Interfacial dominated ferromagnetism in nanograined ZnO: a μSR and DFT study

Diamagnetic oxides can, under certain conditions, become ferromagnetic at room temperature and therefore are promising candidates for future material in spintronic devices. Contrary to early predictions, doping ZnO with uniformly distributed magnetic ions is not essential to obtain ferromagnetic sam...

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Published inScientific reports Vol. 5; no. 1; p. 8871
Main Authors Tietze, Thomas, Audehm, Patrick, Chen, Yu–Chun, Schütz, Gisela, Straumal, Boris B., Protasova, Svetlana G., Mazilkin, Andrey A., Straumal, Petr B., Prokscha, Thomas, Luetkens, Hubertus, Salman, Zaher, Suter, Andreas, Baretzky, Brigitte, Fink, Karin, Wenzel, Wolfgang, Danilov, Denis, Goering, Eberhard
Format Journal Article
LanguageEnglish
Published London Nature Publishing Group UK 09.03.2015
Nature Publishing Group
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147/143
639/301/357/354
639/301/357/997
639/925/357/995
639/925/357/997
Humanities and Social Sciences
multidisciplinary
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Abstract Diamagnetic oxides can, under certain conditions, become ferromagnetic at room temperature and therefore are promising candidates for future material in spintronic devices. Contrary to early predictions, doping ZnO with uniformly distributed magnetic ions is not essential to obtain ferromagnetic samples. Instead, the nanostructure seems to play the key role, as room temperature ferromagnetism was also found in nanograined, undoped ZnO. However, the origin of room temperature ferromagnetism in primarily non–magnetic oxides like ZnO is still unexplained and a controversial subject within the scientific community. Using low energy muon spin relaxation in combination with SQUID and TEM techniques, we demonstrate that the magnetic volume fraction is strongly related to the sample volume fraction occupied by grain boundaries. With molecular dynamics and density functional theory we find ferromagnetic coupled electron states in ZnO grain boundaries. Our results provide evidence and a microscopic model for room temperature ferromagnetism in oxides.
AbstractList Diamagnetic oxides can, under certain conditions, become ferromagnetic at room temperature and therefore are promising candidates for future material in spintronic devices. Contrary to early predictions, doping ZnO with uniformly distributed magnetic ions is not essential to obtain ferromagnetic samples. Instead, the nanostructure seems to play the key role, as room temperature ferromagnetism was also found in nanograined, undoped ZnO. However, the origin of room temperature ferromagnetism in primarily non-magnetic oxides like ZnO is still unexplained and a controversial subject within the scientific community. Using low energy muon spin relaxation in combination with SQUID and TEM techniques, we demonstrate that the magnetic volume fraction is strongly related to the sample volume fraction occupied by grain boundaries. With molecular dynamics and density functional theory we find ferromagnetic coupled electron states in ZnO grain boundaries. Our results provide evidence and a microscopic model for room temperature ferromagnetism in oxides.Diamagnetic oxides can, under certain conditions, become ferromagnetic at room temperature and therefore are promising candidates for future material in spintronic devices. Contrary to early predictions, doping ZnO with uniformly distributed magnetic ions is not essential to obtain ferromagnetic samples. Instead, the nanostructure seems to play the key role, as room temperature ferromagnetism was also found in nanograined, undoped ZnO. However, the origin of room temperature ferromagnetism in primarily non-magnetic oxides like ZnO is still unexplained and a controversial subject within the scientific community. Using low energy muon spin relaxation in combination with SQUID and TEM techniques, we demonstrate that the magnetic volume fraction is strongly related to the sample volume fraction occupied by grain boundaries. With molecular dynamics and density functional theory we find ferromagnetic coupled electron states in ZnO grain boundaries. Our results provide evidence and a microscopic model for room temperature ferromagnetism in oxides.
Diamagnetic oxides can, under certain conditions, become ferromagnetic at room temperature and therefore are promising candidates for future material in spintronic devices. Contrary to early predictions, doping ZnO with uniformly distributed magnetic ions is not essential to obtain ferromagnetic samples. Instead, the nanostructure seems to play the key role, as room temperature ferromagnetism was also found in nanograined, undoped ZnO. However, the origin of room temperature ferromagnetism in primarily non–magnetic oxides like ZnO is still unexplained and a controversial subject within the scientific community. Using low energy muon spin relaxation in combination with SQUID and TEM techniques, we demonstrate that the magnetic volume fraction is strongly related to the sample volume fraction occupied by grain boundaries. With molecular dynamics and density functional theory we find ferromagnetic coupled electron states in ZnO grain boundaries. Our results provide evidence and a microscopic model for room temperature ferromagnetism in oxides.
