Study on the formation, development and coating mechanism of new phases on interface in LiNbO3-coated LiCoO2
Surface coating is one of important methods to improve the electrochemial performances of cathode material for Li-ion batteries. Few work focuses on whether the “the formed coating surface” is “the chosen coating surface” or not. In this study, it has been found that bulk material LiCoO2 (LCO) and t...
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| Published in | Electrochimica acta Vol. 368; p. 137639 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Oxford
Elsevier Ltd
01.02.2021
Elsevier BV |
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| Abstract | Surface coating is one of important methods to improve the electrochemial performances of cathode material for Li-ion batteries. Few work focuses on whether the “the formed coating surface” is “the chosen coating surface” or not. In this study, it has been found that bulk material LiCoO2 (LCO) and the LiNbO3 coating material can react to produce Li3NbO4 and Co3O4 and form new coating layers during heating. The development of the new coating layers after calcination and their effect on the electrochemical performance of LiCoO2 have been thoroughly studied. Different types of coating layers (LiNbO3, LiNbO3/Li3NbO4/Co3O4, Li3NbO4/Co3O4 coating layers) were designed and obtained. The formation of new coating layer played a vital role in improving the electrochemical properties of coated materials. Coated LCO obtained at 650 oC with a LiNbO3/Li3NbO4/Co3O4 new coating layer exhibited the most excellent cycle stability with a capacity retention of 94.3% after 100 cycles at 0.2 C. The coating mechanism was studied. Both the composition and coating surface structure affect the performances of coated LCO. LiNbO3/Li3NbO4/Co3O4-coated LCO had the most uniform and integrated coating layer, maintained well crystal structure after long-term charging-discharging process. In addition, the LiNbO3/Li3NbO4/Co3O4 coating layer has been proved to inhibit the growth of cathode electrolyte interface. |
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| AbstractList | Surface coating is one of important methods to improve the electrochemial performances of cathode material for Li-ion batteries. Few work focuses on whether the "the formed coating surface" is "the chosen coating surface" or not. In this study, it has been found that bulk material LiCoO2 (LCO) and the LiNbO3 coating material can react to produce Li3NbO4 and Co3O4 and form new coating layers during heating. The development of the new coating layers after calcination and their effect on the electrochemical performance of LiCoO2 have been thoroughly studied. Different types of coating layers (LiNbO3, LiNbO3/Li3NbO4/Co3O4, Li3NbO4/Co3O4 coating layers) were designed and obtained. The formation of new coating layer played a vital role in improving the electrochemical properties of coated materials. Coated LCO obtained at 650 oC with a LiNbO3/Li3NbO4/Co3O4 new coating layer exhibited the most excellent cycle stability with a capacity retention of 94.3% after 100 cycles at 0.2 C. The coating mechanism was studied. Both the composition and coating surface structure affect the performances of coated LCO. LiNbO3/Li3NbO4/Co3O4-coated LCO had the most uniform and integrated coating layer, maintained well crystal structure after long-term charging-discharging process. In addition, the LiNbO3/Li3NbO4/Co3O4 coating layer has been proved to inhibit the growth of cathode electrolyte interface. |
| ArticleNumber | 137639 |
| Author | Shi, Xixi Zhang, Yuting Lu, Guozhong Zhang, Lianqi Song, Dawei Zhang, Hongzhou Peng, Wenxiu Wang, Xiaoqing |
| Author_xml | – sequence: 1 givenname: Guozhong surname: Lu fullname: Lu, Guozhong organization: School of Environment and Chemical Engineering, Tianjin Polytechnic University, Tianjin 300387, China – sequence: 2 givenname: Wenxiu surname: Peng fullname: Peng, Wenxiu organization: Shandong Ruifu Lithium Co., Ltd., Taian 271601 China – sequence: 3 givenname: Yuting surname: Zhang fullname: Zhang, Yuting organization: School of Environment and Chemical Engineering, Tianjin Polytechnic University, Tianjin 300387, China – sequence: 4 givenname: Xiaoqing surname: Wang fullname: Wang, Xiaoqing email: xiaoqingwang2012@126.com organization: School of Environment and Chemical Engineering, Tianjin Polytechnic University, Tianjin 300387, China – sequence: 5 givenname: Xixi surname: Shi fullname: Shi, Xixi organization: Tianjin Key Laboratory for Photoelectric Materials and Devices, School of Materials Science and Engineering, Tianjin University of Technology, Tianjin 300384, China – sequence: 6 givenname: Dawei surname: Song fullname: Song, Dawei organization: Tianjin Key Laboratory for Photoelectric Materials and Devices, School of Materials Science and Engineering, Tianjin University of Technology, Tianjin 300384, China – sequence: 7 givenname: Hongzhou surname: Zhang fullname: Zhang, Hongzhou organization: Tianjin Key Laboratory for Photoelectric Materials and Devices, School of Materials Science and Engineering, Tianjin University of Technology, Tianjin 300384, China – sequence: 8 givenname: Lianqi surname: Zhang fullname: Zhang, Lianqi email: tianjinzhanglq@163.com organization: Tianjin Key Laboratory for Photoelectric Materials and Devices, School of Materials Science and Engineering, Tianjin University of Technology, Tianjin 300384, China |
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| Keywords | Lithium-ion batteries Layered oxide materials New phases Coated LiCoO2 Interface |
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| SubjectTerms | Cathodes Coated LiCoO2 Coating Cobalt oxides Crystal structure Electrochemical analysis Electrode materials Interface Layered oxide materials Lithium compounds Lithium niobates Lithium-ion batteries New phases Protective coatings Rechargeable batteries Surface structure |
| Title | Study on the formation, development and coating mechanism of new phases on interface in LiNbO3-coated LiCoO2 |
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