Shape-remodeled macrocapsule of phase change materials for thermal energy storage and thermal management

•A shape-remodeled PCM macrocapsule was fabricated through a cast molding method.•The EBiInSn-based flexible shell can sustain a maximum stretching of 432%.•The prepared PCM macrocapsule can be remodeled as needed to a complicated shape.•An innovative PCM-based conformal thermal control method was d...

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Published inApplied energy Vol. 247; pp. 503 - 516
Main Authors Yu, De-Hai, He, Zhi-Zhu
Format Journal Article
LanguageEnglish
Published Elsevier Ltd 01.08.2019
Subjects
alloys
Bi-In-Sn eutectic alloy
deformation
electronic equipment
encapsulation
engineering
heat
latent heat
melting
microparticles
Octadecanol
PCM macrocapsule
silicone
solidification
thermal conductivity
thermal energy
Thermal energy storage
Thermal management
Thermoelectric power generation
Bi-In-Sn eutectic alloy
Thermoelectric power generation
Thermal energy storage
Thermal management
PCM macrocapsule
Octadecanol
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Abstract •A shape-remodeled PCM macrocapsule was fabricated through a cast molding method.•The EBiInSn-based flexible shell can sustain a maximum stretching of 432%.•The prepared PCM macrocapsule can be remodeled as needed to a complicated shape.•An innovative PCM-based conformal thermal control method was demonstrated.•The thermoelectric generation module based on PCM macrocapsule was developed. This paper reports on a novel phase change material macrocapsule for thermal energy storage, which can be dynamically and repeatably remodeled as needed to a complicated shape with large-scale deformation. In addition, it effectively eliminates the stress mismatch, induced by the volumetric expansion (or shrink) of the phase change material during melting (or solidification), through the self-adaptative deformation of the coated flexible shell. The shape-remodeled macrocapsule, consisting of octadecanol as the core and the silicone elastomer for encapsulation, was prepared through a cast molding method. The high-concentration microparticles of low-melting Bi-In-Sn eutectic alloys were embedded into elastic shell for significantly enhancing its latent heat storage and heat conductivity. The prepared macrocapsule has a high latent heat density of 210.1 MJ/m3, which of the contribution from the shell is about 20%. The thermal conductivity of the macrocapsule core reaches to 1.53 W/m·K with a 428% increase compared with pure octadecanol. The flexible shell attains a high thermal conductivity of 1.98 W/m·K with an 890% increase compared with pure silicone, which also remains a high stretchability with 432% strain. The performance of shape remodeling, energy storage capacity, and heat charging and discharging rates of the macrocapsule were demonstrated in detail. The applications of the prepared macrocapsule as thermal management for the flexible electronic devices and the thermal storage for thermoelectric energy harvesting were also investigated. The present study opens the way for further development of elastic phase change material capsule applications in energy storage systems and thermal control engineering.
AbstractList This paper reports on a novel phase change material macrocapsule for thermal energy storage, which can be dynamically and repeatably remodeled as needed to a complicated shape with large-scale deformation. In addition, it effectively eliminates the stress mismatch, induced by the volumetric expansion (or shrink) of the phase change material during melting (or solidification), through the self-adaptative deformation of the coated flexible shell. The shape-remodeled macrocapsule, consisting of octadecanol as the core and the silicone elastomer for encapsulation, was prepared through a cast molding method. The high-concentration microparticles of low-melting Bi-In-Sn eutectic alloys were embedded into elastic shell for significantly enhancing its latent heat storage and heat conductivity. The prepared macrocapsule has a high latent heat density of 210.1 MJ/m3, which of the contribution from the shell is about 20%. The thermal conductivity of the macrocapsule core reaches to 1.53 W/m·K with a 428% increase compared with pure octadecanol. The flexible shell attains a high thermal conductivity of 1.98 W/m·K with an 890% increase compared with pure silicone, which also remains a high stretchability with 432% strain. The performance of shape remodeling, energy storage capacity, and heat charging and discharging rates of the macrocapsule were demonstrated in detail. The applications of the prepared macrocapsule as thermal management for the flexible electronic devices and the thermal storage for thermoelectric energy harvesting were also investigated. The present study opens the way for further development of elastic phase change material capsule applications in energy storage systems and thermal control engineering.
•A shape-remodeled PCM macrocapsule was fabricated through a cast molding method.•The EBiInSn-based flexible shell can sustain a maximum stretching of 432%.•The prepared PCM macrocapsule can be remodeled as needed to a complicated shape.•An innovative PCM-based conformal thermal control method was demonstrated.•The thermoelectric generation module based on PCM macrocapsule was developed. This paper reports on a novel phase change material macrocapsule for thermal energy storage, which can be dynamically and repeatably remodeled as needed to a complicated shape with large-scale deformation. In addition, it effectively eliminates the stress mismatch, induced by the volumetric expansion (or shrink) of the phase change material during melting (or solidification), through the self-adaptative deformation of the coated flexible shell. The shape-remodeled macrocapsule, consisting of octadecanol as the core and the silicone elastomer for encapsulation, was prepared through a cast molding method. The high-concentration microparticles of low-melting Bi-In-Sn eutectic alloys were embedded into elastic shell for significantly enhancing its latent heat storage and heat conductivity. The prepared macrocapsule has a high latent heat density of 210.1 MJ/m3, which of the contribution from the shell is about 20%. The thermal conductivity of the macrocapsule core reaches to 1.53 W/m·K with a 428% increase compared with pure octadecanol. The flexible shell attains a high thermal conductivity of 1.98 W/m·K with an 890% increase compared with pure silicone, which also remains a high stretchability with 432% strain. The performance of shape remodeling, energy storage capacity, and heat charging and discharging rates of the macrocapsule were demonstrated in detail. The applications of the prepared macrocapsule as thermal management for the flexible electronic devices and the thermal storage for thermoelectric energy harvesting were also investigated. The present study opens the way for further development of elastic phase change material capsule applications in energy storage systems and thermal control engineering.
Author Yu, De-Hai
He, Zhi-Zhu
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  email: zzhe@cau.edu.cn
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Keywords Bi-In-Sn eutectic alloy
Thermoelectric power generation
Thermal energy storage
Thermal management
PCM macrocapsule
Octadecanol
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Snippet •A shape-remodeled PCM macrocapsule was fabricated through a cast molding method.•The EBiInSn-based flexible shell can sustain a maximum stretching of...
This paper reports on a novel phase change material macrocapsule for thermal energy storage, which can be dynamically and repeatably remodeled as needed to a...
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SubjectTerms alloys
Bi-In-Sn eutectic alloy
deformation
electronic equipment
encapsulation
engineering
heat
latent heat
melting
microparticles
Octadecanol
PCM macrocapsule
silicone
solidification
thermal conductivity
thermal energy
Thermal energy storage
Thermal management
Thermoelectric power generation
Title Shape-remodeled macrocapsule of phase change materials for thermal energy storage and thermal management
URI https://dx.doi.org/10.1016/j.apenergy.2019.04.072
https://www.proquest.com/docview/2237537098
Volume 247
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