A photocatalytic degradation self-cleaning composite membrane for oil-water separation inspired by light-trapping effect of moth-eye
Membrane separation technology with superwetting surfaces is ideal for treating water pollution. However, the fouling problem of membranes limits their practical application in this field. Membranes with self-cleaning property during the separation are the key to solve this problem. In this study, i...
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| Published in | Journal of membrane science Vol. 669; p. 121337 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
05.03.2023
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Membrane separation technology with superwetting surfaces is ideal for treating water pollution. However, the fouling problem of membranes limits their practical application in this field. Membranes with self-cleaning property during the separation are the key to solve this problem. In this study, inspired by the light-trapping effect of the moth-eye, a kind of composite membrane with efficient self-cleaning by photocatalytic degradation was proposed. The composite membrane is based on polyvinyl alcohol cross-linked tannic acid (PVA-TA) and its photocatalytic function is achieved by doping magnetic titanium dioxide nanoparticles (MTiO2) as well as MXene. Meanwhile, its surface was constructed by magnetically controlled self-assembly method using MTiO2 to mimic the moth-eye structure. The composite membrane has superhydrophilic/underwater superoleophobic, excellent oil-water separation efficiency (99.85%) and long service life (64 cycles). In addition, due to the light-trapping effect of the bionic moth-eye structure and the redox reaction at the interface of MTiO2-MXene composites under sunlight irradiation, the membrane can achieve efficient and convenient photocatalytic degradation self-cleaning by sunlight irradiation. This study will provide new insights into the self-cleaning method of oil-water separation materials.
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•Construction of high light absorption efficiency surface by magnetron self-assembly method inspired by the light-trapping effect of moth-eye structure.•Redox reaction occur at the interface of MTiO2 and MXene composite under sunlight irradiation.•The composite membrane shows excellent oil-water separation performance and long service life.•The composite membrane has excellent sunlight-catalyzed degradation self-cleaning property. |
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| AbstractList | Membrane separation technology with superwetting surfaces is ideal for treating water pollution. However, the fouling problem of membranes limits their practical application in this field. Membranes with self-cleaning property during the separation are the key to solve this problem. In this study, inspired by the light-trapping effect of the moth-eye, a kind of composite membrane with efficient self-cleaning by photocatalytic degradation was proposed. The composite membrane is based on polyvinyl alcohol cross-linked tannic acid (PVA-TA) and its photocatalytic function is achieved by doping magnetic titanium dioxide nanoparticles (MTiO2) as well as MXene. Meanwhile, its surface was constructed by magnetically controlled self-assembly method using MTiO2 to mimic the moth-eye structure. The composite membrane has superhydrophilic/underwater superoleophobic, excellent oil-water separation efficiency (99.85%) and long service life (64 cycles). In addition, due to the light-trapping effect of the bionic moth-eye structure and the redox reaction at the interface of MTiO2-MXene composites under sunlight irradiation, the membrane can achieve efficient and convenient photocatalytic degradation self-cleaning by sunlight irradiation. This study will provide new insights into the self-cleaning method of oil-water separation materials.
[Display omitted]
•Construction of high light absorption efficiency surface by magnetron self-assembly method inspired by the light-trapping effect of moth-eye structure.•Redox reaction occur at the interface of MTiO2 and MXene composite under sunlight irradiation.•The composite membrane shows excellent oil-water separation performance and long service life.•The composite membrane has excellent sunlight-catalyzed degradation self-cleaning property. Membrane separation technology with superwetting surfaces is ideal for treating water pollution. However, the fouling problem of membranes limits their practical application in this field. Membranes with self-cleaning property during the separation are the key to solve this problem. In this study, inspired by the light-trapping effect of the moth-eye, a kind of composite membrane with efficient self-cleaning by photocatalytic degradation was proposed. The composite membrane is based on polyvinyl alcohol cross-linked tannic acid (PVA-TA) and its photocatalytic function is achieved by doping magnetic titanium dioxide nanoparticles (MTiO₂) as well as MXene. Meanwhile, its surface was constructed by magnetically controlled self-assembly method using MTiO₂ to mimic the moth-eye structure. The composite membrane has superhydrophilic/underwater superoleophobic, excellent oil-water separation efficiency (99.85%) and long service life (64 cycles). In addition, due to the light-trapping effect of the bionic moth-eye structure and the redox reaction at the interface of MTiO₂-MXene composites under sunlight irradiation, the membrane can achieve efficient and convenient photocatalytic degradation self-cleaning by sunlight irradiation. This study will provide new insights into the self-cleaning method of oil-water separation materials. |
| ArticleNumber | 121337 |
| Author | Li, Zhaoxin Jiang, Shuyue Yin, Liang Zhang, Haifeng Chen, Liang Sang, Shengtian |
| Author_xml | – sequence: 1 givenname: Zhaoxin surname: Li fullname: Li, Zhaoxin email: 21B921018@stu.hit.edu.cn organization: MEMS Center, Harbin Institute of Technology, Harbin, 150001, PR China – sequence: 2 givenname: Liang surname: Yin fullname: Yin, Liang email: yinliang2003@126.com organization: MEMS Center, Harbin Institute of Technology, Harbin, 150001, PR China – sequence: 3 givenname: Shuyue surname: Jiang fullname: Jiang, Shuyue email: jiangshuyue@163.com organization: MEMS Center, Harbin Institute of Technology, Harbin, 150001, PR China – sequence: 4 givenname: Liang surname: Chen fullname: Chen, Liang email: cliang@hit.edu.cn organization: MEMS Center, Harbin Institute of Technology, Harbin, 150001, PR China – sequence: 5 givenname: Shengtian surname: Sang fullname: Sang, Shengtian email: stsang@hit.edu.cn organization: MEMS Center, Harbin Institute of Technology, Harbin, 150001, PR China – sequence: 6 givenname: Haifeng surname: Zhang fullname: Zhang, Haifeng email: zhanghf@hit.edu.cn organization: MEMS Center, Harbin Institute of Technology, Harbin, 150001, PR China |
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| Keywords | Oil-water separation Photocatalytic degradation Self-cleaning Light-trapping Redox reaction |
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| SubjectTerms | asymmetric membranes crosslinking durability hydrophilicity irradiation Light-trapping magnetism nanoparticles Oil-water separation photocatalysis Photocatalytic degradation polyvinyl alcohol Redox reaction redox reactions Self-cleaning solar radiation tannins titanium dioxide water pollution |
| Title | A photocatalytic degradation self-cleaning composite membrane for oil-water separation inspired by light-trapping effect of moth-eye |
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