Electrochemically self-cleanable carbon nanotube interlayered membrane for enhanced forward osmosis in wastewater treatment

Forward osmosis (FO) is considered as a promising alternative to pressure-driven membrane processes for wastewater treatment due to its relatively low-energy operation and better fouling resistance, but biofouling still occurs during long-time operation. The electrochemical cleaning strategy is effe...

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Published inJournal of environmental chemical engineering Vol. 10; no. 3; p. 107399
Main Authors Wang, Yun-Jie, Huang, Liang, Fang, Zheng, Wang, Xue-Meng, Gao, Miao, Liu, Hou-Qi, Li, Wen-Wei, Huang, Tian-Yin
Format Journal Article
LanguageEnglish
Published Elsevier Ltd 01.06.2022
Subjects
Biofouling
Carbon nanotubes
Forward osmosis
Reactive chlorine species
Salinity buildup
Carbon nanotubes
Forward osmosis
Salinity buildup
Biofouling
Reactive chlorine species
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Abstract Forward osmosis (FO) is considered as a promising alternative to pressure-driven membrane processes for wastewater treatment due to its relatively low-energy operation and better fouling resistance, but biofouling still occurs during long-time operation. The electrochemical cleaning strategy is effective for membrane fouling control, but has been seldom applied to FO processes so far due to unsatisfactory performance. Here, we fabricated a carbon nanotube-interlayered thin-film composite membrane with high electric conductivity, water permeability and self-cleaning ability to favor FO operation. By taking advantage of the electro-generated oxidative species in situ, especially the reactive chlorine species generated from locally-accumulated chlorine ions, the deposited bacterial cells and extracellular polymeric substances on membrane surface were efficiently removed to sustain the membrane operation. Applying 2.5 V voltage to the fouled membrane for 30 min restored 85% of its original water flux, and remained stable performance in three operating cycles. Overall, our work provides an efficient electrochemical cleaning strategy for FO membrane fouling control, which may further promote the application of FO wastewater treatment technologies. [Display omitted] •Conductive CNT-modified TFC forward osmosis membrane was fabricated.•CNT-TFC membrane exhibited high electrochemical activity and stability.•Reversely-diffused and locally-enriched Cl- was oxidized to generate free chlorine.•Electrochemical cleaning of the membrane efficiently removed the biofoulants.
AbstractList Forward osmosis (FO) is considered as a promising alternative to pressure-driven membrane processes for wastewater treatment due to its relatively low-energy operation and better fouling resistance, but biofouling still occurs during long-time operation. The electrochemical cleaning strategy is effective for membrane fouling control, but has been seldom applied to FO processes so far due to unsatisfactory performance. Here, we fabricated a carbon nanotube-interlayered thin-film composite membrane with high electric conductivity, water permeability and self-cleaning ability to favor FO operation. By taking advantage of the electro-generated oxidative species in situ, especially the reactive chlorine species generated from locally-accumulated chlorine ions, the deposited bacterial cells and extracellular polymeric substances on membrane surface were efficiently removed to sustain the membrane operation. Applying 2.5 V voltage to the fouled membrane for 30 min restored 85% of its original water flux, and remained stable performance in three operating cycles. Overall, our work provides an efficient electrochemical cleaning strategy for FO membrane fouling control, which may further promote the application of FO wastewater treatment technologies. [Display omitted] •Conductive CNT-modified TFC forward osmosis membrane was fabricated.•CNT-TFC membrane exhibited high electrochemical activity and stability.•Reversely-diffused and locally-enriched Cl- was oxidized to generate free chlorine.•Electrochemical cleaning of the membrane efficiently removed the biofoulants.
ArticleNumber 107399
Author Wang, Yun-Jie
Huang, Liang
Li, Wen-Wei
Liu, Hou-Qi
Fang, Zheng
Huang, Tian-Yin
Wang, Xue-Meng
Gao, Miao
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  organization: National and Local Joint Engineering Laboratory for Municipal Sewage Resource Utilization Technology, Suzhou University of Science and Technology, Suzhou 215009, China
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Keywords Carbon nanotubes
Forward osmosis
Salinity buildup
Biofouling
Reactive chlorine species
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Snippet Forward osmosis (FO) is considered as a promising alternative to pressure-driven membrane processes for wastewater treatment due to its relatively low-energy...
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SubjectTerms Biofouling
Carbon nanotubes
Forward osmosis
Reactive chlorine species
Salinity buildup
Title Electrochemically self-cleanable carbon nanotube interlayered membrane for enhanced forward osmosis in wastewater treatment
URI https://dx.doi.org/10.1016/j.jece.2022.107399
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