Interface-induced superconductivity and strain-dependent spin density waves in FeSe/SrTiO3 thin films
The record superconducting transition temperature ( T c ) for the iron-based high-temperature superconductors (Fe-HTS) has long been 56 K. Recently, in single-layer FeSe films grown on SrTiO 3 substrates, indications of a new record of 65 K have been reported. Using in situ photoemission measuremen...
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| Published in | Nature materials Vol. 12; no. 7; pp. 634 - 640 |
|---|---|
| Main Authors | , , , , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
01.07.2013
Nature Publishing Group |
| Subjects | |
| Online Access | Get full text |
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| Abstract | The record superconducting transition temperature (
T
c
) for the iron-based high-temperature superconductors (Fe-HTS) has long been 56 K. Recently, in single-layer FeSe films grown on SrTiO
3
substrates, indications of a new record of 65 K have been reported. Using
in situ
photoemission measurements, we substantiate the presence of spin density waves (SDWs) in FeSe films—a key ingredient of Fe-HTS that was missed in FeSe before—and we find that this weakens with increased thickness or reduced strain. We demonstrate that the superconductivity occurs when the electrons transferred from the oxygen-vacant substrate suppress the otherwise pronounced SDWs in single-layer FeSe. Beyond providing a comprehensive understanding of FeSe films and directions to further enhance its
T
c
, we map out the phase diagram of FeSe as a function of lattice constant, which contains all the essential physics of Fe-HTS. With the simplest structure, cleanest composition and single tuning parameter, monolayer FeSe is an ideal system for testing theories of Fe-HTS.
Iron pnictide superconductors represent a suggestive alternative to cuprate superconductors for achieving high transition temperatures. Using
in situ
angle-resolved photoemission spectroscopy, the electronic properties of FeSe are examined as a function of film thickness, providing valuable insights into the mechanism driving the superconductivity in this material. |
|---|---|
| AbstractList | The record superconducting transition temperature (Tc) for the iron-based high-temperature superconductors (Fe-HTS) has long been 56K. Recently, in single-layer FeSe films grown on SrTiO3 substrates, indications of a new record of 65K have been reported. Using in situ photoemission measurements, we substantiate the presence of spin density waves (SDWs) in FeSe films-a key ingredient of Fe-HTS that was missed in FeSe before-and we find that this weakens with increased thickness or reduced strain. We demonstrate that the superconductivity occurs when the electrons transferred from the oxygen-vacant substrate suppress the otherwise pronounced SDWs in single-layer FeSe. Beyond providing a comprehensive understanding of FeSe films and directions to further enhance its Tc, we map out the phase diagram of FeSe as a function of lattice constant, which contains all the essential physics of Fe-HTS. With the simplest structure, cleanest composition and single tuning parameter, monolayer FeSe is an ideal system for testing theories of Fe-HTS. The record superconducting transition temperature (T(c)) for the iron-based high-temperature superconductors (Fe-HTS) has long been 56 K. Recently, in single-layer FeSe films grown on SrTiO3 substrates, indications of a new record of 65 K have been reported. Using in situ photoemission measurements, we substantiate the presence of spin density waves (SDWs) in FeSe films--a key ingredient of Fe-HTS that was missed in FeSe before--and we find that this weakens with increased thickness or reduced strain. We demonstrate that the superconductivity occurs when the electrons transferred from the oxygen-vacant substrate suppress the otherwise pronounced SDWs in single-layer FeSe. Beyond providing a comprehensive understanding of FeSe films and directions to further enhance its T(c), we map out the phase diagram of FeSe as a function of lattice constant, which contains all the essential physics of Fe-HTS. With the simplest structure, cleanest composition and single tuning parameter, monolayer FeSe is an ideal system for testing theories of Fe-HTS. The record superconducting transition temperature ( T c ) for the iron-based high-temperature superconductors (Fe-HTS) has long been 56 K. Recently, in single-layer FeSe films grown on SrTiO 3 substrates, indications of a new record of 65 K have been reported. Using in situ photoemission measurements, we substantiate the presence of spin density waves (SDWs) in FeSe films—a key ingredient of Fe-HTS that was missed in FeSe before—and we find that this weakens with increased thickness or reduced strain. We demonstrate that the superconductivity occurs when the electrons transferred from the oxygen-vacant substrate suppress the otherwise pronounced SDWs in single-layer FeSe. Beyond providing a comprehensive understanding of FeSe films and directions to further enhance its T c , we map out the phase diagram of FeSe as a function of lattice constant, which contains all the essential physics of Fe-HTS. With the simplest structure, cleanest composition and single tuning parameter, monolayer FeSe is an ideal system for testing theories of Fe-HTS. Iron pnictide superconductors represent a suggestive alternative to cuprate superconductors for achieving high transition temperatures. Using in situ angle-resolved photoemission spectroscopy, the electronic properties of FeSe are examined as a function of film thickness, providing valuable insights into the mechanism driving the superconductivity in this material. The record superconducting transition temperature (T(c)) for the iron-based high-temperature superconductors (Fe-HTS) has long been 56 K. Recently, in single-layer FeSe films grown on SrTiO3 substrates, indications of a new record of 65 K have been reported. Using in situ photoemission measurements, we substantiate the presence of spin density waves (SDWs) in FeSe films--a key ingredient of Fe-HTS that was missed in FeSe before--and we find that this