Concentrated dual-cation electrolyte strategy for aqueous zinc-ion batteries
Rechargeable Zn-ion batteries are highly promising for stationary energy storage because of their low cost and intrinsic safety. However, due to the poor reversibility of Zn anodes and dissolution of oxide cathodes, aqueous Zn-ion batteries encounter rapid performance degradation when operating in c...
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| Published in | Energy & environmental science Vol. 14; no. 8; pp. 4463 - 4473 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Cambridge
Royal Society of Chemistry
11.08.2021
|
| Subjects | |
| Online Access | Get full text |
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| Abstract | Rechargeable Zn-ion batteries are highly promising for stationary energy storage because of their low cost and intrinsic safety. However, due to the poor reversibility of Zn anodes and dissolution of oxide cathodes, aqueous Zn-ion batteries encounter rapid performance degradation when operating in conventional low-concentration electrolytes. Herein, we demonstrate that an aqueous Zn
2+
electrolyte using a supporting Na salt at a high concentration is efficient to address these issues without sacrificing the power densities, cycling stability, and safety of zinc-ion batteries. We show that the high-concentration solute minimizes the number of free water molecules and the changes in the electronic state of the electrolyte. A combination of experimental and theoretical investigations reveals that a unique interphase, formed on the Zn anode, enables reversible and uniform Zn plating. Utilizing a cathode of sodium vanadate synthesized through a scalable strategy, the Zn-sodium vanadate battery with the concentrated bi-cation electrolyte shows improved cycling stability, decent rate performance, and low self-discharge. This work provides new insights on electrolyte engineering to achieve high-performance aqueous batteries.
A dual-cation concentrated electrolyte has been developed to enable a stable Zn anode and a vanadium-oxide-based cathode for efficient aqueous Zn-ion batteries. |
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| AbstractList | Rechargeable Zn-ion batteries are highly promising for stationary energy storage because of their low cost and intrinsic safety. However, due to the poor reversibility of Zn anodes and dissolution of oxide cathodes, aqueous Zn-ion batteries encounter rapid performance degradation when operating in conventional low-concentration electrolytes. Herein, we demonstrate that an aqueous Zn
2+
electrolyte using a supporting Na salt at a high concentration is efficient to address these issues without sacrificing the power densities, cycling stability, and safety of zinc-ion batteries. We show that the high-concentration solute minimizes the number of free water molecules and the changes in the electronic state of the electrolyte. A combination of experimental and theoretical investigations reveals that a unique interphase, formed on the Zn anode, enables reversible and uniform Zn plating. Utilizing a cathode of sodium vanadate synthesized through a scalable strategy, the Zn–sodium vanadate battery with the concentrated bi-cation electrolyte shows improved cycling stability, decent rate performance, and low self-discharge. This work provides new insights on electrolyte engineering to achieve high-performance aqueous batteries. Rechargeable Zn-ion batteries are highly promising for stationary energy storage because of their low cost and intrinsic safety. However, due to the poor reversibility of Zn anodes and dissolution of oxide cathodes, aqueous Zn-ion batteries encounter rapid performance degradation when operating in conventional low-concentration electrolytes. Herein, we demonstrate that an aqueous Zn2+ electrolyte using a supporting Na salt at a high concentration is efficient to address these issues without sacrificing the power densities, cycling stability, and safety of zinc-ion batteries. We show that the high-concentration solute minimizes the number of free water molecules and the changes in the electronic state of the electrolyte. A combination of experimental and theoretical investigations reveals that a unique interphase, formed on the Zn anode, enables reversible and uniform Zn plating. Utilizing a cathode of sodium vanadate synthesized through a scalable strategy, the Zn–sodium vanadate battery with the concentrated bi-cation