Recent progress of Ni-based catalysts for methanol electrooxidation reaction in alkaline media

Methanol as an important hydrogen-rich fuel has received increasing attention in energy storage and conversion techniques, and energy release can be realized in the methanol oxidation reaction (MOR) process. Note that highly efficient catalysts are still required to drive methanol oxidation, and the...

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Published inAdvanced Sensor and Energy Materials Vol. 2; no. 2; p. 100055
Main Authors Liu, Chunru, Yang, Fulin, Schechter, Alex, Feng, Ligang
Format Journal Article
LanguageEnglish
Published Elsevier B.V 01.06.2023
Elsevier
Subjects
Electrocatalysis
Methanol oxidation reaction
Ni-based catalyst
Promotion principle
Electrocatalysis
Methanol oxidation reaction
Ni-based catalyst
Promotion principle
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Abstract Methanol as an important hydrogen-rich fuel has received increasing attention in energy storage and conversion techniques, and energy release can be realized in the methanol oxidation reaction (MOR) process. Note that highly efficient catalysts are still required to drive methanol oxidation, and the Ni-based catalysts have received intensive attention due to their facile active site generation based on the electrochemical-chemical oxidation mechanisms. In light of the significant advances made recently, herein, we reviewed the recent advances of Ni-based catalysts for methanol oxidation in the alkaline medium. The fundamental of methanol oxidation in the alkaline medium was first presented, and then the catalyst design principles including synergistic effect, electronic effect, defect construction, doping effect, as well as surface reconstruction were presented; and the advances of various Ni-based catalysts for MOR are summarized and discussed by combining with some typical examples. The problems and challenges were also concluded for the Ni-based catalyst fabrication, the performance evaluation, and their application. We believe that the summary of this review will be helpful in the design of nickel-based catalysts and understanding the catalysis mechanism of nickel-based materials in alcohol fuel electrochemical reactions. [Display omitted]
AbstractList Methanol as an important hydrogen-rich fuel has received increasing attention in energy storage and conversion techniques, and energy release can be realized in the methanol oxidation reaction (MOR) process. Note that highly efficient catalysts are still required to drive methanol oxidation, and the Ni-based catalysts have received intensive attention due to their facile active site generation based on the electrochemical-chemical oxidation mechanisms. In light of the significant advances made recently, herein, we reviewed the recent advances of Ni-based catalysts for methanol oxidation in the alkaline medium. The fundamental of methanol oxidation in the alkaline medium was first presented, and then the catalyst design principles including synergistic effect, electronic effect, defect construction, doping effect, as well as surface reconstruction were presented; and the advances of various Ni-based catalysts for MOR are summarized and discussed by combining with some typical examples. The problems and challenges were also concluded for the Ni-based catalyst fabrication, the performance evaluation, and their application. We believe that the summary of this review will be helpful in the design of nickel-based catalysts and understanding the catalysis mechanism of nickel-based materials in alcohol fuel electrochemical reactions. [Display omitted]
Methanol as an important hydrogen-rich fuel has received increasing attention in energy storage and conversion techniques, and energy release can be realized in the methanol oxidation reaction (MOR) process. Note that highly efficient catalysts are still required to drive methanol oxidation, and the Ni-based catalysts have received intensive attention due to their facile active site generation based on the electrochemical-chemical oxidation mechanisms. In light of the significant advances made recently, herein, we reviewed the recent advances of Ni-based catalysts for methanol oxidation in the alkaline medium. The fundamental of methanol oxidation in the alkaline medium was first presented, and then the catalyst design principles including synergistic effect, electronic effect, defect construction, doping effect, as well as surface reconstruction were presented; and the advances of various Ni-based catalysts for MOR are summarized and discussed by combining with some typical examples. The problems and challenges were also concluded for the Ni-based catalyst fabrication, the performance evaluation, and their application. We believe that the summary of this review will be helpful in the design of nickel-based catalysts and understanding the catalysis mechanism of nickel-based materials in alcohol fuel electrochemical reactions.
ArticleNumber 100055
Author Yang, Fulin
Feng, Ligang
Liu, Chunru
Schechter, Alex
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  fullname: Yang, Fulin
  organization: School of Chemistry and Chemical Engineering, Yangzhou University, Yangzhou, 225002, PR China
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  givenname: Alex
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  surname: Schechter
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  organization: Department of Chemical Science, Ariel University, Ariel, 40700, Israel
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  givenname: Ligang
  orcidid: 0000-0001-9879-0773
  surname: Feng
  fullname: Feng, Ligang
  email: ligang.feng@yzu.edu.cn, fenglg11@gmail.com
  organization: School of Chemistry and Chemical Engineering, Yangzhou University, Yangzhou, 225002, PR China
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Keywords Electrocatalysis
Methanol oxidation reaction
Ni-based catalyst
Promotion principle
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Snippet Methanol as an important hydrogen-rich fuel has received increasing attention in energy storage and conversion techniques, and energy release can be realized...
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SubjectTerms Electrocatalysis
Methanol oxidation reaction
Ni-based catalyst
Promotion principle
Title Recent progress of Ni-based catalysts for methanol electrooxidation reaction in alkaline media
URI https://dx.doi.org/10.1016/j.asems.2023.100055
https://doaj.org/article/1716131cb647400eb79a315cd0e4b594
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