weakens with increased thickness or reduced strain. We demonstrate that the superconductivity occurs when the electrons transferred from the oxygen-vacant substrate suppress the otherwise pronounced SDWs in single-layer FeSe. Beyond providing a comprehensive understanding of FeSe films and directions to further enhance its T(c), we map out the phase diagram of FeSe as a function of lattice constant, which contains all the essential physics of Fe-HTS. With the simplest structure, cleanest composition and single tuning parameter, monolayer FeSe is an ideal system for testing theories of Fe-HTS.The record superconducting transition temperature (T(c)) for the iron-based high-temperature superconductors (Fe-HTS) has long been 56 K. Recently, in single-layer FeSe films grown on SrTiO3 substrates, indications of a new record of 65 K have been reported. Using in situ photoemission measurements, we substantiate the presence of spin density waves (SDWs) in FeSe films--a key ingredient of Fe-HTS that was missed in FeSe before--and we find that this weakens with increased thickness or reduced strain. We demonstrate that the superconductivity occurs when the electrons transferred from the oxygen-vacant substrate suppress the otherwise pronounced SDWs in single-layer FeSe. Beyond providing a comprehensive understanding of FeSe films and directions to further enhance its T(c), we map out the phase diagram of FeSe as a function of lattice constant, which contains all the essential physics of Fe-HTS. With the simplest structure, cleanest composition and single tuning parameter, monolayer FeSe is an ideal system for testing theories of Fe-HTS. |
| Author | Jiang, Juan Chen, Fei Peng, Rui Xu, Haichao Tan, Shiyong Lai, Xinchun Xiang, Tao Fan, Qin Hu, Jiangping Feng, Donglai Ye, Zirong Xia, Miao Xu, Difei Zhang, Tong Xie, Binping Zhang, Yan Xie, Xin |
| Author_xml | – sequence: 1 givenname: Shiyong surname: Tan fullname: Tan, Shiyong organization: Department of Physics, State Key Laboratory of Surface Physics, and Advanced Materials Laboratory, Fudan University, China Academy of Engineering Physics – sequence: 2 givenname: Yan surname: Zhang fullname: Zhang, Yan organization: Department of Physics, State Key Laboratory of Surface Physics, and Advanced Materials Laboratory, Fudan University – sequence: 3 givenname: Miao surname: Xia fullname: Xia, Miao organization: Department of Physics, State Key Laboratory of Surface Physics, and Advanced Materials Laboratory, Fudan University – sequence: 4 givenname: Zirong surname: Ye fullname: Ye, Zirong organization: Department of Physics, State Key Laboratory of Surface Physics, and Advanced Materials Laboratory, Fudan University – sequence: 5 givenname: Fei surname: Chen fullname: Chen, Fei organization: Department of Physics, State Key Laboratory of Surface Physics, and Advanced Materials Laboratory, Fudan University – sequence: 6 givenname: Xin surname: Xie fullname: Xie, Xin organization: Department of Physics, State Key Laboratory of Surface Physics, and Advanced Materials Laboratory, Fudan University – sequence: 7 givenname: Rui surname: Peng fullname: Peng, Rui organization: Department of Physics, State Key Laboratory of Surface Physics, and Advanced Materials Laboratory, Fudan University – sequence: 8 givenname: Difei surname: Xu fullname: Xu, Difei organization: Department of Physics, State Key Laboratory of Surface Physics, and Advanced Materials Laboratory, Fudan University – sequence: 9 givenname: Qin surname: Fan fullname: Fan, Qin organization: Department of Physics, State Key Laboratory of Surface Physics, and Advanced Materials Laboratory, Fudan University – sequence: 10 givenname: Haichao surname: Xu fullname: Xu, Haichao organization: Department of Physics, State Key Laboratory of Surface Physics, and Advanced Materials Laboratory, Fudan University – sequence: 11 givenname: Juan surname: Jiang fullname: Jiang, Juan organization: Department of Physics, State Key Laboratory of Surface Physics, and Advanced Materials Laboratory, Fudan University – sequence: 12 givenname: Tong surname: Zhang fullname: Zhang, Tong organization: Department of Physics, State Key Laboratory of Surface Physics, and Advanced Materials Laboratory, Fudan University – sequence: 13 givenname: Xinchun surname: Lai fullname: Lai, Xinchun organization: China Academy of Engineering Physics – sequence: 14 givenname: Tao surname: Xiang fullname: Xiang, Tao organization: Institute of Physics, Chinese Academy of Sciences – sequence: 15 givenname: Jiangping surname: Hu fullname: Hu, Jiangping organization: Institute of Physics, Chinese Academy of Sciences – sequence: 16 givenname: Binping surname: Xie fullname: Xie, Binping organization: Department of Physics, State Key Laboratory of Surface Physics, and Advanced Materials Laboratory, Fudan University – sequence: 17 givenname: Donglai surname: Feng fullname: Feng, Donglai email: dlfeng@fudan.edu.cn organization: Department of Physics, State Key Laboratory of Surface Physics, and Advanced Materials Laboratory, Fudan University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/23708327$$D View this record in MEDLINE/PubMed |
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| Snippet | The record superconducting transition temperature (
T
c
) for the iron-based high-temperature superconductors (Fe-HTS) has long been 56 K. Recently, in... The record superconducting transition temperature (T(c)) for the iron-based high-temperature superconductors (Fe-HTS) has long been 56 K. Recently, in... The record superconducting transition temperature (Tc) for the iron-based high-temperature superconductors (Fe-HTS) has long been 56K. Recently, in... |
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| SubjectTerms | 639/301/119/1003 639/301/119/544 Biomaterials Condensed Matter Physics Density High temperature Interfaces Materials Science Nanotechnology Optical and Electronic Materials Physics Strain rate Substrates Superconductivity Thin films Transition temperatures |
| Title | Interface-induced superconductivity and strain-dependent spin density waves in FeSe/SrTiO3 thin films |
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