electrolyte shows improved cycling stability, decent rate performance, and low self-discharge. This work provides new insights on electrolyte engineering to achieve high-performance aqueous batteries. Rechargeable Zn-ion batteries are highly promising for stationary energy storage because of their low cost and intrinsic safety. However, due to the poor reversibility of Zn anodes and dissolution of oxide cathodes, aqueous Zn-ion batteries encounter rapid performance degradation when operating in conventional low-concentration electrolytes. Herein, we demonstrate that an aqueous Zn 2+ electrolyte using a supporting Na salt at a high concentration is efficient to address these issues without sacrificing the power densities, cycling stability, and safety of zinc-ion batteries. We show that the high-concentration solute minimizes the number of free water molecules and the changes in the electronic state of the electrolyte. A combination of experimental and theoretical investigations reveals that a unique interphase, formed on the Zn anode, enables reversible and uniform Zn plating. Utilizing a cathode of sodium vanadate synthesized through a scalable strategy, the Zn-sodium vanadate battery with the concentrated bi-cation electrolyte shows improved cycling stability, decent rate performance, and low self-discharge. This work provides new insights on electrolyte engineering to achieve high-performance aqueous batteries. A dual-cation concentrated electrolyte has been developed to enable a stable Zn anode and a vanadium-oxide-based cathode for efficient aqueous Zn-ion batteries. |
| Author | Lei, Yongjiu Mohammed, Omar F Alshareef, Husam N Zheng, Xueli Emwas, Abdul-Hamid Yin, Jun Zhu, Yunpei Cui, Yi |
| AuthorAffiliation | Advanced Membranes & Porous Materials Center King Abdullah University of Science and Technology (KAUST) Stanford University Materials Science and Engineering Core Labs Division of Physical Science and Engineering KAUST Catalysis Center Department of Materials Science and Engineering Stanford Institute for Materials and Energy Sciences SLAC National Accelerator Laboratory |
| AuthorAffiliation_xml | – name: KAUST Catalysis Center – name: Advanced Membranes & Porous Materials Center – name: Division of Physical Science and Engineering – name: Core Labs – name: Materials Science and Engineering – name: King Abdullah University of Science and Technology (KAUST) – name: Stanford Institute for Materials and Energy Sciences – name: Stanford University – name: SLAC National Accelerator Laboratory – name: Department of Materials Science and Engineering |
| Author_xml | – sequence: 1 givenname: Yunpei surname: Zhu fullname: Zhu, Yunpei – sequence: 2 givenname: Jun surname: Yin fullname: Yin, Jun – sequence: 3 givenname: Xueli surname: Zheng fullname: Zheng, Xueli – sequence: 4 givenname: Abdul-Hamid surname: Emwas fullname: Emwas, Abdul-Hamid – sequence: 5 givenname: Yongjiu surname: Lei fullname: Lei, Yongjiu – sequence: 6 givenname: Omar F surname: Mohammed fullname: Mohammed, Omar F – sequence: 7 givenname: Yi surname: Cui fullname: Cui, Yi – sequence: 8 givenname: Husam N surname: Alshareef fullname: Alshareef, Husam N |
| BackLink | https://www.osti.gov/servlets/purl/1820151$$D View this record in Osti.gov |
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| ContentType | Journal Article |
| Copyright | Copyright Royal Society of Chemistry 2021 |
| Copyright_xml | – notice: Copyright Royal Society of Chemistry 2021 |
| CorporateAuthor | SLAC National Accelerator Lab., Menlo Park, CA (United States) |
| CorporateAuthor_xml | – name: SLAC National Accelerator Lab., Menlo Park, CA (United States) |
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| DOI | 10.1039/d1ee01472b |
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| Snippet | Rechargeable Zn-ion batteries are highly promising for stationary energy storage because of their low cost and intrinsic safety. However, due to the poor... |
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| SubjectTerms | Anodes Anodic dissolution Cathodes Cathodic dissolution Cations Cycles Dissolution Electrolytes Electron states ENERGY STORAGE Performance degradation Rechargeable batteries Safety Sodium Sodium compounds Stability Storage batteries Vanadate Vanadates Water chemistry Zinc |
| Title | Concentrated dual-cation electrolyte strategy for aqueous zinc-ion batteries |
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