Defect engineering in Boron Nitride for catalysis
Catalytic processes are critical steps in numerous industrial processes. The discovery of high reactivity of defects in metal-free two-dimensional materials has bolstered their emergence as catalysts. Here we consider the effect of defect-inducing methods in hexagonal boron nitride (h-BN) on their p...
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| Published in | MRS communications Vol. 8; no. 3; pp. 1236 - 1243 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
New York, USA
Cambridge University Press
01.09.2018
Springer International Publishing |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Catalytic processes are critical steps in numerous industrial processes. The discovery of high reactivity of defects in metal-free two-dimensional materials has bolstered their emergence as catalysts. Here we consider the effect of defect-inducing methods in hexagonal boron nitride (h-BN) on their performance for olefin and CO2 hydrogenation. We compare the changes introduced by ball milling and heat treatment in h-BN and show how varying the treatment conditions can impact the properties. We provide some evidence of the reactivity of the powders. Our results highlight how characterization can be exploited to assess the potential catalytic activity of h-BN for heterogeneous catalysis. |
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| AbstractList | Catalytic processes are critical steps in numerous industrial processes. The discovery of high reactivity of defects in metal-free two-dimensional materials has bolstered their emergence as catalysts. Here we consider the effect of defect-inducing methods in hexagonal boron nitride (h-BN) on their performance for olefin and CO2 hydrogenation. We compare the changes introduced by ball milling and heat treatment in h-BN and show how varying the treatment conditions can impact the properties. We provide some evidence of the reactivity of the powders. Our results highlight how characterization can be exploited to assess the potential catalytic activity of h-BN for heterogeneous catalysis. Catalytic processes are critical steps in numerous industrial processes. The discovery of high reactivity of defects in metal-free two-dimensional materials has bolstered their emergence as catalysts. Here we consider the effect of defect-inducing methods in hexagonal boron nitride ( h -BN) on their performance for olefin and CO 2 hydrogenation. We compare the changes introduced by ball milling and heat treatment in h -BN and show how varying the treatment conditions can impact the properties. We provide some evidence of the reactivity of the powders. Our results highlight how characterization can be exploited to assess the potential catalytic activity of h -BN for heterogeneous catalysis. |
| Author | Ding, Yi Tetard, Laurene Nash, David Khater, Ahmad Blair, Richard Torres-Davila, Fernand |
| Author_xml | – sequence: 1 givenname: Yi surname: Ding fullname: Ding, Yi organization: NanoScience Technology Center, University of Central Florida, 12424 Research Parkway, Orlando, FL 32826, USA – sequence: 2 givenname: Fernand surname: Torres-Davila fullname: Torres-Davila, Fernand organization: NanoScience Technology Center, University of Central Florida, 12424 Research Parkway, Orlando, FL 32826, USA – sequence: 3 givenname: Ahmad surname: Khater fullname: Khater, Ahmad organization: NanoScience Technology Center, University of Central Florida, 12424 Research Parkway, Orlando, FL 32826, USA – sequence: 4 givenname: David surname: Nash fullname: Nash, David organization: Physics Department, University of Central Florida, 4111 Libra Drive, Orlando, FL 32816, USA – sequence: 5 givenname: Richard surname: Blair fullname: Blair, Richard organization: Florida Space Institute, University of Central Florida, 4111 Libra Drive, Orlando, FL 32816, USA – sequence: 6 givenname: Laurene surname: Tetard fullname: Tetard, Laurene email: Laurene.Tetard@ucf.edu organization: NanoScience Technology Center, University of Central Florida, 12424 Research Parkway, Orlando, FL 32826, USA |
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| SubjectTerms | Ball milling Biomaterials Boron Boron nitride Catalysis Catalytic activity Characterization and Evaluation of Materials Defects Heat treatment Hydrogenation Mass spectrometry Materials Engineering Materials Science Metal oxides Microscopy Nanotechnology Nitrogen NMR Nuclear magnetic resonance Plasma etching Polymer Sciences Research Letter Research Letters Scientific imaging Studies |
| Title | Defect engineering in Boron Nitride for catalysis |
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