Highly efficient fluorescence/phosphorescence hybrid white organic light-emitting devices based on a bipolar blue emitter to precisely control charges and excitons
Hybrid white organic light-emitting diodes (WOLEDs) combining blue fluorophores and green/red (or yellow) phosphors are still preferred for OLED production applications due to their advantages of good stability and high efficiency. One major challenge is to have a suitable blue fluorophore material...
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Published in | Journal of materials chemistry. C, Materials for optical and electronic devices Vol. 8; no. 22; pp. 7543 - 7551 |
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Main Authors | , , , , , , , , |
Format | Journal Article |
Language | English |
Published |
Cambridge
Royal Society of Chemistry
14.06.2020
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Subjects | |
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Abstract | Hybrid white organic light-emitting diodes (WOLEDs) combining blue fluorophores and green/red (or yellow) phosphors are still preferred for OLED production applications due to their advantages of good stability and high efficiency. One major challenge is to have a suitable blue fluorophore material to fully utilize the electrically generated excitons for fluorophore and phosphor emitters. Here, we employed an efficient blue fluorophore (
PBI-PPI-TPA
) with a high triplet energy of 2.48 eV as the blue emitter as well as the host for phosphors, whereby a series of highly efficient hybrid WOLEDs were successfully achieved. The two-color (BO) WOLEDs exhibited a maximum forward-viewing EQE/PE of up to 23.6%/77.8 lm W
−1
, and retained 20.0%/49.5 lm W
−1
at 1000 cd m
−2
, thus exhibiting high-efficiency and low-efficiency roll-off. Furthermore, three-color (BYR) hybrid WOLEDs were also fabricated by adopting blue-yellow-red cascade energy transfer to ensure that all the excitons could be effectively utilized for the white emission. The resulting devices achieved a peak EQE/PE of 21.5%/53.2 lm W
−1
, retained 17.2%/26.8 lm W
−1
at 1000 cd m
−2
, and the color rendering index (CRI) was doubled with respect to the two-color WOLEDs, showing a good trade-off between the efficiency and CRI. All these results are among the best reported for hybrid WOLEDs.
Highly efficient fluorescence/phosphorescence hybrid WOLEDs have been realized by employing a new efficient blue fluorescent material. |
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AbstractList | Hybrid white organic light-emitting diodes (WOLEDs) combining blue fluorophores and green/red (or yellow) phosphors are still preferred for OLED production applications due to their advantages of good stability and high efficiency. One major challenge is to have a suitable blue fluorophore material to fully utilize the electrically generated excitons for fluorophore and phosphor emitters. Here, we employed an efficient blue fluorophore (
PBI-PPI-TPA
) with a high triplet energy of 2.48 eV as the blue emitter as well as the host for phosphors, whereby a series of highly efficient hybrid WOLEDs were successfully achieved. The two-color (BO) WOLEDs exhibited a maximum forward-viewing EQE/PE of up to 23.6%/77.8 lm W
−1
, and retained 20.0%/49.5 lm W
−1
at 1000 cd m
−2
, thus exhibiting high-efficiency and low-efficiency roll-off. Furthermore, three-color (BYR) hybrid WOLEDs were also fabricated by adopting blue-yellow-red cascade energy transfer to ensure that all the excitons could be effectively utilized for the white emission. The resulting devices achieved a peak EQE/PE of 21.5%/53.2 lm W
−1
, retained 17.2%/26.8 lm W
−1
at 1000 cd m
−2