ArticleNumber 8871
Author Luetkens, Hubertus
Mazilkin, Andrey A.
Schütz, Gisela
Prokscha, Thomas
Fink, Karin
Chen, Yu–Chun
Straumal, Boris B.
Suter, Andreas
Wenzel, Wolfgang
Audehm, Patrick
Straumal, Petr B.
Goering, Eberhard
Protasova, Svetlana G.
Salman, Zaher
Baretzky, Brigitte
Danilov, Denis
Tietze, Thomas
Author_xml – sequence: 1
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  surname: Tietze
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  surname: Audehm
  fullname: Audehm, Patrick
  organization: Max-Planck-Institute for Intelligent Systems
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  givenname: Yu–Chun
  surname: Chen
  fullname: Chen, Yu–Chun
  organization: Max-Planck-Institute for Intelligent Systems
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  givenname: Gisela
  surname: Schütz
  fullname: Schütz, Gisela
  organization: Max-Planck-Institute for Intelligent Systems
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  givenname: Boris B.
  surname: Straumal
  fullname: Straumal, Boris B.
  organization: Moscow Institute of Physics and Technology (State University), Institute of Solid State Physics, Russian Academy of Sciences, National Research Technological University “MISiS”, Karlsruhe Institute of Technology, Institute of Nanotechnology
– sequence: 6
  givenname: Svetlana G.
  surname: Protasova
  fullname: Protasova, Svetlana G.
  organization: Institute of Solid State Physics, Russian Academy of Sciences
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  givenname: Andrey A.
  surname: Mazilkin
  fullname: Mazilkin, Andrey A.
  organization: Institute of Solid State Physics, Russian Academy of Sciences, Karlsruhe Institute of Technology, Institute of Nanotechnology
– sequence: 8
  givenname: Petr B.
  surname: Straumal
  fullname: Straumal, Petr B.
  organization: National Research Technological University “MISiS”, A.A. Baikov Institute of Metallurgy and Materials Science RAS
– sequence: 9
  givenname: Thomas
  surname: Prokscha
  fullname: Prokscha, Thomas
  organization: Laboratory for Muon Spin Spectroscopy, Paul Scherrer Institut
– sequence: 10
  givenname: Hubertus
  surname: Luetkens
  fullname: Luetkens, Hubertus
  organization: Laboratory for Muon Spin Spectroscopy, Paul Scherrer Institut
– sequence: 11
  givenname: Zaher
  surname: Salman
  fullname: Salman, Zaher
  organization: Laboratory for Muon Spin Spectroscopy, Paul Scherrer Institut
– sequence: 12
  givenname: Andreas
  surname: Suter
  fullname: Suter, Andreas
  organization: Laboratory for Muon Spin Spectroscopy, Paul Scherrer Institut
– sequence: 13
  givenname: Brigitte
  surname: Baretzky
  fullname: Baretzky, Brigitte
  organization: Karlsruhe Institute of Technology, Institute of Nanotechnology
– sequence: 14
  givenname: Karin
  surname: Fink
  fullname: Fink, Karin
  organization: Karlsruhe Institute of Technology, Institute of Nanotechnology
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  surname: Wenzel
  fullname: Wenzel, Wolfgang
  organization: Karlsruhe Institute of Technology, Institute of Nanotechnology
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  surname: Danilov
  fullname: Danilov, Denis
  organization: Karlsruhe Institute of Technology, Institute of Nanotechnology
– sequence: 17
  givenname: Eberhard
  surname: Goering
  fullname: Goering, Eberhard
  organization: Max-Planck-Institute for Intelligent Systems
BackLink https://www.ncbi.nlm.nih.gov/pubmed/25747456$$D View this record in MEDLINE/PubMed
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Snippet Diamagnetic oxides can, under certain conditions, become ferromagnetic at room temperature and therefore are promising candidates for future material in...
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Title Interfacial dominated ferromagnetism in nanograined ZnO: a μSR and DFT study
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