Importance of long-range interactions in chemical reactions at cold and ultracold temperatures
We review the recent progress achieved in the theoretical description of chemical reactions at low temperatures. In particular, we discuss the crucial role played by the van der Waals interaction potential in quantum-mechanical scattering calculations of atom-diatom collisions in the cold and ultrac...
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| Published in | International reviews in physical chemistry Vol. 25; no. 3; pp. 283 - 311 |
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| Main Authors | , |
| Format | Journal Article |
| Language | English |
| Published |
Taylor & Francis Group
01.07.2006
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| Abstract | We review the recent progress achieved in the theoretical description of chemical reactions at low temperatures. In particular, we discuss the crucial role played by the van der Waals interaction potential in quantum-mechanical scattering calculations of atom-diatom collisions in the cold and ultracold regimes, where abstraction reactions proceed by tunnelling. The importance of zero-energy resonances in enhancing the reactivity in the zero-temperature limit is assessed. The impact of Feshbach resonances associated with the decay of metastable states of van der Waals complexes on reactive scattering is addressed through a series of examples. Finally, we discuss the sensitivity of the reaction dynamics to the topology of the van der Waals well. |
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| AbstractList | We review the recent progress achieved in the theoretical description of chemical reactions at low temperatures. In particular, we discuss the crucial role played by the van der Waals interaction potential in quantum-mechanical scattering calculations of atom-diatom collisions in the cold and ultracold regimes, where abstraction reactions proceed by tunnelling. The importance of zero-energy resonances in enhancing the reactivity in the zero-temperature limit is assessed. The impact of Feshbach resonances associated with the decay of metastable states of van der Waals complexes on reactive scattering is addressed through a series of examples. Finally, we discuss the sensitivity of the reaction dynamics to the topology of the van der Waals well. |
| Author | Weck, Philippe F. Balakrishnan, N. |
| Author_xml | – sequence: 1 givenname: Philippe F. surname: Weck fullname: Weck, Philippe F. email: weckp@unlv.nevada.edu organization: Department of Chemistry , University of Nevada Las Vegas – sequence: 2 givenname: N. surname: Balakrishnan fullname: Balakrishnan, N. organization: Department of Chemistry , University of Nevada Las Vegas |
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| Title | Importance of long-range interactions in chemical reactions at cold and ultracold temperatures |
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