Exploration of photocatalytic activities of titanosilicate ETS-10 and transition metal incorporated ETS-10
Microporous titanium silicate [ETS-10, (Na,K) 2TiSi 5O 13] and transition metal ions incorporated titanium silicates were investigated for the photocatalytic decomposition of acetaldehyde. ETS-10 with a photoexcitable linear chain of titanium and oxygen decomposed acetaldehyde under UV radiation and...
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| Published in | Microporous and mesoporous materials Vol. 67; no. 2; pp. 181 - 187 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Amsterdam
Elsevier Inc
06.02.2004
Elsevier |
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| Abstract | Microporous titanium silicate [ETS-10, (Na,K)
2TiSi
5O
13] and transition metal ions incorporated titanium silicates were investigated for the photocatalytic decomposition of acetaldehyde. ETS-10 with a photoexcitable linear chain of titanium and oxygen decomposed acetaldehyde under UV radiation and the rate constant for the decrease of acetaldehyde (0.010 m
−1) is comparable to that of pure TiO
2 (0.013 m
−1). Interesting visible (
λ>420 nm) and UV light activity was found for ETS-10 samples incorporated with Cr and Co [ETS-10 with Cr(or)Co/Ti=0.05] and for materials synthesized by ion-exchange reactions such as Co-ETS-10 and Ag-ETS-10. All other ion-exchanged (Na,K)
2−
x
M
′
x
TiSi
5O
13 (M
′=Cr(III), Mn(II), Fe(III), Co(II), Ni(II), and Cu(II)) samples were found to be active photocatalysts that can decompose acetaldehyde under UV radiation. Materials synthesized were characterized by a variety of techniques such as powder X-ray diffraction, BET surface area and UV–VIS diffuse reflectance measurements. |
|---|---|
| AbstractList | Microporous titanium silicate [ETS-10, (Na,K)
2TiSi
5O
13] and transition metal ions incorporated titanium silicates were investigated for the photocatalytic decomposition of acetaldehyde. ETS-10 with a photoexcitable linear chain of titanium and oxygen decomposed acetaldehyde under UV radiation and the rate constant for the decrease of acetaldehyde (0.010 m
−1) is comparable to that of pure TiO
2 (0.013 m
−1). Interesting visible (
λ>420 nm) and UV light activity was found for ETS-10 samples incorporated with Cr and Co [ETS-10 with Cr(or)Co/Ti=0.05] and for materials synthesized by ion-exchange reactions such as Co-ETS-10 and Ag-ETS-10. All other ion-exchanged (Na,K)
2−
x
M
′
x
TiSi
5O
13 (M
′=Cr(III), Mn(II), Fe(III), Co(II), Ni(II), and Cu(II)) samples were found to be active photocatalysts that can decompose acetaldehyde under UV radiation. Materials synthesized were characterized by a variety of techniques such as powder X-ray diffraction, BET surface area and UV–VIS diffuse reflectance measurements. |
| Author | Martyanov, Igor N. Uma, Sitharaman Klabunde, Kenneth J. Rodrigues, Shalini |
| Author_xml | – sequence: 1 givenname: Sitharaman surname: Uma fullname: Uma, Sitharaman – sequence: 2 givenname: Shalini surname: Rodrigues fullname: Rodrigues, Shalini – sequence: 3 givenname: Igor N. surname: Martyanov fullname: Martyanov, Igor N. – sequence: 4 givenname: Kenneth J. surname: Klabunde fullname: Klabunde, Kenneth J. email: kenjk@ksu.edu |
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| Keywords | Ion-exchange Transition metal ETS-10 Decomposition of acetaldehyde Photocatalysis Carbon dioxide Aldehyde Porous material Acetaldehyde Heterogeneous catalysis Microporosity Ultraviolet radiation Titanium silicate Transition metal Ions Preparation Visible radiation Oxidation Gaseous phase reaction Modified material |
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| Snippet | Microporous titanium silicate [ETS-10, (Na,K)
2TiSi
5O
13] and transition metal ions incorporated titanium silicates were investigated for the photocatalytic... |
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| SubjectTerms | Chemistry Decomposition of acetaldehyde ETS-10 Exact sciences and technology General and physical chemistry Ion-exchange Photocatalysis Photochemistry Physical chemistry of induced reactions (with radiations, particles and ultrasonics) Transition metal |
| Title | Exploration of photocatalytic activities of titanosilicate ETS-10 and transition metal incorporated ETS-10 |
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