The influence of samarium (Sm) on the discharge and electrochemical behaviors of the magnesium alloy AZ80 as an anode for the Mg-air battery
The influence of Sm on the microstructure, electrochemical properties, and discharge performance of cast AZ80 as the anode for Mg-air battery are investigated. AZ80 containing Sm has refined α-Mg grains and contains the Al2Sm phase. With increasing Sm content, the number and size of the Mg17Al12 pha...
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| Published in | Electrochimica acta Vol. 348; p. 136315 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Oxford
Elsevier Ltd
10.07.2020
Elsevier BV |
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| Abstract | The influence of Sm on the microstructure, electrochemical properties, and discharge performance of cast AZ80 as the anode for Mg-air battery are investigated. AZ80 containing Sm has refined α-Mg grains and contains the Al2Sm phase. With increasing Sm content, the number and size of the Mg17Al12 phase particles are reduced. The AZ80-xSm anodes have higher electrochemical activity and lower self-corrosion rates than AZ80. The AZ80-xSm anodes also have a high discharge performance and a stable discharge voltage, which is attributed to the refined structure and Al2Sm particles. The AZ80-3Sm anode has the best discharge capacity of 1439 mAh g−1 and the best anode efficiency of 65% at 40 mA cm−2, which are 17% and 20% higher than for the AZ80 anode. This anode has an output peak energy of 1719 mWh g−1 at both 10 and 20 mA cm−2, compared with 1510 mWh g−1 for AZ80 at only 20 mA cm−2. The AZ80-xSm anodes have smoother discharge surface morphology, which is beneficial to the exfoliation of discharge products. |
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| AbstractList | The influence of Sm on the microstructure, electrochemical properties, and discharge performance of cast AZ80 as the anode for Mg-air battery are investigated. AZ80 containing Sm has refined α-Mg grains and contains the Al2Sm phase. With increasing Sm content, the number and size of the Mg17Al12 phase particles are reduced. The AZ80-xSm anodes have higher electrochemical activity and lower self-corrosion rates than AZ80. The AZ80-xSm anodes also have a high discharge performance and a stable discharge voltage, which is attributed to the refined structure and Al2Sm particles. The AZ80-3Sm anode has the best discharge capacity of 1439 mAh g−1 and the best anode efficiency of 65% at 40 mA cm−2, which are 17% and 20% higher than for the AZ80 anode. This anode has an output peak energy of 1719 mWh g−1 at both 10 and 20 mA cm−2, compared with 1510 mWh g−1 for AZ80 at only 20 mA cm−2. The AZ80-xSm anodes have smoother discharge surface morphology, which is beneficial to the exfoliation of discharge products. The influence of Sm on the microstructure, electrochemical properties, and discharge performance of cast AZ80 as the anode for Mg-air battery are investigated. AZ80 containing Sm has refined α-Mg grains and contains the Al2Sm phase. With increasing Sm content, the number and size of the Mg17Al12 phase particles are reduced. The AZ80-xSm anodes have higher electrochemical activity and lower self-corrosion rates than AZ80. The AZ80-xSm anodes also have a high discharge performance and a stable discharge voltage, which is attributed to the refined structure and Al2Sm particles. The AZ80-3Sm anode has the best discharge capacity of 1439 mAh g−1 and the best anode efficiency of 65% at 40 mA cm−2, which are 17% and 20% higher than for the AZ80 anode. This anode has an output peak energy of 1719 mWh g−1 at both 10 and 20 mA cm−2, compared with 1510 mWh g−1 for AZ80 at only 20 mA cm−2. The AZ80-xSm anodes have smoother discharge surface morphology, which is beneficial to the exfoliation of discharge products. |
| ArticleNumber | 136315 |
| Author | Liao, Qiyu Atrens, Andrej Le, Qichi Zou, Qi Chen, Xingrui Wang, Henan |
| Author_xml | – sequence: 1 givenname: Xingrui surname: Chen fullname: Chen, Xingrui email: neuchenxr@163.com organization: Key Lab of Electromagnetic Processing of Materials, Ministry of Education, Northeastern University, 314 Mailbox, Shenyang, 110819, People’s Republic of China – sequence: 2 givenname: Qiyu surname: Liao fullname: Liao, Qiyu organization: Key Lab of Electromagnetic Processing of Materials, Ministry of Education, Northeastern University, 314 Mailbox, Shenyang, 110819, People’s Republic of China – sequence: 3 givenname: Qichi surname: Le fullname: Le, Qichi email: qichil@mail.neu.edu.cn organization: Key Lab of Electromagnetic Processing of Materials, Ministry of Education, Northeastern University, 314 Mailbox, Shenyang, 110819, People’s Republic of China – sequence: 4 givenname: Qi surname: Zou fullname: Zou, Qi organization: Key Lab of Electromagnetic Processing of Materials, Ministry of Education, Northeastern University, 314 Mailbox, Shenyang, 110819, People’s Republic of China – sequence: 5 givenname: Henan surname: Wang fullname: Wang, Henan organization: Key Lab of Electromagnetic Processing of Materials, Ministry of Education, Northeastern University, 314 Mailbox, Shenyang, 110819, People’s Republic of China – sequence: 6 givenname: Andrej surname: Atrens fullname: Atrens, Andrej email: andrejs.atrens@uq.edu.au organization: School of Mechanical and Mining Engineering, The University of Queensland, St. Lucia, QLD, 4072, Australia |
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| SubjectTerms | Anodes Corrosion rate Discharge Discharge performance Electrochemical analysis Electrochemical behaviors Magnesium alloy Magnesium base alloys Metal air batteries Mg-air batteries Morphology RE element Samarium |
| Title | The influence of samarium (Sm) on the discharge and electrochemical behaviors of the magnesium alloy AZ80 as an anode for the Mg-air battery |
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