Construction of nanowall-supported-nanorod nico ldh array electrode with high mass-loading on carbon cloth for high-performance asymmetric supercapacitors
•Nanowall-supported-nanorod nico LDH arrays with open holey framework are obtained.•Electrode with high loading of 5.85 mg cm−2 shows the capacitance of 7.73 F cm−2.•All-solid-state asymmetric supercapacitor delivers 6.37 mWh cm−3 at 62.5 mW cm−2. Carbon cloth is regarded as a promising substrate fo...
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| Published in | Electrochimica acta Vol. 362; p. 137081 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Oxford
Elsevier Ltd
01.12.2020
Elsevier BV |
| Subjects | |
| Online Access | Get full text |
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| Abstract | •Nanowall-supported-nanorod nico LDH arrays with open holey framework are obtained.•Electrode with high loading of 5.85 mg cm−2 shows the capacitance of 7.73 F cm−2.•All-solid-state asymmetric supercapacitor delivers 6.37 mWh cm−3 at 62.5 mW cm−2.
Carbon cloth is regarded as a promising substrate for supercapacitors due to its good electrical conductivity, light weight and flexibility. However, its relatively hydrophobic property prevents the large-scale growth of active substances, restricting the potential practical applications. In this paper, by using NiCo LDH nanowall array as a hydrophilic substrate, a high mass-loading nanowall-supported-nanorod NiCo LDH arrays are formed via an alternate solvo/hydrothermal synthesis and subsequently alkali conversion process. The strong substrate adhesion of NiCo LDH nanoarrays ensures efficient electron transfer of the electrode. Moreover, the as-achieved open holey framework, integrated by free-standing nanorods and porous nanowalls, provides a hierarchical nanostructure for realizing the enhanced capacitive performance. Consequently, nanowall-supported-nanorod NiCo LDH electrode achieves a high capacitance of 7.73 F cm−2 at a current density of 5 mA cm−2 with excellent rate performance. When assembled into an all-solid-state hybrid supercapacitor, it delivers a maximum working voltage of 1.8 V, and an energy density of 0.46 mWh cm−2 (6.37 mWh cm−3) at a power density of 4.5 mW cm−2 (62.5 mW cm−2). Therefore, this work provides a proof-of-concept design for the high-performance supercapacitor electrode with carbon cloth substrate.
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| AbstractList | Carbon cloth is regarded as a promising substrate for supercapacitors due to its good electrical conductivity, light weight and flexibility. However, its relatively hydrophobic property prevents the large-scale growth of active substances, restricting the potential practical applications. In this paper, by using NiCo LDH nanowall array as a hydrophilic substrate, a high mass-loading nanowall-supported-nanorod NiCo LDH arrays are formed via an alternate solvo/hydrothermal synthesis and subsequently alkali conversion process. The strong substrate adhesion of NiCo LDH nanoarrays ensures efficient electron transfer of the electrode. Moreover, the as-achieved open holey framework, integrated by free-standing nanorods and porous nanowalls, provides a hierarchical nanostructure for realizing the enhanced capacitive performance. Consequently, nanowall-supported-nanorod NiCo LDH electrode achieves a high capacitance of 7.73 F cm−2 at a current density of 5 mA cm−2 with excellent rate performance. When assembled into an all-solid-state hybrid supercapacitor, it delivers a maximum working voltage of 1.8 V, and an energy density of 0.46 mWh cm−2 (6.37 mWh cm−3) at a power density of 4.5 mW cm−2 (62.5 mW cm−2). Therefore, this work provides a proof-of-concept design for the high-performance supercapacitor electrode with carbon cloth substrate. •Nanowall-supported-nanorod nico LDH arrays with open holey framework are obtained.•Electrode with high loading of 5.85 mg cm−2 shows the capacitance of 7.73 F cm−2.•All-solid-state asymmetric supercapacitor delivers 6.37 mWh cm−3 at 62.5 mW cm−2. Carbon cloth is regarded as a promising substrate for supercapacitors due to its good electrical conductivity, light weight and flexibility. However, its relatively hydrophobic property prevents the large-scale growth of active substances, restricting the potential practical applications. In this paper, by using NiCo LDH nanowall array as a hydrophilic substrate, a high mass-loading nanowall-supported-nanorod NiCo LDH arrays are formed via an alternate solvo/hydrothermal synthesis and subsequently alkali conversion process. The strong substrate adhesion of NiCo LDH nanoarrays ensures efficient electron transfer of the electrode. Moreover, the as-achieved open holey framework, integrated by free-standing nanorods and porous nanowalls, provides a hierarchical nanostructure for realizing the enhanced capacitive performance. Consequently, nanowall-supported-nanorod NiCo LDH electrode achieves a high capacitance of 7.73 F cm−2 at a current density of 5 mA cm−2 with excellent rate performance. When assembled into an all-solid-state hybrid supercapacitor, it delivers a maximum working voltage of 1.8 V, and an energy density of 0.46 mWh cm−2 (6.37 mWh cm−3) at a power density of 4.5 mW cm−2 (62.5 mW cm−2). Therefore, this work provides a proof-of-concept design for the high-performance supercapacitor electrode with carbon cloth substrate. [Display omitted] |
| ArticleNumber | 137081 |
| Author | Ye, Jing Chen, Shihuan Chen, Huizhen Yang, Luhuan Xu, Xuetang Liao, Shuqing Wang, Fan Yang, Tianyi |
| Author_xml | – sequence: 1 givenname: Tianyi surname: Yang fullname: Yang, Tianyi – sequence: 2 givenname: Jing surname: Ye fullname: Ye, Jing – sequence: 3 givenname: Shihuan surname: Chen fullname: Chen, Shihuan – sequence: 4 givenname: Shuqing surname: Liao fullname: Liao, Shuqing – sequence: 5 givenname: Huizhen surname: Chen fullname: Chen, Huizhen – sequence: 6 givenname: Luhuan surname: Yang fullname: Yang, Luhuan – sequence: 7 givenname: Xuetang surname: Xu fullname: Xu, Xuetang email: xxtang@gxu.edu.cn – sequence: 8 givenname: Fan orcidid: 0000-0002-6106-4724 surname: Wang fullname: Wang, Fan email: fanwang@gxu.edu.cn |
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| Snippet | •Nanowall-supported-nanorod nico LDH arrays with open holey framework are obtained.•Electrode with high loading of 5.85 mg cm−2 shows the capacitance of 7.73 F... Carbon cloth is regarded as a promising substrate for supercapacitors due to its good electrical conductivity, light weight and flexibility. However, its... |
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| SubjectTerms | Adhesive strength Areal capacitance Arrays Carbon Cloth Data integration Electrical resistivity Electrodes Electron transfer Flux density High mass-loading Intermetallic compounds Nanorods NiCo LDH Substrates Supercapacitor Supercapacitors Weight reduction |
| Title | Construction of nanowall-supported-nanorod nico ldh array electrode with high mass-loading on carbon cloth for high-performance asymmetric supercapacitors |
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