Concentration- and temperature- dependent luminescence quenching and optical transition of Sr2GdTaO6: Eu3+ phosphor for potential applications in white LEDs

•Novel Sr2GdTaO6: Eu3+ phosphors with double perovskite structure were successfully prepared.•Effective red luminescence emission was observed in Sr2GdTaO6: Eu3+ phosphors.•Effects of the Eu3+ doping concentration on luminescence properties were investigated in detail.•Possible mechanism for the inf...

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Published inResults in physics Vol. 56; p. 107238
Main Authors Wang, Li, Zhang, Yuhang, Gao, Duan, Sha, Xuezhu, Chen, Xin, Zhang, Yanqiu, Zhang, Jinsu, Zhang, Xizhen, Cao, Yongze, Wang, Yichao, Li, Xiangping, Xu, Sai, Yu, Hongquan, Chen, Baojiu
Format Journal Article
LanguageEnglish
Published Elsevier B.V 01.01.2024
Elsevier
Subjects
Concentration quenching
Eu3
Judd-Ofelt analysis
Sr2GdTaO6
Thermal quenching
Judd-Ofelt analysis
Eu3
Sr2GdTaO6
Thermal quenching
Concentration quenching
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Abstract •Novel Sr2GdTaO6: Eu3+ phosphors with double perovskite structure were successfully prepared.•Effective red luminescence emission was observed in Sr2GdTaO6: Eu3+ phosphors.•Effects of the Eu3+ doping concentration on luminescence properties were investigated in detail.•Possible mechanism for the influence of temperature on thermal quenching was discussed.•Optical transitive properties were evaluated using the Judd-Ofelt theory. A series of Eu3+ doped Sr2GdTaO6 (SGT) phosphors with double perovskite structure were synthesized via a high-temperature solid-state reaction approach. The crystal structure, morphology and luminescence properties were characterized by means of X-ray diffraction, transmission electron microscope, luminescence spectroscopy and fluorescence decay lifetimes, respectively. Under the excitation of 394 nm, intense red emission in the visible region was observed in Eu3+ doped SGT phosphors, and the critical quenching concentration of Eu3+ in SGT phosphors was derived to be 15 mol%. The chromaticity coordinates and color purity of SGT: 15 mol% Eu3+ were calculated to be (0.61, 0.36) an 93.82 %, respectively. Meanwhile, it was also confirmed that the electric quadrupole–quadrupole interaction is responsible for the luminescence concentration quenching of Eu3+. The internal quantum efficiency of SGT: Eu3+ phosphors with different Eu3+ concentrations were calculated. Furthermore, the crossover process was confirmed to be the main mechanism for luminescence thermal quenching based on the temperature-dependent emission spectra and temperature-dependent fluorescence lifetimes. In addition, the Judd-Ofelt parameters, radiative transition rates and branch ratios from the 5D0 emitting states to various lower energy states were evaluated with the aid of the Judd-Ofelt theory, respectively. All results indicate that SGT: Eu3+ samples are a promising red-emitting phosphor.
AbstractList •Novel Sr2GdTaO6: Eu3+ phosphors with double perovskite structure were successfully prepared.•Effective red luminescence emission was observed in Sr2GdTaO6: Eu3+ phosphors.•Effects of the Eu3+ doping concentration on luminescence properties were investigated in detail.•Possible mechanism for the influence of temperature on thermal quenching was discussed.•Optical transitive properties were evaluated using the Judd-Ofelt theory. A series of Eu3+ doped Sr2GdTaO6 (SGT) phosphors with double perovskite structure were synthesized via a high-temperature solid-state reaction approach. The crystal structure, morphology and luminescence properties were characterized by means of X-ray diffraction, transmission electron microscope, luminescence spectroscopy and fluorescence decay lifetimes, respectively. Under the excitation of 394 nm, intense red emission in the visible region was observed in Eu3+ doped SGT phosphors, and the critical quenching concentration of Eu3+ in SGT phosphors was derived to be 15 mol%. The chromaticity coordinates and color purity of SGT: 15 mol% Eu3+ were calculated to be (0.61, 0.36) an 93.82 %, respectively. Meanwhile, it was also confirmed that the electric quadrupole–quadrupole interaction is responsible for the luminescence concentration quenching of Eu3+. The internal quantum efficiency of SGT: Eu3+ phosphors with different Eu3+ concentrations were calculated. Furthermore, the crossover process was confirmed to be the main mechanism for luminescence thermal quenching based on the temperature-dependent emission spectra and temperature-dependent fluorescence lifetimes. In addition, the Judd-Ofelt parameters, radiative transition rates and branch ratios from the 5D0 emitting states to various lower energy states were evaluated with the aid of the Judd-Ofelt theory, respectively. All results indicate that SGT: Eu3+ samples are a promising red-emitting phosphor.
A series of Eu3+ doped Sr2GdTaO6 (SGT) phosphors with double perovskite structure were synthesized via a high-temperature solid-state reaction approach. The crystal structure, morphology and luminescence properties were characterized by means of X-ray diffraction, transmission electron microscope, luminescence spectroscopy and fluorescence decay lifetimes, respectively. Under the excitation of 394 nm, intense red emission in the visible region was observed in Eu3+ doped SGT phosphors, and the critical quenching concentration of Eu3+ in SGT phosphors was derived to be 15 mol%. The chromaticity coordinates and color purity of SGT: 15 mol% Eu3+ were calculated to be (0.61, 0.36) an 93.82 %, respectively. Meanwhile, it was also confirmed that the electric quadrupole–quadrupole interaction is responsible for the luminescence concentration quenching of Eu3+. The internal quantum efficiency of SGT: Eu3+ phosphors with different Eu3+ concentrations were calculated. Furthermore, the crossover process was confirmed to be the main mechanism for luminescence thermal quenching based on the temperature-dependent emission spectra and temperature-dependent fluorescence lifetimes. In addition, the Judd-Ofelt parameters, radiative transition rates and branch ratios from the 5D0 emitting states to various lower energy states were evaluated with the aid of the Judd-Ofelt theory, respectively. All results indicate that SGT: Eu3+ samples are a promising red-emitting phosphor.
ArticleNumber 107238
Author Wang, Li
Chen, Baojiu
Zhang, Yanqiu
Zhang, Xizhen
Xu, Sai
Sha, Xuezhu
Chen, Xin
Yu, Hongquan
Zhang, Jinsu
Wang, Yichao
Zhang, Yuhang
Li, Xiangping
Cao, Yongze
Gao, Duan
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Keywords Judd-Ofelt analysis
Eu3
Sr2GdTaO6
Thermal quenching
Concentration quenching
Language English
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SSID ssj0001645511
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Snippet •Novel Sr2GdTaO6: Eu3+ phosphors with double perovskite structure were successfully prepared.•Effective red luminescence emission was observed in Sr2GdTaO6:...
A series of Eu3+ doped Sr2GdTaO6 (SGT) phosphors with double perovskite structure were synthesized via a high-temperature solid-state reaction approach. The...
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StartPage 107238
SubjectTerms Concentration quenching
Eu3
Judd-Ofelt analysis
Sr2GdTaO6
Thermal quenching
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Title Concentration- and temperature- dependent luminescence quenching and optical transition of Sr2GdTaO6: Eu3+ phosphor for potential applications in white LEDs
URI https://dx.doi.org/10.1016/j.rinp.2023.107238
https://doaj.org/article/8a261c3d1a274a62b32a4f230f179d8c
Volume 56
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