, and the color rendering index (CRI) was doubled with respect to the two-color WOLEDs, showing a good trade-off between the efficiency and CRI. All these results are among the best reported for hybrid WOLEDs. Hybrid white organic light-emitting diodes (WOLEDs) combining blue fluorophores and green/red (or yellow) phosphors are still preferred for OLED production applications due to their advantages of good stability and high efficiency. One major challenge is to have a suitable blue fluorophore material to fully utilize the electrically generated excitons for fluorophore and phosphor emitters. Here, we employed an efficient blue fluorophore (PBI-PPI-TPA) with a high triplet energy of 2.48 eV as the blue emitter as well as the host for phosphors, whereby a series of highly efficient hybrid WOLEDs were successfully achieved. The two-color (BO) WOLEDs exhibited a maximum forward-viewing EQE/PE of up to 23.6%/77.8 lm W−1, and retained 20.0%/49.5 lm W−1 at 1000 cd m−2, thus exhibiting high-efficiency and low-efficiency roll-off. Furthermore, three-color (BYR) hybrid WOLEDs were also fabricated by adopting blue-yellow-red cascade energy transfer to ensure that all the excitons could be effectively utilized for the white emission. The resulting devices achieved a peak EQE/PE of 21.5%/53.2 lm W−1, retained 17.2%/26.8 lm W−1 at 1000 cd m−2, and the color rendering index (CRI) was doubled with respect to the two-color WOLEDs, showing a good trade-off between the efficiency and CRI. All these results are among the best reported for hybrid WOLEDs. Hybrid white organic light-emitting diodes (WOLEDs) combining blue fluorophores and green/red (or yellow) phosphors are still preferred for OLED production applications due to their advantages of good stability and high efficiency. One major challenge is to have a suitable blue fluorophore material to fully utilize the electrically generated excitons for fluorophore and phosphor emitters. Here, we employed an efficient blue fluorophore ( PBI-PPI-TPA ) with a high triplet energy of 2.48 eV as the blue emitter as well as the host for phosphors, whereby a series of highly efficient hybrid WOLEDs were successfully achieved. The two-color (BO) WOLEDs exhibited a maximum forward-viewing EQE/PE of up to 23.6%/77.8 lm W −1 , and retained 20.0%/49.5 lm W −1 at 1000 cd m −2 , thus exhibiting high-efficiency and low-efficiency roll-off. Furthermore, three-color (BYR) hybrid WOLEDs were also fabricated by adopting blue-yellow-red cascade energy transfer to ensure that all the excitons could be effectively utilized for the white emission. The resulting devices achieved a peak EQE/PE of 21.5%/53.2 lm W −1 , retained 17.2%/26.8 lm W −1 at 1000 cd m −2 , and the color rendering index (CRI) was doubled with respect to the two-color WOLEDs, showing a good trade-off between the efficiency and CRI. All these results are among the best reported for hybrid WOLEDs. Highly efficient fluorescence/phosphorescence hybrid WOLEDs have been realized by employing a new efficient blue fluorescent material. |
Author | Dai, Yanfeng Zhu, Jieji Ma, Dongge Yang, Dezhi Qiao, Xianfeng Tong, Qingxiao Chen, Yuwen Wu, Yibing Yao, Jingwen |
AuthorAffiliation | South China University of Technology Institute of Polymer Optoelectronic Materials and Devices Shantou University Guangdong Provincial Key Laboratory of Luminescence from Molecular Aggregates Department of Chemistry and Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province State Key Laboratory of Luminescent Materials and Devices |
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CitedBy_id | crossref_primary_10_1002_adom_202101518 crossref_primary_10_1039_D2QM01008A crossref_primary_10_1016_j_cej_2023_145867 crossref_primary_10_1016_j_optmat_2021_111059 crossref_primary_10_1039_D0CC05602B crossref_primary_10_1063_5_0067935 crossref_primary_10_1039_D0TC04934D crossref_primary_10_1039_D3TC03449F crossref_primary_10_1002_chem_202100717 crossref_primary_10_1039_D2TC03601K crossref_primary_10_1039_D4CP00737A crossref_primary_10_1002_adom_202200915 crossref_primary_10_1016_j_synthmet_2020_116666 crossref_primary_10_1002_adfm_202100704 crossref_primary_10_1016_j_jiec_2021_09_014 crossref_primary_10_1016_j_dyepig_2021_110077 crossref_primary_10_1016_j_dyepig_2021_109868 crossref_primary_10_1002_adom_202100298 crossref_primary_10_1016_j_molstruc_2021_132090 crossref_primary_10_3788_IRLA20230222 |
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SubjectTerms | Chemical compounds Devices Efficiency Emitters Energy transfer Excitons Fluorescence Organic light emitting diodes Phosphorescence Phosphors |
Title | Highly efficient fluorescence/phosphorescence hybrid white organic light-emitting devices based on a bipolar blue emitter to precisely control charges and excitons |
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