Facile water-stability evaluation of metal-organic frameworks and the property of selective removal of dyes from aqueous solution
A facile and universal method was developed to evaluate the relative water stability of porous MOFs and morphological evolution was achieved by controlling the volume ratio of DMF and H 2 O. The relative water stability of the studied MOFs is in the order HKUST-1 > MOF-505 ∼ UMCM-150 > NOTT-10...
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| Published in | Dalton transactions : an international journal of inorganic chemistry Vol. 45; no. 21; pp. 8753 - 8759 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
01.01.2016
|
| Subjects | |
| Online Access | Get full text |
| ISSN | 1477-9226 1477-9234 |
| DOI | 10.1039/c6dt00886k |
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| Abstract | A facile and universal method was developed to evaluate the relative water stability of porous MOFs and morphological evolution was achieved by controlling the volume ratio of DMF and H
2
O. The relative water stability of the studied MOFs is in the order HKUST-1 > MOF-505 ∼ UMCM-150 > NOTT-101 > DUT-23(Cu) > [Zn
2
(BPnDC)
2
(DABCO)] ∼ [Cu
3
(TPTrC)
2
(DABCO)] > MOF-5. In addition, DUT-23(Cu) [Cu
6
(BTB)
4
(BPY)
3
] (H
3
BTB = 4,4′,4′′-benzene-1,3,5-triyl-tribenzoic acid, BPY = 4,4′-bipyridine) nanoparticles obtained with a volume ratio of DMF and H
2
O of 18 : 2 show excellent adsorption capacity for methylene blue (MB) (814 mg g
−1
) with high selectivity compared with methyl orange, rhodamine B, and acid chrome blue K dyes due to the size and the electrostatic repulsion effects in aqueous solution.
A facile method was developed to evaluate the relative water stability of MOFs by controlling the volume ratio of DMF and H
2
O. |
|---|---|
| AbstractList | A facile and universal method was developed to evaluate the relative water stability of porous MOFs and morphological evolution was achieved by controlling the volume ratio of DMF and H
2
O. The relative water stability of the studied MOFs is in the order HKUST-1 > MOF-505 ∼ UMCM-150 > NOTT-101 > DUT-23(Cu) > [Zn
2
(BPnDC)
2
(DABCO)] ∼ [Cu
3
(TPTrC)
2
(DABCO)] > MOF-5. In addition, DUT-23(Cu) [Cu
6
(BTB)
4
(BPY)
3
] (H
3
BTB = 4,4′,4′′-benzene-1,3,5-triyl-tribenzoic acid, BPY = 4,4′-bipyridine) nanoparticles obtained with a volume ratio of DMF and H
2
O of 18 : 2 show excellent adsorption capacity for methylene blue (MB) (814 mg g
−1
) with high selectivity compared with methyl orange, rhodamine B, and acid chrome blue K dyes due to the size and the electrostatic repulsion effects in aqueous solution. A facile and universal method was developed to evaluate the relative water stability of porous MOFs and morphological evolution was achieved by controlling the volume ratio of DMF and H2O. The relative water stability of the studied MOFs is in the order HKUST-1 > MOF-505 ∼ UMCM-150 > NOTT-101 > DUT-23(Cu) > [Zn2(BPnDC)2(DABCO)] ∼ [Cu3(TPTrC)2(DABCO)] > MOF-5. In addition, DUT-23(Cu) [Cu6(BTB)4(BPY)3] (H3BTB = 4,4',4''-benzene-1,3,5-triyl-tribenzoic acid, BPY = 4,4'-bipyridine) nanoparticles obtained with a volume ratio of DMF and H2O of 18 : 2 show excellent adsorption capacity for methylene blue (MB) (814 mg g(-1)) with high selectivity compared with methyl orange, rhodamine B, and acid chrome blue K dyes due to the size and the electrostatic repulsion effects in aqueous solution. A facile and universal method