), in which the one-dimensional (1D) Cu(OH)2 nanorod core provides the scaffold for the growth of MnO2 nanosheets and a short ion and electronic diffusion pathway and the two-dimensional (2D) MnO2 nanosheets shell provides enormous active sites due to their large surface area. The obtained Cu(OH)2@MnO2/CF nanorods array displays an excellent areal capacitance of 708.62 mF cm−2 at the current density of 2 mA cm−2 (283.45 F g−1 at 0.8 A g−1). Additionally, the assembled Cu(OH)2@MnO2/CF//activated carbon (AC) asymmetric supercapacitor shows an outstanding energy density of 18.36 Wh kg−1 at a power density of 750 W kg−1. Two such capacitors connected in series can light up a red LED bulb for over fifteen minutes. Manganese dioxide (MnO₂) with high theoretical capacity (1380 F g⁻¹), high natural abundance and low cost has been considered as one of the most competitive active materials for preparing the electrode of supercapacitors. However, the poor electrical conductivity limits its broad applications. To solve this problem, we design a hierarchical Cu(OH)₂@MnO₂ core-shell nanorods array on copper foam (CF), in which the one-dimensional (1D) Cu(OH)₂ nanorod core provides the scaffold for the growth of MnO₂ nanosheets and a short ion and electronic diffusion pathway and the two-dimensional (2D) MnO₂ nanosheets shell provides enormous active sites due to their large surface area. The obtained Cu(OH)₂@MnO₂/CF nanorods array displays an excellent areal capacitance of 708.62 mF cm⁻² at the current density of 2 mA cm⁻² (283.45 F g⁻¹ at 0.8 A g⁻¹). Additionally, the assembled Cu(OH)₂@MnO₂/CF//activated carbon (AC) asymmetric supercapacitor shows an outstanding energy density of 18.36 Wh kg⁻¹ at a power density of 750 W kg⁻¹. Two such capacitors connected in series can light up a red LED bulb for over fifteen minutes. Manganese dioxide (MnO2) with high theoretical capacity (1380 F g-1), high natural abundance and low cost has been considered as one of the most competitive active materials for preparing the electrode of supercapacitors. However, the poor electrical conductivity limits its broad applications. To solve this problem, we design a hierarchical Cu(OH)2@MnO2 core-shell nanorods array on copper foam (CF), in which the one-dimensional (1D) Cu(OH)2 nanorod core provides the scaffold for the growth of MnO2 nanosheets and a short ion and electronic diffusion pathway and the two-dimensional (2D) MnO2 nanosheets shell provides enormous active sites due to their large surface area. The obtained Cu(OH)2@MnO2/CF nanorods array displays an excellent areal capacitance of 708.62 mF cm-2 at the current density of 2 mA cm-2 (283.45 F g-1 at 0.8 A g-1). Additionally, the assembled Cu(OH)2@MnO2/CF//activated carbon (AC) asymmetric supercapacitor shows an outstanding energy density of 18.36 Wh kg-1 at a power density of 750 W kg-1. Two such capacitors connected in series can light up a red LED bulb for over fifteen minutes.Manganese dioxide (MnO2) with high theoretical capacity (1380 F g-1), high natural abundance and low cost has been considered as one of the most competitive active materials for preparing the electrode of supercapacitors. However, the poor electrical conductivity limits its broad applications. To solve this problem, we design a hierarchical Cu(OH)2@MnO2 core-shell nanorods array on copper foam (CF), in which the one-dimensional (1D) Cu(OH)2 nanorod core provides the scaffold for the growth of MnO2 nanosheets and a short ion and electronic diffusion pathway and the two-dimensional (2D) MnO2 nanosheets shell provides enormous active sites due to their large surface area. The obtained Cu(OH)2@MnO2/CF nanorods array displays an excellent areal capacitance of 708.62 mF cm-2 at the current density of 2 mA cm-2 (283.45 F g-1 at 0.8 A g-1). Additionally, the assembled Cu(OH)2@MnO2/CF//activated carbon (AC) asymmetric supercapacitor shows an outstanding energy density of 18.36 Wh kg-1 at a power density of 750 W kg-1. Two such capacitors connected in series can light up a red LED bulb for over fifteen minutes. |
| Author | Zhong, Yuxue Liu, Ying Cao, Xueying Liu, Jingquan Wang, Huining Cui, Liang Yan, Guowen |
| Author_xml | – sequence: 1 givenname: Huining surname: Wang fullname: Wang, Huining organization: College of Material Science and Engineering, Institute for Graphene Applied Technology Innovation, Collaborative Innovation Centre for Marine Biomass Fibers, Materials and Textiles of Shandong Province, Qingdao University, Qingdao 266071, Shandong, China – sequence: 2 givenname: Guowen surname: Yan fullname: Yan, Guowen organization: College of Material Science and Engineering, Institute for Graphene Applied Technology Innovation, Collaborative Innovation Centre for Marine Biomass Fibers, Materials and Textiles of Shandong Province, Qingdao University, Qingdao 266071, Shandong, China – sequence: 3 givenname: Xueying surname: Cao fullname: Cao, Xueying organization: College of Material Science and Engineering, Institute for Graphene Applied Technology Innovation, Collaborative Innovation Centre for Marine Biomass Fibers, Materials and Textiles of Shandong Province, Qingdao University, Qingdao 266071, Shandong, China – sequence: 4 givenname: Ying surname: Liu fullname: Liu, Ying organization: College of Material Science and Engineering, Institute for Graphene Applied Technology Innovation, Collaborative Innovation Centre for Marine Biomass Fibers, Materials and Textiles of Shandong Province, Qingdao University, Qingdao 266071, Shandong, China – sequence: 5 givenname: Yuxue surname: Zhong fullname: Zhong, Yuxue organization: College of Material Science and Engineering, Institute for Graphene Applied Technology Innovation, Collaborative Innovation Centre for Marine Biomass Fibers, Materials and Textiles of Shandong Province, Qingdao University, Qingdao 266071, Shandong, China – sequence: 6 givenname: Liang surname: Cui fullname: Cui, Liang email: cuiliang@lyu.edu.cn organization: College of Material Science and Engineering, Linyi University, Linyi 276000, Shandong, China – sequence: 7 givenname: Jingquan surname: Liu fullname: Liu, Jingquan email: jliu@qdu.edu.cn organization: College of Material Science and Engineering, Institute for Graphene Applied Technology Innovation, Collaborative Innovation Centre for Marine Biomass Fibers, Materials and Textiles of Shandong Province, Qingdao University, Qingdao 266071, Shandong, China |
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Manganese dioxide (MnO2) with high theoretical capacity (1380 F g−1), high natural abundance and low cost has been considered as one of the... Manganese dioxide (MnO2) with high theoretical capacity (1380 F g-1), high natural abundance and low cost has been considered as one of the most competitive... Manganese dioxide (MnO₂) with high theoretical capacity (1380 F g⁻¹), high natural abundance and low cost has been considered as one of the most competitive... |
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| SubjectTerms | activated carbon active sites Asymmetric supercapcitors capacitance copper copper hydroxide copper nanoparticles Core–shell hierarchical structure Cu(OH)2 nanorods array electrical conductivity electrochemical capacitors electrodes energy density foams lamps manganese dioxide MnO2 nanorods nanosheets surface area |
| Title | Hierarchical Cu(OH)2@MnO2 core-shell nanorods array in situ generated on three-dimensional copper foam for high-performance supercapacitors |
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