was developed to evaluate the relative water stability of porous MOFs and morphological evolution was achieved by controlling the volume ratio of DMF and H sub(2)O. The relative water stability of the studied MOFs is in the order HKUST-1 > MOF-505 similar to UMCM-150 > NOTT-101 > DUT-23(Cu) > [Zn sub(2)(BPnDC) sub(2)(DABCO)] similar to [Cu sub(3)(TPTrC) sub(2)(DABCO)] > MOF-5. In addition, DUT-23(Cu) [Cu sub(6)(BTB) sub(4)(BPY) sub(3)] (H sub(3)BTB = 4,4',4''-benzene-1,3,5-triyl-tribenzoic acid, BPY = 4,4'-bipyridine) nanoparticles obtained with a volume ratio of DMF and H sub(2)O of 18 : 2 show excellent adsorption capacity for methylene blue (MB) (814 mg g super(-1)) with high selectivity compared with methyl orange, rhodamine B, and acid chrome blue K dyes due to the size and the electrostatic repulsion effects in aqueous solution. A facile and universal method was developed to evaluate the relative water stability of porous MOFs and morphological evolution was achieved by controlling the volume ratio of DMF and H 2 O. The relative water stability of the studied MOFs is in the order HKUST-1 > MOF-505 ∼ UMCM-150 > NOTT-101 > DUT-23(Cu) > [Zn 2 (BPnDC) 2 (DABCO)] ∼ [Cu 3 (TPTrC) 2 (DABCO)] > MOF-5. In addition, DUT-23(Cu) [Cu 6 (BTB) 4 (BPY) 3 ] (H 3 BTB = 4,4′,4′′-benzene-1,3,5-triyl-tribenzoic acid, BPY = 4,4′-bipyridine) nanoparticles obtained with a volume ratio of DMF and H 2 O of 18 : 2 show excellent adsorption capacity for methylene blue (MB) (814 mg g −1 ) with high selectivity compared with methyl orange, rhodamine B, and acid chrome blue K dyes due to the size and the electrostatic repulsion effects in aqueous solution. A facile method was developed to evaluate the relative water stability of MOFs by controlling the volume ratio of DMF and H 2 O. |
| Author | Kang, Yan-Shang Yang, Ji-Min Guo, Fan Qi, Zhao-Peng Sun, Wei-Yin |
| AuthorAffiliation | State Key Laboratory of Coordination Chemistry Huangshan University Coordination Chemistry Institute Collaborative Innovation Center of Advanced Microstructures Nanjing National Laboratory of Microstructures Nanjing University School of Chemistry and Chemical Engineering |
| AuthorAffiliation_xml | – sequence: 0 name: Nanjing National Laboratory of Microstructures – sequence: 0 name: School of Chemistry and Chemical Engineering – sequence: 0 name: Collaborative Innovation Center of Advanced Microstructures – sequence: 0 name: Coordination Chemistry Institute – sequence: 0 name: Huangshan University – sequence: 0 name: State Key Laboratory of Coordination Chemistry – sequence: 0 name: Nanjing University |
| Author_xml | – sequence: 1 givenname: Zhao-Peng surname: Qi fullname: Qi, Zhao-Peng – sequence: 2 givenname: Ji-Min surname: Yang fullname: Yang, Ji-Min – sequence: 3 givenname: Yan-Shang surname: Kang fullname: Kang, Yan-Shang – sequence: 4 givenname: Fan surname: Guo fullname: Guo, Fan – sequence: 5 givenname: Wei-Yin surname: Sun fullname: Sun, Wei-Yin |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/27139895$$D View this record in MEDLINE/PubMed |
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| SubjectTerms | Aqueous solutions Dyes Electrostatics Evolution Metal-organic frameworks Methylene blue Nanoparticles Water stability |
| Title | Facile water-stability evaluation of metal-organic frameworks and the property of selective removal of dyes from aqueous solution |
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